☆ 4.7 Review

Application and development of zero-valent iron (ZVI)-based materials for environmental remediation: A scientometric and visualization analysis

ENVIRONMENTAL RESEARCH (2024)

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Hao Cheng et al.

Summary: Commercial molybdenum carbide (Mo2C) and ferrous iron (Fe2+) were investigated as co-catalysts for the activation of H2O2 in the treatment of organic contaminants. The presence of Mo2C effectively decomposed H2O2 and accelerated the conversion of Fe3+/Fe2+ compared to traditional Fenton process. Mo2C/Fe2+/H2O2 exhibited a significantly higher catalytic reactivity than MoS2, and the degradation rate constant of Rhodamine B in Mo2C/Fe2+/H2O2 was three times higher than that in Fe2+/H2O2. XPS analysis showed that Mo(II) and Mo(IV) played major roles in Fe3+ reduction, and EPR analysis confirmed the involvement of .OH, O-2(-), and O-1(2) in Mo2C/Fe2+/H2O2. ECOSAR toxicity assessment revealed a decrease in the toxicity of RhB degradation products after treatment. Overall, this study presents a promising Mo2C co-catalyzed Fenton process for efficient abatement of organic contaminants.

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Article Environmental Sciences

Molybdenum disulfide co-catalysis boosting nanoscale zero-valent iron based Fenton-like process: Performance and mechanism

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Summary: In this study, molybdenum sulfide (MoS2) was used as a co-catalyst to enhance the performance of the nanoscale zero-valent iron (nZVI) based Fenton-like process for Rhodamine B (RhB) degradation. The addition of MoS2 significantly accelerated H2O2 decomposition and increased the RhB degradation rate constant compared to the conventional Fenton process. Furthermore, the effective pH range was expanded to 9.0 with a high removal rate of RhB. The MoS2/nZVI system exhibited stability and reusability. The involvement of various reactive species, such as hydroxyl radicals, superoxide anions, and singlet oxygen, was confirmed through quenching tests and electron paramagnetic resonance. The toxicity of degradation products decreased after treatment, indicating the potential of this MoS2 co-catalytic nZVI-based Fenton-like process for organic wastewater treatment.

ENVIRONMENTAL RESEARCH (2023)

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Article Agricultural Engineering

Enhanced elimination of Cr(VI) from aqueous media by polyethyleneimine modified corn straw biochar supported sulfide nanoscale zero valent iron: Performance and mechanism

Haoran Tian et al.

Summary: A novel polyethyleneimine modified corn straw biochar supported sulfide nanoscale zero-valent iron (S-nZVI@PBC) was developed to enhance the removal of Cr(VI) from aqueous media. The characteristics of S-nZVI@PBC and its mechanism for Cr(VI) removal were explored, and it was found that the adsorption process followed a pseudo-second-order model and Langmuir isotherm model. The primary mechanisms for Cr(VI) removal were adsorption, reduction, and co-precipitation. S-nZVI@PBC showed higher stability and reusability compared to nZVI, making it a promising tool for treating Cr(VI)-containing wastewater.

BIORESOURCE TECHNOLOGY (2023)

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Synergistic effect and mechanism of Cd(II) and As(III) adsorption by biochar supported sulfide nanoscale zero-valent iron

Xiaoyu Zheng et al.

Summary: Biochar derived from bamboo was utilized as a support for sulfide nanoscale zero-valent iron (S-nZVI@BC) for the simultaneous removal of Cd(II) and As (III) from water. The successful synthesis of S-nZVI@BC was confirmed by SEM and XRD characterization. Co-adsorption of Cd(II) and As(III) onto S-nZVI@BC followed the pseudo-second-order model and Langmuir model, with higher adsorption capacity compared to single adsorption. The optimal Cd(II)-to-As(III) concentration ratio was 1:2, and the presence of Ca2+ and Mg2+ inhibited Cd(II) removal, while phosphate and humic acid inhibited As(III) removal. S-nZVI@BC exhibited better electrochemical properties and the primary mechanisms for Cd(II) and As(III) removal were electrostatic adsorption, complexation, co-precipitation, and redox. This study provides insights into the efficient removal of Cd(II) and As(III) from wastewater using S-nZVI@BC.

ENVIRONMENTAL RESEARCH (2023)

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In situ remediation of Cr(VI) contaminated groundwater by ZVI-PRB and the corresponding indigenous microbial community responses: a field-scale study

Qing Wang et al.

Summary: The study found that a permeable reactive barrier (PRB) successfully reduced hexavalent chromium (Cr (VI)) concentrations through chemical reduction, impacting the indigenous microbial community structure. Competitive growth among Cr(VI)-reducing bacteria was observed in the PRB area, while Cr(VI)-reducing bacteria were enriched downgradient, indicating further bio-reduction of Cr(VI) to Cr(III). This bio-reduction could serve as a secondary mechanism for prolonged removal of Cr(VI) from groundwater, influenced by environmental factors such as pH, dissolved oxygen, Cr(VI) levels, oxidation-reduction potential, and temperature.

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Luping Zeng et al.

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Umair Azhar et al.

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Liu Fei et al.

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Effective and stable adsorptive removal of Cadmium(II) and Lead(II) using selenium nanoparticles modified by microbial SmtA metallothionein

Zijie Zhou et al.

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Ruirui Sun et al.

Summary: Nano zero-valent iron loaded porous carbon derived from microplastics was designed as a heterogeneous catalyst for degradation of persistent organic pollutants. The catalyst exhibited high carbon yield and large surface area, leading to effective degradation of various pollutants. Hydroxyl radicals generated from the activation of H2O2 enhanced by zero-valent iron in Fe/MMPC were identified as the predominant species in the catalytic reactions.

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Insights into the mechanism underlying remediation of Cr(VI) contaminated aquifer using nanoscale zero-valent iron@reduced graphene oxide

Liming Ren et al.

Summary: In this study, the mechanism of Cr(VI) contaminated aquifer remediation using nZVI@rGO was explored through experiments and characterization analysis. The results showed that the large reactive conjugated structure of rGO enhanced the electron transfer efficiency between Cr(VI) and nZVI@rGO, while the uniform accommodation of Cr(III) precipitates on rGO effectively retarded the surface passivation of nZVI.

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Yun-fei Zhang et al.

Summary: This review provides a systematic and comprehensive summary of commonly used strategies to enhance the reactivity of zero-valent iron (ZVI). The purpose is to understand the mechanisms, advantages, and shortcomings of these strategies, as well as to forecast the future development of ZVI technologies.

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Efficient adsorption of heavy metals from wastewater on nanocomposite beads prepared by chitosan and paper sludge

Kehan Xu et al.

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Advances in design and synthesis of stabilized zero-valent iron nanoparticles for groundwater remediation

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ENVIRONMENTAL SCIENCE & TECHNOLOGY (2001)

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Article Engineering, Environmental

Remediation of Cr(VI) and Pb(II) aqueous solutions using supported, nanoscale zero-valent iron

SM Ponder et al.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2000)

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Article Engineering, Environmental

Pathways and kinetics of chlorinated ethylene and chlorinated acetylene reaction with Fe(O) particles

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ENVIRONMENTAL SCIENCE & TECHNOLOGY (2000)

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