期刊
ENERGY & FUELS
卷 37, 期 23, 页码 18441-18455出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.energyfuels.3c03057
关键词
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Magnesium-based batteries have emerged as an alternative to conventional lithium-ion batteries due to the use of magnesium metal anodes with high theoretical specific capacity, abundant reserves, and low cost. However, the lack of high-energy cathode materials remains a major hindrance to their application.
Due to the use of magnesium metal anodes with high theoretical specific capacity, abundant reserves, and low cost, magnesium-based batteries have become one of the alternatives to conventional lithium-ion batteries. Although significant progress in reversible magnesium deposition of the magnesium anode and efficient Mg-ion transport of the electrolytes has been achieved, the application of magnesium-based batteries is still greatly hindered by the lack of high-energy cathode materials. The metal-chalcogenide cathode materials with dual-redox centers (i.e., the redox of both the cation and anion) may offer high capacity and could be good candidates for achieving high-energy electrode couples using the magnesium metal anode. This review aims to highlight the recent progress on these cathode materials for magnesium batteries and hybrid-cation batteries using the magnesium metal anode. The perspectives and challenges for the future development of these cathode materials are analyzed.
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