Tailoring of the Interfacial Dzyaloshinskii-Moriya Interaction in Perpendicularly Magnetized Epitaxial Multilayers by Crystal Engineering

The interplay between the interfacial crystalline structure and Dzyaloshinskii-Moriya interaction (DMI) was investigated by Fe insertion in epitaxial Pt/Co/Ir perpendicular magnetized multilayers. The experimental results with the support of first-principles calculation indicate that the Fe/Ir interface exhibits a positive interfacial DMI (iDMI) originating from the fcc crystalline structure inserted by 2 monolayers (ML) Fe, while a negative one from the structure with a layer shifting of 1-ML Fe insertion. The total iDMI of the multilayers increases (decreases) due to the additive enhancement (competitive counteraction) between the iDMI of Fe/Ir and Pt/Co interfaces. Comparing the iDMI of single-crystalline and textured multilayers, the iDMI of multilayers is found to be particularly sensitive to the crystallinity nearby the heterointerfaces. This work is of vital importance to reveal a deeper insight into the physical mechanism of the iDMI and provides a viable strategy for tailoring the iDMI of the multilayers by crystal engineering.

Automated summary

The interplay between the interfacial crystalline structure and Dzyaloshinskii-Moriya interaction (DMI) was studied in Fe-inserted Pt/Co/Ir perpendicular magnetized multilayers. It was found that the Fe/Ir interface exhibits positive interfacial DMI (iDMI) with 2 ML Fe insertion, while negative iDMI with a layer shifting of 1-ML Fe insertion. The total iDMI of the multilayers increases (decreases) due to the additive enhancement (competitive counteraction) between the iDMI of Fe/Ir and Pt/Co interfaces. The crystallinity nearby the heterointerfaces was found to significantly affect the iDMI of the multilayers. This work provides valuable insights into the physical mechanism of iDMI and offers a viable strategy for tailoring the iDMI of multilayers through crystal engineering.