This review summarizes the recent research progress on graphene-based electrodes in the field of ion electrosorption, especially in water desalination utilizing capacitive deionization (CDI) technology. The latest advances in graphene-based electrodes, such as 3D graphene, graphene/metal oxide composites, graphene/carbon composites, heteroatom-doped graphene, and graphene/polymer composites, are presented. Furthermore, the challenges and future possible developments in the electrosorption area are also addressed, providing insights for researchers to design graphene-based electrodes towards practical applications.
Due to its unique advantages such as flexible planar structure, ultrahigh specific surface area, superior electrical conductivity and electrical double-layer capacitance in theory, graphene has unparalleled virtues compared with other carbon materials. This review summarizes the recent research progress of various graphene-based electrodes on ion electrosorption fields, especially for water desalination utilizing capacitive deionization (CDI) technology. We present the latest advances of graphene-based electrodes, such as 3D graphene, graphene/metal oxide (MO) composites, graphene/carbon composites, heteroatom-doped graphene and graphene/polymer composites. Furthermore, a brief outlook on the challenges and future possible developments in the electrosorption area are also addressed for researchers to design graphene-based electrodes towards practical application.
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