Defect-engineered metal-organic frameworks (MOF-808) towards the improved adsorptive removal of organic dyes and chromium (vi) species from water

Article Engineering, Environmental

Defect-engineering of Zr(IV)-based metal-organic frameworks for regulating CO2 photoreduction

Shi-Qing Wang et al.

Summary: The study found that defects in MOFs can significantly enhance the photocatalytic performance of CO2 reduction, with the ligand-vacant UiO-66-NH2-LV exhibiting the best photocatalytic activity.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Engineering, Environmental

Preparation of multivariate zirconia metal-organic frameworks for highly efficient adsorption of endocrine disrupting compounds

Lizhen Han et al.

Summary: The preparation of multivariate Zr-MOFs via mixed-ligands strategy allows for the control of morphology, adsorption, and removal properties, with 57%TCPP@MOF-808 showing excellent stability and high adsorption capacity for endocrine disrupting compounds. The use of 57%TCPP@MOF-808 as sorbent in dispersive solid-phase extraction led to successful extraction of EDCs with high recoveries and enrichment factors, demonstrating its potential in environmental pollutant detection.

JOURNAL OF HAZARDOUS MATERIALS (2022)

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Review Chemistry, Multidisciplinary

Metal-Organic Frameworks (MOFs)-Based Mixed Matrix Membranes (MMMs) for Gas Separation: A Review on Advanced Materials in Harsh Environmental Applications

Shu Hua Goh et al.

Summary: This article reviews the development of MOFs-based MMMs in the past 3 years, discussing gas transport estimation models, preparation methods, and challenges in developing MMMs. The application and separation performance of various MOFs-based MMMs, including those using advanced MOFs materials, are summarized. The latest exploration of MOF materials for harsh operating conditions is emphasized. The outlook and future opportunities of MMMs are contemplated.

SMALL (2022)

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Review Environmental Sciences

Adsorption of pollutants in wastewater via biosorbents, nanoparticles and magnetic biosorbents: A review

Guat Teng Tee et al.

Summary: This critical review focuses on the preparation, modification, application and regeneration of biosorbents, nanoparticles, and magnetic biosorbents for wastewater treatment. The development of magnetic biosorbents is highlighted due to their variable active sites, high specific surface area, easy separation, and low cost. Chemical activations such as acid, alkali, and salt activations are discussed to improve the adsorption performance of biosorbents. The surface characteristics and chemistry of biosorbents and magnetic biosorbents, including electrostatic interaction, 7C-7C interaction, and hydrogen bonding, are emphasized. The effects of solution pH, adsorbent dosage, initial concentration of pollutants, adsorption duration, and temperature on the adsorption capacity and removal efficiency are analyzed. The review concludes with a summary, challenges, and future outlook of magnetic biosorbents, aiming to provide insights for cost-effective and scalable adsorbents for environmental remediation.

ENVIRONMENTAL RESEARCH (2022)

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Article Engineering, Chemical

Green synthesis of MOF-808 with modulation of particle sizes and defects for efficient phosphate sequestration

Yu Tao et al.

Summary: In this work, a facile and green method is applied to synthesize hydrophilic MOF-808(Zr) and modulate its defect content and particle size using different amounts of iron nitrate to obtain serial XF-MOF-808 with enhanced phosphate adsorption performance. The 0.5F-MOF-808 exhibits exceptional adsorption capacity and rapid diffusion rate for phosphate, surpassing pristine MOF-808 and other reported adsorbents. The modified MOF also shows wide pH tolerance and excellent selectivity for phosphate adsorption from simulated wastewater, making it a promising material for phosphate adsorption and recovery.

SEPARATION AND PURIFICATION TECHNOLOGY (2022)

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Article Chemistry, Physical

Oriented construction of efficient intrinsic proton transport pathways in MOF-808

Xiao-Min Li et al.

Summary: By replacing the coordinating groups in MOF-808, we have successfully synthesized proton conductors MOF-808-IMC and MOF-808-IMDC, which exhibit higher proton conductivity than the original MOF-808. Among them, MOF-808-IMDC shows good cycling stability and durability, suggesting its potential as a fuel cell membrane.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Article Chemistry, Physical

Controlled growth and composition of multivariate metal-organic frameworks-199 via a reaction-diffusion process

Razan Issa et al.

Summary: In this paper, the authors used the reaction-diffusion framework to successfully synthesize MOF-199 single crystals, and then utilized this method to synthesize multivariate metal-organic frameworks with enhanced properties. By integrating organic linkers with different functional groups into the crystal structure, defects were created, resulting in the synthesis of MTV-MOFs. The effects of the linkers on the morphology, thermal stability, and surface area of the synthesized MTV-MOFs were investigated, demonstrating improved adsorptive capabilities for methylene blue and rhodamine B in aqueous solution.

NANO RESEARCH (2021)

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Review Nanoscience & Nanotechnology

Generating Catalytic Sites in UiO-66 through Defect Engineering

Xiao Feng et al.

Summary: UiO-66 is considered as an epitome of metal-organic frameworks (MOFs) due to its stability and capability to withstand high numbers of defects without structural collapse. Numerous studies have focused on constructing catalytic sites in UiO-66 through defect engineering to enhance performance.

ACS APPLIED MATERIALS & INTERFACES (2021)

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Article Chemistry, Multidisciplinary

Elucidating the Structural Evolution of a Highly Porous Responsive Metal-Organic Framework (DUT-49(M)) upon Guest Desorption by Time-Resolved in Situ Powder X-ray Diffraction

Bikash Garai et al.

Summary: This study monitored the solvent desorption process in the pores of DUT-49(M) frameworks in real-time using PXRD, revealing the continuous and discontinuous phase transitions from the open pore phase to the intermediate pore phase and from the intermediate pore phase to the contracted pore phase for DUT-49(Cu) and DUT-49(Ni).

CRYSTAL GROWTH & DESIGN (2021)

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Article Chemistry, Multidisciplinary

Enhancing the Catalytic Activity of MOF-808 Towards Peptide Bond Hydrolysis through Synthetic Modulations

Charlotte Simms et al.

Summary: The study evaluated the impact of metal precursor on the reactivity of MOFs in catalysis, and investigated the effects of synthesis temperature and duration.

CHEMISTRY-A EUROPEAN JOURNAL (2021)

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Review Environmental Sciences

Adsorptive removal of dyes from wastewater using a metal-organic framework: A review

Md Jamal Uddin et al.

Summary: Metal-organic frameworks (MOFs) are a promising adsorbent for efficient dye removal and degradation in industrial wastewater treatment. The performance of MOFs is influenced by factors such as their structure type, functional groups, ligands, and pH level.

CHEMOSPHERE (2021)

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Article Chemistry, Multidisciplinary

Tuning the Properties of MOF-808 via Defect Engineering and Metal Nanoparticle Encapsulation

Rifan Hardian et al.

Summary: Defect engineering and metal encapsulation are valuable approaches to fine-tune the reactivity of metal-organic frameworks. This study quantified the reactivity of pristine, defective, and Pt encapsulated MOF-808, revealing competitive effects between crystal morphology and missing linker defects, which can impact the stability of the MOF. Despite leading to a loss in porosity, defects are beneficial for the stability of MOF-808 towards water and can be used to tune adsorption properties.

CHEMISTRY-A EUROPEAN JOURNAL (2021)

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Article Chemistry, Applied

The joint effect of naphthalene-system and defects on dye removal by UiO-66 derivatives

Vera V. Butova et al.

Summary: UiO-66 derivates show promising photocatalytic performance in dye removal, especially with the inclusion of molecules such as 1,4-benzene dicarboxylate and 1,4-naphthalene dicarboxylate. The presence of naphthalene groups can improve photocatalytic efficiency by reducing the bandgap of the material. Additionally, defects in the MOF structure also play a role in influencing photocatalytic efficiency.

MICROPOROUS AND MESOPOROUS MATERIALS (2021)

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Article Chemistry, Applied

Selective adsorption and separation of dyes from aqueous solution by a zirconium-based porous framework material

Shifang Jia et al.

Summary: The water-stable zirconium-based metal-organic framework MOF-808 has demonstrated superior adsorption and separation capabilities for anionic fluorescein sodium (FS) and cationic rhodamine B (RhB). The efficient separation is attributed to the pore sieving effect and various host-guest interactions driving the adsorption process. This work highlights the potential of MOF-808 as a promising material for efficient dye separation and offers new insights for developing adsorbents with distinct pore and chemical properties of MOFs.

APPLIED ORGANOMETALLIC CHEMISTRY (2021)

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Review Chemistry, Multidisciplinary

Surfactant Adsorption Isotherms: A Review

Shams Kalam et al.

Summary: This paper provides a brief overview of surfactant adsorption isotherms on rock surfaces, focusing on adsorption theories and commonly used models like Langmuir and Freundlich. More complex adsorption isotherms such as Redlich-Peterson and Sips are also discussed, which involve three parameters and can help select the appropriate model for experimental data.

ACS OMEGA (2021)

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Article Multidisciplinary Sciences

The removal of anionic and cationic dyes from an aqueous solution using biomass-based activated carbon

Nurul Umairah M. Nizam et al.

Summary: This study successfully synthesized cost-effective and efficient PAC for removing dyes from industrial wastewater by optimizing the synthesis conditions. The PAC showed high adsorption capacity and rate, with multiple adsorption mechanisms involved in the process, leading to effective dye removal. The presence of functional groups and active sites on the PAC contributed to its considerable affinity for adsorption, making it a promising adsorbent for dye removal applications.

SCIENTIFIC REPORTS (2021)

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Article Chemistry, Multidisciplinary

Efficient Removal of Chromium(VI) Anionic Species and Dye Anions from Water Using MOF-808 Materials Synthesized with the Assistance of Formic Acid

Khoa D. Nguyen et al.

Summary: This study presents a simple method to prepare MOF-808 with tailored particle sizes and demonstrates its high uptake capacity and stable adsorption ability for ionic pollutants and dyes, making it a promising platform for water remediation.

NANOMATERIALS (2021)

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Review Chemistry, Multidisciplinary

Recent advances in vacancy engineering of metal-organic frameworks and their derivatives for electrocatalysis

Yuhang Wu et al.

Summary: Metal-organic frameworks (MOFs) and their derivatives have attracted considerable interest in electrocatalysis due to their multiple active sites and large specific surface areas, with vacancies playing a vital role in promoting electrocatalytic processes. Understanding the classification, synthetic strategy, and application of vacancies in electrocatalysis could lead to the development of new effective catalysts in MOFs and their derivatives.

SUSMAT (2021)

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Review Nanoscience & Nanotechnology

Zirconium-Based Metal-Organic Frameworks for the Catalytic Hydrolysis of Organophosphorus Nerve Agents

Kent O. Kirlikovali et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

Multivariate Modulation of the Zr MOF UiO-66 for Defect-Controlled Combination Anticancer Drug Delivery

Isabel Lazaro et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Applied

Synthesis of pearl necklace-like ZIF-8@chitosan/PVA nanofiber with synergistic effect for recycling aqueous dye removal

Niyaz Mohammad Mahmoodi et al.

CARBOHYDRATE POLYMERS (2020)

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Article Chemistry, Multidisciplinary

Engineering a Highly Defective Stable UiO-66 with Tunable Lewis-Bronsted Acidity: The Role of the Hemilabile Linker

Xiao Feng et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Multidisciplinary

Creation of Active Sites in MOF-808(Zr) by a Facile Route for Oxidative Desulfurization of Model Diesel Oil

Yulong Gu et al.

CHEMISTRYSELECT (2020)

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Article Chemistry, Applied

Defect creation by benzoic acid in Cu-Based Metal-Organic frameworks for enhancing sulfur capture

Hong-Yan Zhang et al.

MICROPOROUS AND MESOPOROUS MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Chromium Speciation in Zirconium-Based Metal-Organic Frameworks for Environmental Remediation

Paula G. Saiz et al.

CHEMISTRY-A EUROPEAN JOURNAL (2020)

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Article Chemistry, Physical

New 1D chiral Zr-MOFs based on in situ imine linker formation as catalysts for asymmetric C-C coupling reactions

Khoa D. Nguyen et al.

JOURNAL OF CATALYSIS (2020)

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Article Chemistry, Physical

Tuning the Catalytic Properties of UiO-66 Metal-Organic Frameworks: From Lewis to Defect-Induced Bronsted Acidity

F. G. Cirujano et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2020)

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Review Materials Science, Multidisciplinary

What triggers dye adsorption by metal organic frameworks? The current perspectives

M. Shahnawaz Khan et al.

MATERIALS ADVANCES (2020)

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Article Nanoscience & Nanotechnology

NO2 Removal under Ambient Conditions by Nanoporous Multivariate Zirconium-Based Metal-Organic Framework

Xinbo Wang et al.

ACS APPLIED NANO MATERIALS (2020)

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Article Green & Sustainable Science & Technology

Adsorption kinetic modeling using pseudo-first order and pseudo-second order rate laws: A review

Emmanuel D. Revellame et al.

CLEANER ENGINEERING AND TECHNOLOGY (2020)

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Article Nanoscience & Nanotechnology

Defect Control in Zr-Based Metal-Organic Framework Nanoparticles for Arsenic Removal from Water

Nisrine Assaad et al.

ACS APPLIED NANO MATERIALS (2020)

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Review Chemistry, Multidisciplinary

Coordinatively unsaturated metal sites (open metal sites) in metal-organic frameworks: design and applications

Ulku Kokcam-Demir et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Review Chemistry, Inorganic & Nuclear

Metal-organic frameworks in Germany: From synthesis to function

Jack D. Evans et al.

COORDINATION CHEMISTRY REVIEWS (2019)

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Article Chemistry, Multidisciplinary

Highly Defective UiO-66 Materials for the Adsorptive Removal of Perfluorooctanesulfonate

Chelsea A. Clark et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2019)

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Review Chemistry, Inorganic & Nuclear

Reticular chemistry in the rational synthesis of functional zirconium cluster-based MOFs

Zhijie Chen et al.

COORDINATION CHEMISTRY REVIEWS (2019)

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Article Chemistry, Physical

Effect of free carboxylic acid groups in UiO-66 analogues on the adsorption of dyes from water: Plausible mechanisms for adsorption and gate-opening behavior

Wei Zhang et al.

JOURNAL OF MOLECULAR LIQUIDS (2019)

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Article Chemistry, Physical

Insights into the role of zirconium in proline functionalized metal-organic frameworks attaining high enantio- and diastereoselectivity

Khoa D. Nguyen et al.

JOURNAL OF CATALYSIS (2019)

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Article Thermodynamics

Thermal analysis, structure, spectroscopy and DFT calculations of a pharmaceutical cocrystal of salicylic acid and salicylamide

Hirihattaya Phetmung et al.

JOURNAL OF THERMAL ANALYSIS AND CALORIMETRY (2019)

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Review Materials Science, Multidisciplinary

Metal-organic frameworks: Structures and functional applications

Long Jiao et al.

MATERIALS TODAY (2019)

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Article Chemistry, Multidisciplinary

An analysis of the effect of zirconium precursors of MOF-808 on its thermal stability, and structural and surface properties

Carolina Ardila-Suarez et al.

CRYSTENGCOMM (2019)

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Article Chemistry, Physical

A multifunctional Zr(iv)-based metal-organic framework for highly efficient elimination of Cr(vi) from the aqueous phase

Junmin Liu et al.

JOURNAL OF MATERIALS CHEMISTRY A (2019)

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Review Chemistry, Multidisciplinary

Stable Metal-Organic Frameworks: Design, Synthesis, and Applications

Shuai Yuan et al.

ADVANCED MATERIALS (2018)

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Review Chemistry, Multidisciplinary

Defective Metal-Organic Frameworks

Stefano Dissegna et al.

ADVANCED MATERIALS (2018)

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Article Chemistry, Physical

Selective dye adsorption by highly water stable metal-organic framework: Long term stability analysis in aqueous media

Hossein Molavi et al.

APPLIED SURFACE SCIENCE (2018)

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Article Chemistry, Multidisciplinary

Stepwise Methane-to-Methanol Conversion on CuO/SBA-15

Ha V. Le et al.

CHEMISTRY-A EUROPEAN JOURNAL (2018)

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Article Chemistry, Multidisciplinary

A Zwitterionic Ligand-Based Cationic Metal-Organic Framework for Rapidly Selective Dye Capture and Highly Efficient Cr2O72- Removal

Chenghui Zhang et al.

CHEMISTRY-A EUROPEAN JOURNAL (2018)

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Article Multidisciplinary Sciences

A versatile MOF-based trap for heavy metal ion capture and dispersion

Yaguang Peng et al.

NATURE COMMUNICATIONS (2018)

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Article Chemistry, Physical

Catalytic properties of pristine and defect-engineered Zr-MOF-808 metal organic frameworks

H-H. Mautschke et al.

CATALYSIS SCIENCE & TECHNOLOGY (2018)

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Article Chemistry, Physical

An ultrastable Zr-MOF for fast capture and highly luminescence detection of Cr2O72- simultaneously in an aqueous phase

Xiaodong Sun et al.

JOURNAL OF MATERIALS CHEMISTRY A (2018)

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Article Chemistry, Physical

A facile approach to fabricate an immobilized-phosphate zirconium based metal-organic framework composite (UiO-66-P) and its activity in the adsorption and separation of organic dyes

Ji-Min Yang

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2017)

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Article Chemistry, Multidisciplinary

Using water adsorption measurements to access the chemistry of defects in the metal-organic framework UiO-66

Stefano Dissegna et al.

CRYSTENGCOMM (2017)

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Article Engineering, Environmental

Rational construction of defects in a metal-organic framework for highly efficient adsorption and separation of dyes

Keke Wang et al.

CHEMICAL ENGINEERING JOURNAL (2016)

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Article Chemistry, Physical

Defect Engineering: Tuning the Porosity and Composition of the Metal-Organic Framework UiO-66 via Modulated Synthesis

Greig C. Shearer et al.

CHEMISTRY OF MATERIALS (2016)

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Article Chemistry, Multidisciplinary

Exploration of MOF nanoparticle sizes using various physical characterization methods - is what you measure what you get?

Patrick Hirschle et al.

CRYSTENGCOMM (2016)

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Article Chemistry, Inorganic & Nuclear

Origin of highly active metal-organic framework catalysts: defects? Defects!

J. Canivet et al.

DALTON TRANSACTIONS (2016)

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Review Chemistry, Inorganic & Nuclear

What Can Electron Microscopy Tell Us Beyond Crystal Structures?

Wuzong Zhou et al.

EUROPEAN JOURNAL OF INORGANIC CHEMISTRY (2016)

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Article Chemistry, Inorganic & Nuclear

Postsynthetic Inner-Surface Functionalization of the Highly Stable Zirconium-Based Metal-Organic Framework DUT-67

Franziska Drache et al.

INORGANIC CHEMISTRY (2016)

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Article Acoustics

Ultrasonically assisted hydrothermal synthesis of activated carbon-HKUST-1-MOF hybrid for efficient simultaneous ultrasound-assisted removal of ternary organic dyes and antibacterial investigation: Taguchi optimization

F. Nasiri Azad et al.

ULTRASONICS SONOCHEMISTRY (2016)

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Article Engineering, Environmental

Adsorption of azo dyes from aqueous solution by the hybrid MOFs/GO

Ling Li et al.

WATER SCIENCE AND TECHNOLOGY (2016)

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Review Chemistry, Multidisciplinary

Defect-Engineered Metal-Organic Frameworks

Zhenlan Fang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2015)

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Article Chemistry, Physical

Selective adsorption of cationic dyes by UiO-66-NH2

Qi Chen et al.

APPLIED SURFACE SCIENCE (2015)

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Article Chemistry, Multidisciplinary

Robust, Chiral, and Porous BINAP-Based Metal-Organic Frameworks for Highly Enantioselective Cyclization Reactions

Takahiro Sawano et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2015)

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Review Chemistry, Multidisciplinary

Tuning the structure and function of metal-organic frameworks via linker design

Weigang Lu et al.

CHEMICAL SOCIETY REVIEWS (2014)

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Article Chemistry, Multidisciplinary

Water Adsorption in Porous Metal-Organic Frameworks and Related Materials

Hiroyasu Furukawa et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2014)

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Article Chemistry, Multidisciplinary

Superacidity in Sulfated Metal-Organic Framework-808

Juncong Jiang et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2014)

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Article Chemistry, Multidisciplinary

Unusual and Highly Tunable Missing-Linker Defects in Zirconium Metal-Organic Framework UiO-66 and Their Important Effects on Gas Adsorption

Hui Wu et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2013)

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Article Chemistry, Multidisciplinary

Synthesis Modulation as a Tool To Increase the Catalytic Activity of Metal-Organic Frameworks: The Unique Case of UiO-66(Zr)

Frederik Vermoortele et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2013)

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Review Multidisciplinary Sciences

The Chemistry and Applications of Metal-Organic Frameworks

Hiroyasu Furukawa et al.

SCIENCE (2013)

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Article Chemistry, Applied

Modulated synthesis of Zr-fumarate MOF

Gesa Wissmann et al.

MICROPOROUS AND MESOPOROUS MATERIALS (2012)

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Article Chemistry, Physical

Synthesis, structural properties, and catalytic behavior of Cu-BTC and mixed-linker Cu-BTC-PyDC in the oxidation of benzene derivatives

Stefan Marx et al.

JOURNAL OF CATALYSIS (2011)

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Article Engineering, Environmental

Adsorptive removal of methyl orange and methylene blue from aqueous solution with a metal-organic framework material, iron terephthalate (MOF-235)

Enamul Haque et al.

JOURNAL OF HAZARDOUS MATERIALS (2011)

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Letter Nanoscience & Nanotechnology

The Scherrer equation versus the 'Debye-Scherrer equation'

Uwe Holzwarth et al.

NATURE NANOTECHNOLOGY (2011)

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Article Chemistry, Physical

Intercalation of anionic organic ultraviolet ray absorbers into layered zinc hydroxide nitrate

Ana Cristina Trindade Cursino et al.

JOURNAL OF COLLOID AND INTERFACE SCIENCE (2010)

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Article Engineering, Environmental

Adsorptive removal of methyl orange from aqueous solution with metal-organic frameworks, porous chromium-benzenedicarboxylates

Enamul Haque et al.

JOURNAL OF HAZARDOUS MATERIALS (2010)

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Defect-engineered metal-organic frameworks (MOF-808) towards the improved adsorptive removal of organic dyes and chromium (vi) species from water

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