4.7 Article

Black carbon over tropical Indian coast during the COVID-19 lockdown: inconspicuous role of coastal meteorology

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ENVIRONMENTAL SCIENCE AND POLLUTION RESEARCH
卷 30, 期 15, 页码 44773-44781

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SPRINGER HEIDELBERG
DOI: 10.1007/s11356-023-25370-5

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Aerosols; Black carbon; Fossil-fuel emissions; Continental air; Biomass burning; Marine air; Transport; COVID-19 lockdown; Pollution; India

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We conducted in situ measurements of black carbon (BC) concentration in Chennai, India from January to June 2020. The results showed an unprecedented reduction in BC concentration during the COVID-19 lockdown, despite stronger precipitation. The study also revealed that BC depletion was more pronounced in continental air than in marine air, and there was a shift from fossil-fuel dominance to biomass burning dominance as a BC source.
Black carbon (BC) aerosols critically impact the climate and hydrological cycle. The impact of anthropogenic emissions and coastal meteorology on BC dynamics, however, remains unclear over tropical India, a globally identified hotspot. In this regard, we have performed in situ measurements of BC over a megacity (Chennai, 12 degrees 59 ' 26.5 '' N, 80 degrees 13 ' 51.8 '' E) on the eastern coast of India during January-June 2020, comprising the period of COVID-19-induced strict lockdown. Our measurements revealed an unprecedented reduction in BC concentration by an order of magnitude as reported by other studies for various other pollutants. This was despite having stronger precipitation during pre-lockdown and lesser precipitation washout during the lockdown. Our analyses, taking mesoscale dynamics into account, unravels stronger BC depletion in the continental air than marine air. Additionally, the BC source regime also shifted from a fossil-fuel dominance to a biomass burning dominance as a result of lockdown, indicating relative reduction in fossil fuel combustion. Considering the rarity of such a low concentration of BC in a tropical megacity environment, our observations and findings under near-natural or background levels of BC may be invaluable to validate model simulations dealing with BC dynamics and its climatic impacts in the Anthropocene.

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