☆ 4.4 Review

Electrocatalytic oxidation of 5-hydroxymethylfurfural for sustainable 2,5-furandicarboxylic acid production-From mechanism to catalysts design

SUSMAT (2023)

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Article Chemistry, Multidisciplinary

High-valance molybdenum doped Co3O4 nanowires: Origin of the superior activity for 5-hydroxymethyl-furfural oxidation

Bingying Xia et al.

Summary: In this study, the electronic structure of Co3O4 was modified by doping with high valance Mo6+ to enhance its electrocatalytic ability for 5-hydroxymethyl-furfural (HMF) oxidation. Experimental results showed that Mo6+-doped Co3O4 had a stronger adsorption ability for HMF, leading to more favorable oxidation. This research provides a valuable reference for developing efficient heteroatom-doped electrocatalysts for HMF oxidation.

CHINESE CHEMICAL LETTERS (2023)

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Article Chemistry, Multidisciplinary

Doping-Modulated Strain Enhancing the Phosphate Tolerance on PtFe Alloys for High-Temperature Proton Exchange Membrane Fuel Cells

Wei Li et al.

Summary: In this study, the phosphate tolerance of PtFe ordered intermetallic alloys was enhanced through a doping-modulated strain strategy with Cu as a dopant, leading to improved performance in HT-PEMFCs. The Cu doping helped to create compressive strain in PtFe crystals, altering the electronic structure of electrocatalysts and weakening the adsorption energy between phosphoric acid and Pt surfaces. The HT-PEMFCs assembled with these cathodic electrocatalysts showed higher peak power and stability compared to commercial Pt/C electrocatalysts.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Tailoring Competitive Adsorption Sites by Oxygen-Vacancy on Cobalt Oxides to Enhance the Electrooxidation of Biomass

Yuxuan Lu et al.

Summary: The electrooxidation of 5-hydroxymethylfurfural (HMF) provides a green route to obtain high-value chemicals from biomass. The study reveals the adsorption behavior of HMF and OH- on Co3O4, with oxygen vacancy playing a crucial role. Modulating adsorption sites leads to excellent activity for the HMFOR process.

ADVANCED MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Selective Electrooxidation of Biomass-Derived Alcohols to Aldehydes in a Neutral Medium: Promoted Water Dissociation over a Nickel-Oxide-Supported Ruthenium Single-Atom Catalyst

Ruixiang Ge et al.

Summary: This study reports the selective electrooxidation of biomass-derived alcohols to aldehydes using single-atom ruthenium on nickel oxide as a catalyst in neutral medium. It demonstrates high efficiency and potential for sustainable production of value-added aldehyde compounds.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2022)

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Article Chemistry, Multidisciplinary

Hierarchical NiSx/Ni2P nanotube arrays with abundant interfaces for efficient electrocatalytic oxidation of 5-hydroxymethylfurfural

Baolong Zhang et al.

Summary: The electrochemical oxidation of 5-hydroxymethylfurfural to 2,5-furandicarboxylic acid has received attention recently. A strategy for synthesis of metal sulfide/metal phosphide nanotube arrays was proposed, which showed improved performance in the electrocatalytic oxidation of HMF.

GREEN CHEMISTRY (2022)

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Article Chemistry, Multidisciplinary

Controllable and facile preparation of Co9S8-Ni3S2 heterostructures embedded with N,S,O-tri-doped carbon for electrocatalytic oxidation of 5-hydroxymethylfurfural

Yibin Zhang et al.

Summary: Electrochemical oxidation of HMF into FDCA is a promising strategy, and finding cost-effective catalysts is crucial. In this study, carbon-based heterostructures were prepared using a facile method, and their excellent performance was confirmed.

GREEN CHEMISTRY (2022)

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Article Chemistry, Multidisciplinary

Oxygen Vacancy and Core-Shell Heterojunction Engineering of Anemone-Like CoP@CoOOH Bifunctional Electrocatalyst for Efficient Overall Water Splitting

Bing Zhang et al.

Summary: This study successfully prepared an anemone-like CoP@CoOOH core-shell heterojunction catalyst using oxygen-vacancy and core-shell heterojunction engineering strategy, which exhibited excellent HER and OER activities in both neutral and alkaline media. The core-shell heterojunction accelerated the catalytic kinetics, while oxygen-vacancies reduced the kinetic barrier, ultimately enhancing the OER performance.

SMALL (2022)

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Article Chemistry, Physical

Efficient Electrocatalytic Oxidation of 5-Hydroxymethylfurfural Coupled with 4-Nitrophenol Hydrogenation in a Water System

Xuliang Pang et al.

Summary: In this study, Cu foam decorated with Cu(OH)(2) was used as an efficient catalyst for the electrocatalytic conversion of HMF to FDCA. The CuOOH active species were identified as the main catalytic sites for HMF oxidation, and the oxidation pathway of HMF was revealed. A strategy of simultaneously producing two types of value-added chemicals at both electrodes was proposed.

ACS CATALYSIS (2022)

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Article Chemistry, Physical

Grass-like NixSey nanowire arrays shelled with NiFe LDH nanosheets as a 3D hierarchical core-shell electrocatalyst for efficient upgrading of biomass-derived 5-hydroxymethylfurfural and furfural

Yan Zhong et al.

Summary: In this study, a novel 3D hierarchical NixSey-NiFe layered double hydroxide core-shell nanostructure was reported for efficient electrocatalytic oxidation of biomass-derived compounds, showing outstanding catalytic performance and stability.

CATALYSIS SCIENCE & TECHNOLOGY (2022)

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Article Chemistry, Multidisciplinary

Engineering the Electronic Structure of NiFe Layered Double Hydroxide Nanosheet Array by Implanting Cationic Vacancies for Efficient Electrochemical Conversion of 5-Hydroxymethylfurfural to 2,5-Furandicarboxylic Acid

Yu-Feng Qi et al.

Summary: Utilizing a carbon paper-supported nickel-iron layered double hydroxide nanosheet array with abundant cationic vacancies as an electrode enables efficient conversion of HMF to FDCA, achieving high conversion and yield rates with excellent stability and electrocatalytic performance enhancements.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2022)

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Article Chemistry, Physical

Strain-induced in situ formation of NiOOH species on Co-Co bond for selective electrooxidation of 5-hydroxymethylfurfural and efficient hydrogen production

Zhaoyu Zhou et al.

Summary: Replacing water oxidation with the selective electrochemical conversion of HMF to FDCA is an efficient strategy to promote hydrogen production. High selectivity and Faradaic efficiency were achieved using a NiCo2O4 electrode, with the amount of generated hydrogen through coupling with HMF oxidation significantly higher than that of water splitting. The main active species for the selective electrooxidation of HMF to FDCA was identified as NiOOH.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Physical

Length Ultrathin polycrystalline Co3O4 nanosheets with enriched oxygen vacancies for efficient electrochemical oxygen evolution and 5-hydroxymethylfurfural oxidation

Ruyi Zhong et al.

Summary: Surfactant-free, freestanding, and hierarchical two-dimensional polycrystalline cobalt oxide nanosheets with enriched oxygen vacancies (Co3O4-VO) were synthesized. These Co3O4-VO nanosheets outperformed the original nanosheets and conventionally calcined Co3O4 in electrochemical oxygen evolution and HMF oxidation to FDCA due to their preserved 2D structure and elimination of surfactant, exposing abundant active sites. The strain-induced oxygen vacancies at grain boundaries of Co3O4 nanocrystallines were also proposed to contribute to the improved electrooxidation performance. Furthermore, Co3O4-VO showed remarkable long-term stability in 1 M KOH chronoamperometric test.

APPLIED SURFACE SCIENCE (2022)

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Article Engineering, Environmental

Substrate molecule adsorption energy: An activity descriptor for electrochemical oxidation of 5-Hydroxymethylfurfural (HMF)

Yuechao Yang et al.

Summary: This study reveals that the adsorption energy of substrate molecules is an activity descriptor for electrochemical alcohol and aldehyde oxidation. Proper adsorption energy of the substrate molecules can achieve optimal catalytic activity. This finding is significant for the design of advanced catalysts and the utilization and production of renewable resources.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

Design and Application of a High-Surface-Area Mesoporous δ-MnO2 Electrocatalyst for Biomass Oxidative Valorization

Changlong Wang et al.

Summary: This study synthesized a mesoporous delta-MnO2 electrocatalyst with high surface area, high pore volume, and narrow pore size distributions using a nanocasting route. The electrocatalyst exhibited high efficiency, selectivity, and robustness for the electrochemical oxidation of 5-hydroxymethylfurfural (HMF) to 2,5-furandicarboxylic acid (FDCA) under alkaline conditions. The reaction kinetics and pathways of the electrochemical HMF oxidation over this advanced electrocatalyst were investigated and provided insights.

CHEMISTRY OF MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Electrochemical Oxidation of HMF via Hydrogen Atom Transfer and Hydride Transfer on NiOOH and the Impact of NiOOH Composition

Michael T. Bender et al.

Summary: This study quantitatively examines the impact of two different dehydrogenation mechanisms on the oxidation of HMF and its intermediates, providing new insights for the rational design of more efficient electrochemical dehydrogenation catalysts.

CHEMSUSCHEM (2022)

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Article Chemistry, Multidisciplinary

Construction of Synergistic Ni3S2-MoS2 Nanoheterojunctions on Ni Foam as Bifunctional Electrocatalyst for Hydrogen Evolution Integrated with Biomass Valorization

Shaowei Yang et al.

Summary: A Ni3S2-MoS2 nanoheterojunction catalyst with strong electronic interactions was prepared in this study, showing high efficiency in both hydrogen evolution reaction (HER) and electrooxidation of 5-hydroxymethylfurfural (HMF). The findings are significant for developing efficient electrocatalysts and continuous production of high value-added products and H2.

SMALL (2022)

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Article Chemistry, Physical

Integrated Catalytic Sites for Highly Efficient Electrochemical Oxidation of the Aldehyde and Hydroxyl Groups in 5-Hydroxymethylfurfural

Yuxuan Lu et al.

Summary: This study investigates the different catalytic processes of HMFOR and identifies direct and synergistic oxidation types. The introduction of nickel into cobalt oxide catalysts improves the hydroxyl activity and achieves optimal HMFOR performance.

ACS CATALYSIS (2022)

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Article Chemistry, Physical

Collaborative Electrochemical Oxidation of the Alcohol andAldehyde Groups of 5-Hydroxymethylfurfural by NiOOH andCu(OH)2for Superior 2,5-Furandicarboxylic Acid Production

Jongin Woo et al.

Summary: In this study, the different reactivities of NiOOH and Cu(OH)2 towards the electrochemical oxidation of alcohol and aldehyde were analyzed, and their characteristics were utilized to enhance the conversion performance of HMF to FDCA. NiOOH exhibited good reactivity for alcohol oxidation, while Cu(OH)2 showed good reactivity for aldehyde oxidation. The mixed electrode of NiOOH-Cu(OH)2 showed higher activity and faster conversion of HMF. By preparing a nanoframe structure, the oxidation kinetics of NiOOH/Cu(OH)2 for HMF was further enhanced, achieving instantaneous conversion to FDCA.

ACS CATALYSIS (2022)

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Article Chemistry, Multidisciplinary

Technoeconomic and Life-Cycle Assessment for Electrocatalytic Production of Furandicarboxylic Acid

Poojan Patel et al.

Summary: This study assesses the economic aspects and environmental impacts of the electrochemical production of FDCA. It is found that the electrochemical method shows potential in terms of both economics and environmental impact, and further improvements can be made by reducing the environmental impact of HMF production. However, there is still a need to lower the current density to improve the process economics.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2022)

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Article Chemistry, Multidisciplinary

Efficient Electrooxidation of 5-Hydroxymethylfurfural Using Co-Doped Ni3S2 Catalyst: Promising for H2 Production under Industrial-Level Current Density

Yan Sun et al.

Summary: In this study, a new type of non-noble metal electrocatalyst was successfully prepared for the oxidation reaction of organic compounds. The catalyst exhibited low potential and high current density, showing high efficiency for the oxidation reaction of HMF. The research also demonstrated the importance of the catalyst in promoting H-2 production and its potential for the electrooxidation of other biomass-derived chemicals.

ADVANCED SCIENCE (2022)

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Article Chemistry, Physical

A dynamic Ni(OH)(2)-NiOOH/NiFeP heterojunction enabling high-performance E-upgrading of hydroxymethylfurfural

Ruipeng Luo et al.

Summary: The facile upgrading of 5-hydroxymethylfurfural (HMF) via controllable oxidation of aldehyde and hydroxymethyl groups has attracted attention due to the industrial value of 2,5-furandicarboxylic acid (FDCA). The Ni(OH)2-NiOOH/NiFeP heterojunction exhibits outstanding performance in HMF oxidation, producing FDCA with high yield and Faradaic efficiency. A NiOOH-centered dual-circle mechanism is proposed to understand the intertwined and competitive processes of HMF oxidation and oxygen evolution.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Physical

In-situ chemical corrosive nickel foam as high-efficient electrocatalyst for 5-hydroxymethylfurfural oxidation

Guangxue Yang et al.

Summary: In this study, a nickel hydroxide nanosheet-loaded nickel foam catalyst was successfully synthesized using the chemical in-situ corrosion method to explore the electrochemical oxidation of 5-hydroxymethylfurfural (HMF) for the preparation of 2,5-furandicarboxylic acid (FDCA). The prepared catalyst exhibited excellent HMF conversion rate, FDCA selectivity, and Faraday efficiency. Moreover, the catalytic activity and selectivity could be adjusted by varying the electrolysis potential. This combination of corrosion technology and biomass conversion provides insights for the design of stable and controllable electrocatalysts in future energy conversion processes.

APPLIED SURFACE SCIENCE (2022)

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Article Multidisciplinary Sciences

Unraveling the mechanism for paired electrocatalysis of organics with water as a feedstock

Ganceng Yang et al.

Summary: The production of value-added chemicals using renewable energy and cost-effective water has attracted significant interest. In this study, the authors developed a paired electrocatalytic system to produce 4-aminobenzyl alcohol and 2,5-furandicarboxylic acid. The electroreduction and electrooxidation of organics with water as a feedstock show promising potential for the production of value-added chemicals. Through comprehensive investigations, the researchers gained insights into the reaction mechanism and proposed explicit reaction pathways. The paired electrolyzer, powered by a solar cell, exhibited excellent performance with low voltage, high faradaic efficiency, and remarkable cycle stability. This work provides valuable guidance for the sustainable synthesis of various value-added chemicals through paired electrocatalysis.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Multidisciplinary

Simultaneous CO2 Reduction and 5-Hydroxymethylfurfural Oxidation to Value-Added Products by Electrocatalysis

Jiahui Bi et al.

Summary: This study presents a novel paired electrolysis system integrating cathodic CO2RR and anodic HMFOR, which efficiently convert CO2 and HMF simultaneously. By utilizing specific catalysts and electrolytes, the system achieves high efficiency with low onset voltage, demonstrating outstanding performance in terms of FE and current density for both CO2RR and HMFOR processes.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2022)

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Review Chemistry, Multidisciplinary

Confinement Engineering of Electrocatalyst Surfaces and Interfaces

Wei Li et al.

Summary: The electrocatalytic performance of nanomaterials can be enhanced by fine-tuning the coordination environment and number of low-coordination atoms. Confinement engineering, which modulates electron transfer properties, atomic arrangement, and molecular structure in a confined region, is an effective strategy for precise chemical synthesis of electrocatalysts. It not only alters the coordination environments to adjust the formation mechanism of active centers, but also regulates the physicochemical properties of electrocatalysts. This optimization leads to improved performance in terms of activity, stability, and selectivity by optimizing the nucleation, transportation, and stabilization of intermediate species.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Heterogeneous-Interface-Enhanced Adsorption of Organic and Hydroxyl for Biomass Electrooxidation

Peng Zhou et al.

Summary: The CuO-PdO heterogeneous interface was successfully constructed, resulting in an advanced onset-potential and higher current density for the electrocatalytic oxidation of 5-hydroxymethylfurfural (HMF). The introduction of PdO enhanced the adsorption capacity of the organic molecule and promoted the adsorption and activation of OH- species at the CuO-PdO interface.

ADVANCED MATERIALS (2022)

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Article Chemistry, Physical

Bifunctional integrated electrode for high-efficient hydrogen production coupled with 5-hydroxymethylfurfural oxidation

Yuke Song et al.

Summary: This study demonstrates a bifunctional CoNiP nanosheet integrated electrode to boost the efficiency of the hydrogen evolution reaction (HER) and replace the oxygen evolution reaction (OER). The electrode exhibits high Faradaic efficiency for a specific oxidation reaction and low overpotential for HER, indicating its high efficiency. The findings suggest the potential application of this electrode in constructing an electrochemical device for efficient hydrogen generation coupled with biomass oxidation.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Physical

CoP-CoOOH heterojunction with modulating interfacial electronic structure: A robust biomass-upgrading electrocatalyst

Honglei Wang et al.

Summary: The modulation of the electron density at the interface leads to the formation of a heterojunction (CoP-CoOOH), which enhances the activity and efficiency of the 5-hydroxymethylfurfural (HMF) oxidation reaction. The coupling with a flow reactor overcomes the diffusion limitation and improves the selectivity and efficiency of the reaction at high concentrations.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Review Chemistry, Multidisciplinary

Recent advances in the design of single-atom electrocatalysts by defect engineering

Wei Li et al.

Summary: This study highlights the latest advances in designing single-atom catalysts through defect engineering, evaluates the effects of different support materials on catalytic performance, and discusses the current challenges and opportunities in the field.

FRONTIERS IN CHEMISTRY (2022)

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Article Chemistry, Physical

Nickel-vanadium-cobalt ternary layered double hydroxide for efficient electrocatalytic upgrading of 5-hydroxymethylfurfural to 2,5-furancarboxylic acid at low potential

Lifang Gao et al.

Summary: In this study, a NiVCo-LDHs catalyst was developed by introducing vanadium and cobalt into nickel (oxy)hydroxide for the electrocatalytic preparation of FDCA from HMF. The catalyst exhibited high oxidation current density and durability, and achieved high yield and faradaic efficiency at a low potential. Further investigation showed that the introduction of vanadium provided high intrinsic catalytic activity.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Article Chemistry, Multidisciplinary

Phosphorus vacancy-engineered Ce-doped CoP nanosheets for the electrocatalytic oxidation of 5-hydroxymethylfurfural

Jiahui Bi et al.

Summary: In this study, porous Ce-CoP nanosheets were designed through a deep eutectic solvent approach, and they achieved efficient electrooxidation of HMF to FDCA. In 1 M KOH electrolyte, the conversion of HMF, the yield of FDCA, and the faradaic efficiency were all at high levels.

CHEMICAL COMMUNICATIONS (2022)

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Article Engineering, Environmental

Nickel oxide nanoparticles with oxygen vacancies for boosting biomass-upgrading

Honglei Wang et al.

Summary: This study used a laser ablation strategy to fabricate oxygen-enriched nickel oxide catalysts with varying oxygen vacancy content for 5-hydroxymethylfurfural oxidation. The results showed that oxygen vacancies promoted low-valent Ni preoxidation and surface reconstruction, synergistically enhancing the oxidation reaction.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

CoP nanorods anchored on Ni2P-NiCoP nanosheets with abundant heterogeneous interfaces boosting the electrocatalytic oxidation of 5-hydroxymethyl-furfural

Mingjun Zhou et al.

Summary: This study reports a material composed of multiple metal phosphides embedded in N-doped carbon for efficient electrocatalytic oxidation of biomass-derived platform molecules. The material exhibits high FDCA yield and FE.

CATALYSIS SCIENCE & TECHNOLOGY (2022)

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Article Chemistry, Physical

Bimetallic sites and coordination effects: electronic structure engineering of NiCo-based sulfide for 5-hydroxymethylfurfural electrooxidation

Zhefei Zhao et al.

Summary: In this study, hierarchical NiCo-based sulfide nanosheets were used to investigate the role of dual-sites and coordinating anions in improving the electrocatalytic performance of HMF oxidation. The results showed that the Ni-Co dual sites and coordinating S species synergistically accelerated the reactions and lowered the energy barriers, leading to high catalytic activity and selectivity for FDCA generation.

CATALYSIS SCIENCE & TECHNOLOGY (2022)

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Article Chemistry, Physical

Biomass upgrading coupled with H2 production via a nonprecious and versatile Cu-doped nickel nanotube electrocatalyst

Lingxia Zheng et al.

Summary: Utilizing Cu-doped Ni nanotubes as an alloy catalyst enables efficient electrocatalytic oxidation of 5-hydroxymethylfurfural and simultaneous H-2 generation at a lower cell potential, demonstrating better energy consumption efficiency in a hybrid water splitting configuration. The catalyst maintains high reaction conversion and product selectivity even at high HMF concentrations, showcasing excellent catalytic activity and versatility for various organic substrates.

JOURNAL OF MATERIALS CHEMISTRY A (2022)

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Article Chemistry, Multidisciplinary

Boosting the electro-oxidation of 5-hydroxymethyl-furfural on a Co-CoSx heterojunction by intensified spin polarization

Jianmin Chen et al.

Summary: This study reports the fabrication of a yolk-shell polyhedron catalyst assembled with N-doped carbon nanotubes and embedded Co-CoSx nanoparticles for efficient HMF electrooxidation. The catalyst exhibits excellent activity and selectivity for HMF electrooxidation at low applied potential.

CHEMICAL SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Spectroscopic and Electrokinetic Evidence for a Bifunctional Mechanism of the Oxygen Evolution Reaction**

Lichen Bai et al.

Summary: The study experimentally validated two different mechanisms for oxygen evolution reaction catalysts: one is a bifunctional mechanism, and the other is a conventional four-step proton-coupled electron transfer mechanism.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Tuning the Selective Adsorption Site of Biomass on Co3O4 by Ir Single Atoms for Electrosynthesis

Yuxuan Lu et al.

Summary: The adsorption behavior of HMF on Co3O4 has been studied, and the adsorption energy can be tuned by decorating with single-atom Ir, enhancing the overall conversion efficiency of HMF on electrocatalysts.

ADVANCED MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Formic Acid Electro-Synthesis by Concurrent Cathodic CO2 Reduction and Anodic CH3OH Oxidation

Xinfa Wei et al.

Summary: This study presents a strategy for efficient formic acid synthesis by conducting concurrent cathodic CO2 reduction and anodic partial methanol oxidation reactions, resulting in significantly lowered potential and high Faraday efficiency in CO2 reduction.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

Ultrathin layered double hydroxides nanosheets array towards efficient electrooxidation of 5-hydroxymethylfurfural coupled with hydrogen generation

Yingjie Song et al.

Summary: An efficient integrated electrocatalyst based on ultrathin layered double hydroxides nanosheet array with abundant oxygen vacancies for the oxidation of organic compounds was reported. High faradaic efficiency at high potential and largely depressed oxygen evolution reaction process were achieved. Furthermore, a two-electrode electrolyzer assembled based on this electrocatalyst exhibited low voltage for organic oxidation, high hydrogen yield, and excellent stability.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Review Chemistry, Multidisciplinary

Innovative Protocols in the Catalytic Oxidation of 5-Hydroxymethylfurfural

Ting Su et al.

Summary: This Minireview discusses recent advancements in the catalytic oxidation of HMF to 2,5-furandicarboxylic acid (FDCA) and other intermediates using noble, non-noble, and metal-free systems deploying emerging protocols.

CHEMSUSCHEM (2021)

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Article Engineering, Environmental

Anion-cation-dual doped tremella-like nickel phosphides for electrocatalytic water oxidation

Xiaoli Jiang et al.

Summary: This research successfully synthesized N/Fe dual-doped nickel phosphides for the first time, showing significant improvement in electronic structure, surface states, and microtopography, leading to enhanced electrocatalytic performance. Computational simulations demonstrated that dual doping can optimize adsorption free energy and improve intrinsic electrocatalytic activity. Consequently, N/Fe-Ni2P/Ni12P5 exhibited outstanding OER performance and long-term durability at high current densities.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Engineering, Environmental

Refining d-band center in Ni0.85Se by Mo doping: A strategy for boosting hydrogen generation via coupling electrocatalytic oxidation 5-hydroxymethylfurfural

Chunming Yang et al.

Summary: The study found that Mo doping can increase the transmission speed of electrons within the catalyst, lower the d-band center of Ni in NF@Ni0.85Se, reduce H* adsorption energy, and promote the hydrogen evolution reaction (HER) and organic hydrogen adsorption process.

CHEMICAL ENGINEERING JOURNAL (2021)

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Article Chemistry, Multidisciplinary

Nanoengineered Electrodes for Biomass-Derived 5-Hydroxymethylfurfural Electrocatalytic Oxidation to 2, 5-Furandicarboxylic Acid

Dimitrios A. Giannakoudalds et al.

Summary: The electrochemical oxidation of HMF to FDCA presents a promising and sustainable alternative in the field of biomass valorization, with potential for higher efficiency through the rational design of nanocatalysts and nanoengineered anodes. Additionally, combining heterogeneous photocatalysis with photoelectrodes can reduce the reliance on external voltage and further enhance the overall reaction efficiency.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2021)

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Article Chemistry, Multidisciplinary

Regulating the Local Charge Distribution of Ni Active Sites for the Urea Oxidation Reaction

Liping Wang et al.

Summary: A tungsten-doped nickel catalyst (Ni-WOx) was developed with superior activity towards the urea oxidation reaction, accelerating the reaction kinetics and increasing the turnover frequency. Experimental results demonstrated that tungsten doping led to the formation of Ni3+ sites with superior activity, facilitating the catalytic reaction.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Selectively Upgrading Lignin Derivatives to Carboxylates through Electrochemical Oxidative C(OH)-C Bond Cleavage by a Mn-Doped Cobalt Oxyhydroxide Catalyst

Hua Zhou et al.

Summary: The study presents an efficient electrochemical strategy for upgrading lignin derivatives to carboxylates using MnCoOOH catalyst, with yields of 80-99% and operational stability up to 200 hours. A tandem oxidation mechanism is revealed, allowing for effective transformation of lignin derivatives into carboxylates.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Review Chemistry, Applied

2,5-Furandicarboxylic acid production via catalytic oxidation of 5-hydroxymethylfurfural: Catalysts, processes and reaction mechanism

Chunlin Chen et al.

Summary: The conversion of biomass into value-added chemicals, particularly using 5-hydroxymethylfurfural as a key platform molecule, has garnered significant attention. The oxidation product 2,5-furandicarboxylic acid shows promise as an alternative to petroleum-based terephthalic acid for the synthesis of biodegradable plastics.

JOURNAL OF ENERGY CHEMISTRY (2021)

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Article Chemistry, Physical

Understanding Hydrogen Atom and Hydride Transfer Processes during Electrochemical Alcohol and Aldehyde Oxidation

Michael T. Bender et al.

Summary: This study investigated the key factors and steps affecting the kinetics of two oxidation pathways by examining the pH and the concentration of aliphatic and aromatic alcohols and aldehydes. Through experiments and kinetic isotope effect studies, the researchers obtained a comprehensive mechanistic understanding of the two pathways. The ability of alcohols and aldehydes to outcompete OH- for adsorption on Ni4+ sites was proposed as a key predictor of which oxidation pathway will be favored.

ACS CATALYSIS (2021)

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Article Chemistry, Multidisciplinary

An Overall Reaction Integrated with Highly Selective Oxidation of 5-Hydroxymethylfurfural and Efficient Hydrogen Evolution

Yanan Xie et al.

Summary: The integration of thermodynamically favorable electrooxidation reactions of biomass derivatives with hydrogen evolution reaction has been demonstrated, yielding value-added chemicals and hydrogen simultaneously. Utilizing a hierarchically layered double hydroxide catalyst, the selective electrooxidation of 5-hydroxymethylfurfural into 2,5-furandicarboxylic acid was achieved with high efficiency and selectivity, indicating a promising new strategy for sustainable energy development.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Highly Efficient Electro-reforming of 5-Hydroxymethylfurfural on Vertically Oriented Nickel Nanosheet/Carbon Hybrid Catalysts: Structure-Function Relationships

Xingyu Lu et al.

Summary: The study demonstrates the promising prospect of Ni-promoted electrocatalytic biomass reforming in high value-added product synthesis and presents a novel hybrid catalyst of Ni nanosheet forests for efficient electrooxidation reactions.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Understanding the Roles of Electrogenerated Co3+ and Co4+ in Selectivity-Tuned 5-Hydroxymethylfurfural Oxidation

Xiaohui Deng et al.

Summary: The study demonstrates that Co3+ and Co4+ species in Co-based electrocatalyst play distinct roles in the electrochemical oxidation of 5-hydroxymethylfurfural (HMF), with Co4+ being crucial for the initial oxidation of hydroxyl groups. By tuning the applied potential, selective production of 5-hydroxymethyl-2-furancarboxylic acid and 2,5-furandicarboxylic acid can be achieved. This work provides essential mechanistic insights for Co-catalyzed organic oxidation reactions and may guide the design of more efficient electrocatalysts.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Defect-Rich High-Entropy Oxide Nanosheets for Efficient 5-Hydroxymethylfurfural Electrooxidation

Kaizhi Gu et al.

Summary: A low-temperature plasma strategy was used to prepare defect-rich HEOs nanosheets with high surface area, which showed improved catalytic activity for organic compound oxidation and outperformed HEOs prepared by high-temperature methods. This method provides new opportunities for synthesizing nanostructured HEOs with great potential applications.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

In Situ Growth of Ultrathin Ni(OH)2 Nanosheets as Catalyst for Electrocatalytic Oxidation Reactions

Jifang Zhang et al.

Summary: A method for growing ultrathin nickel hydroxide nanosheets on nickel foam has been developed for efficient oxidation of HMF to FDCA. Mechanistic studies reveal that FDCA is generated through two further oxidation steps.

CHEMSUSCHEM (2021)

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Article Chemistry, Physical

Nitrogen modulated NiMoO4 with enhanced activity for the electrochemical oxidation of 5-hydroxymethylfurfural to 2,5-furandicarboxylic acid

Wei Wang et al.

Summary: The study demonstrates the efficient electrocatalytic oxidation of 5-hydroxymethylfurfural (HMF) to 2,5-furandicarboxylic acid (FDCA) using nitrogen-modulated NiMoO4 growth on Ni foam. The nitrogen-modulated catalyst shows high conversion rate, yield, and efficiency in comparison to NiMoO4. This work provides insights into tuning the activity of catalysts for biomass refineries.

CATALYSIS SCIENCE & TECHNOLOGY (2021)

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Article Chemistry, Multidisciplinary

Platinum Modulates Redox Properties and 5-Hydroxymethylfurfural Adsorption Kinetics of Ni(OH)2 for Biomass Upgrading

Bo Zhou et al.

Summary: In this study, platinum modification of nickel hydroxide improved the current density of the 5-hydroxymethylfurfural oxidation reaction (HMFOR) and optimized the formation of active Ni(OH)O species. Platinum also reduced the adsorption energy of HMF, enhancing the catalytic process.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Physical

Surface reconstruction of NiCoP for enhanced biomass upgrading

Honglei Wang et al.

Summary: The cactus-like NiCoP nanoplate prepared as a robust electrocatalyst enables the oxidation of 5-hydroxymethylfurfural (HMF) into 2,5-furandicarboxylic acid (FDCA) at high concentration. In situ Raman spectroelectrochemical analysis reveals the dynamic structural evolution of the NiCoP surface during the electrooxidation of HMF. The flow-through mode reactor design optimizes mass transfer processes, leading to high conversion rates and yields of HMF and FDCA, especially at high HMF concentrations up to 300 mM.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Physical

Construction of a hierarchically structured, NiCo-Cu-based trifunctional electrocatalyst for efficient overall water splitting and 5-hydroxymethylfurfural oxidation

Ruijuan Zheng et al.

Summary: Cu nanowire arrays grown on a three-dimensional Cu foam substrate are modified by nickel-cobalt layered double hydroxide nanosheets, forming a self-supporting trifunctional electrocatalyst with excellent performance in alkaline solution for efficient water electrolysis.

SUSTAINABLE ENERGY & FUELS (2021)

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Review Chemistry, Multidisciplinary

Electrochemical oxidation of biomass derived 5-hydroxymethylfurfural (HMF): pathway, mechanism, catalysts and coupling reactions

Yuechao Yang et al.

Summary: Electrochemical conversion is becoming a powerful and promising method for producing high-value chemicals, particularly the electrooxidation of HMF to FDCA which may replace petroleum-based PET. This review discusses the reaction pathway/mechanism, catalysts, and coupling reactions of HMF electrochemical oxidation, providing insights for utilizing and producing renewable resources.

GREEN CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Rational incorporation of defects within metal-organic frameworks generates highly active electrocatalytic sites

Nina Heidary et al.

Summary: Metal-organic frameworks (MOFs) offer unparalleled control over catalytically active sites in heterogeneous electrocatalysis. By utilizing organic linkers to generate coordinatively-unsaturated active sites, the electrocatalytic activity can be enhanced, leading to improved conversion efficiency in model reactions.

CHEMICAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

Electrochemical upgrading of biomass-derived 5-hydroxymethylfurfural and furfural over oxygen vacancy-rich NiCoMn-layered double hydroxides nanosheets

Biying Liu et al.

Summary: A highly efficient ternary NiCoMn-layered double hydroxides (NiCoMn-LDHs) nanosheet catalyst with oxygen vacancy-rich properties has been developed for the electrooxidation of HMF and furfural to FDCA and FurAc, showing high yields and good faradaic efficiency. The mechanism for its superior performance lies in the exposure of more active sites with oxygen vacancies, promoting synergistic effects between HMF and furfural oxidation reactions.

GREEN CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Electrochemical biomass upgrading on CoOOH nanosheets in a hybrid water electrolyzer

Ruya Zhang et al.

Summary: By utilizing cobalt oxyhydroxide (CoOOH) nanosheets as the anodic electrocatalyst in a hybrid water electrolyzer with 5-hydroxymethylfurfural, a high value product of 2,5-furandicarboxylic acid can be produced on the anode with high conversion, selectivity, and Faraday efficiency at a low operating voltage of approximately 1.423 V.

GREEN CHEMISTRY (2021)

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Article Chemistry, Multidisciplinary

Sulfur Vacancy-Promoted Highly Selective Electrosynthesis of Functionalized Aminoarenes via Transfer Hydrogenation of Nitroarenes with H2O over a Co3S4- x Nanosheet Cathode

Yige Zhao et al.

Summary: A selective hydrogenation strategy utilizing H2O as the hydrogen source, combined with the design of sulfur vacancies, has been demonstrated to be highly efficient in converting nitroarenes to aminoarenes at low potential using Ti mesh-supported Co3S4 ultrathin nanosheets. This method shows outstanding selectivity and compatibility with highly reducible functional groups.

CCS CHEMISTRY (2021)

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Article Multidisciplinary Sciences

Potential-tuned selective electrosynthesis of azoxy-, azo- and amino-aromatics over a CoP nanosheet cathode

Xiaodan Chong et al.

NATIONAL SCIENCE REVIEW (2020)

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Article Chemistry, Multidisciplinary

Synergistically Tuning Electronic Structure of Porous β-Mo2C Spheres by Co Doping and Mo-Vacancies Defect Engineering for Optimizing Hydrogen Evolution Reaction Activity

Yufei Ma et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Hydration-Effect-Promoting Ni-Fe Oxyhydroxide Catalysts for Neutral Water Oxidation

Ning Wang et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Physical

NiSe@NiOx core-shell nanowires as a non-precious electrocatalyst for upgrading 5-hydroxymethylfurfural into 2,5-furandicarboxylic acid

Lifang Gao et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Review Chemistry, Multidisciplinary

Defect Engineering for Fuel-Cell Electrocatalysts

Wei Li et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Interfacial Engineering of MoO2-FeP Heterojunction for Highly Efficient Hydrogen Evolution Coupled with Biomass Electrooxidation

Ganceng Yang et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Identifying the Transfer Kinetics of Adsorbed Hydroxyl as a Descriptor of Alkaline Hydrogen Evolution Reaction

Baoguang Mao et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Multidisciplinary

Hierarchically nanostructured NiO-Co3O4 with rich interface defects for the electro-oxidation of 5-hydroxymethylfurfural

Yuxuan Lu et al.

SCIENCE CHINA-CHEMISTRY (2020)

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Article Chemistry, Physical

Mechanistic Investigation of Biomass Oxidation Using Nickel Oxide Nanoparticles in a CO2-Saturated Electrolyte for Paired Electrolysis

Seungwoo Choi et al.

JOURNAL OF PHYSICAL CHEMISTRY LETTERS (2020)

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Article Chemistry, Physical

Trimetallic NiCoFe-Layered Double Hydroxides Nanosheets Efficient for Oxygen Evolution and Highly Selective Oxidation of Biomass-Derived 5-Hydroxymethylfurfural

Man Zhang et al.

ACS CATALYSIS (2020)

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Article Chemistry, Physical

4-Nitrophenol Reduction: Probing the Putative Mechanism of the Model Reaction

Jyah Strachan et al.

ACS CATALYSIS (2020)

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Article Chemistry, Multidisciplinary

Identifying the Geometric Site Dependence of Spinel Oxides for the Electrooxidation of 5-Hydroxymethylfurfural

Yuxuan Lu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Physical

The vital role of surface Bronsted acid/base sites for the photocatalytic formation of free •OH radicals

Liyong Ding et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Engineering, Chemical

Improved Performance of Nickel Boride by Phosphorus Doping as an Efficient Electrocatalyst for the Oxidation of 5-Hydroxymethylfurfural to 2,5-Furandicarboxylic Acid

Xiaojie Song et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2020)

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Review Chemistry, Physical

Defect Chemistry in Heterogeneous Catalysis: Recognition, Understanding, and Utilization

Chao Xie et al.

ACS CATALYSIS (2020)

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Article Chemistry, Multidisciplinary

Activity Origins and Design Principles of Nickel-Based Catalysts for Nucleophile Electrooxidation

Wei Chen et al.

CHEM (2020)

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Article Chemistry, Multidisciplinary

Unraveling Two Pathways for Electrochemical Alcohol and Aldehyde Oxidation on NiOOH

Michael T. Bender et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Multidisciplinary

Ni, Co hydroxide triggers electrocatalytic production of high-purity benzoic acid over 400 mA cm-2

Hongling Huang et al.

ENERGY & ENVIRONMENTAL SCIENCE (2020)

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Article Chemistry, Multidisciplinary

Sustainable 2,5-furandicarboxylic synthesis by a direct 5-hydroxymethylfurfural fuel cell based on a bifunctional PtNiSx catalyst

Jialu Wang et al.

CHEMICAL COMMUNICATIONS (2020)

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Article Chemistry, Multidisciplinary

Topotactically Transformed Polygonal Mesopores on Ternary Layered Double Hydroxides Exposing Under-Coordinated Metal Centers for Accelerated Water Dissociation

Hao Sun et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Physical

Two-dimensional metal-organic framework nanosheets for highly efficient electrocatalytic biomass 5-(hydroxymethyl)furfural (HMF) valorization

Mengke Cai et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Chemistry, Multidisciplinary

Electrochemical biomass valorization on gold-metal oxide nanoscale heterojunctions enables investigation of both catalyst and reaction dynamics with operando surface-enhanced Raman spectroscopy

Nina Heidary et al.

CHEMICAL SCIENCE (2020)

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Article Chemistry, Physical

Electrocatalysis of 5-hydroxymethylfurfural at cobalt based spinel catalysts with filamentous nanoarchitecture in alkaline media

Myung Jong Kang et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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Article Chemistry, Multidisciplinary

Paired Electrocatalytic Oxygenation and Hydrogenation of Organic Substrates with Water as the Oxygen and Hydrogen Source

Peili Zhang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Chemistry, Physical

Facile synthesis of petal-like NiCo/NiO-CoO/nanoporous carbon composite based on mixed-metallic MOFs and their application for electrocatalytic oxidation of methanol

Sharifeh Rezaee et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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Article Chemistry, Multidisciplinary

Continuous-Flow Oxidation of HMF to FDCA by Resin-Supported Platinum Catalysts in Neat Water

Francesca Liguori et al.

CHEMSUSCHEM (2019)

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Review Chemistry, Multidisciplinary

Understanding the Roadmap for Electrochemical Reduction of CO2 to Multi-Carbon Oxygenates and Hydrocarbons on Copper-Based Catalysts

Yao Zheng et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Energy & Fuels

Co-electrolysis of CO2 and glycerol as a pathway to carbon chemicals with improved technoeconomics due to low electricity consumption

Sumit Verma et al.

NATURE ENERGY (2019)

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Review Chemistry, Multidisciplinary

Progress and Perspectives of Electrochemical CO2 Reduction on Copper in Aqueous Electrolyte

Stephanie Nitopi et al.

CHEMICAL REVIEWS (2019)

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Review Materials Science, Multidisciplinary

Insight into the design of defect electrocatalysts: From electronic structure to adsorption energy

Chao Xie et al.

MATERIALS TODAY (2019)

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Article Chemistry, Multidisciplinary

Electrochemical Valorization of Glycerol on Ni-Rich Bimetallic NiPd Nanoparticles: Insight into Product Selectivity Using in Situ Polarization Modulation Infrared-Reflection Absorption Spectroscopy

Mohamed S. E. Houache et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2019)

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Article Chemistry, Multidisciplinary

Biomass Valorization via Paired Electrosynthesis Over Vanadium Nitride-Based Electrocatalysts

Suiqin Li et al.

ADVANCED FUNCTIONAL MATERIALS (2019)

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Article Chemistry, Multidisciplinary

Electrochemically Determined O-H Bond Dissociation Free Energies of NiO Electrodes Predict Proton-Coupled Electron Transfer Reactivity

Catherine F. Wise et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Multidisciplinary

Single-Crystal Cobalt Phosphate Nanosheets for Biomimetic Oxygen Evolution in Neutral Electrolytes

Yue Shao et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Review Chemistry, Multidisciplinary

Electrochemical Oxidation of 5-Hydroxymethylfurfural on Nickel Nitride/Carbon Nanosheets: Reaction Pathway Determined by In Situ Sum Frequency Generation Vibrational Spectroscopy

Nana Zhang et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2019)

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Article Multidisciplinary Sciences

Boosting selective nitrogen reduction to ammonia on electron-deficient copper nanoparticles

Yun-Xiao Lin et al.

NATURE COMMUNICATIONS (2019)

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Article Chemistry, Multidisciplinary

Schottky Barrier Induced Coupled Interface of Electron-Rich N-Doped Carbon and Electron-Deficient Cu: In-Built Lewis Acid-Base Pairs for Highly Efficient CO2 Fixation

Yong-Xing Liu et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2019)

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Article Chemistry, Physical

A Comparative Study of Nickel, Cobalt, and Iron Oxyhydroxide Anodes for the Electrochemical Oxidation of 5-Hydroxymethylfurfural to 2,5-Furandicarboxylic Acid

Brandon J. Taitt et al.

ACS CATALYSIS (2019)

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Article Chemistry, Physical

Ruthenium(iii) polyethyleneimine complexes for bifunctional ammonia production and biomass upgrading

Guang-Rui Xu et al.

JOURNAL OF MATERIALS CHEMISTRY A (2019)

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Article Chemistry, Multidisciplinary

Electrocatalytic Oxidation of 5-(Hydroxymethyl)furfural Using High-Surface-Area Nickel Boride

Stefan Barwe et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2018)

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Article Chemistry, Multidisciplinary

Bleaching'' glycerol in a microfluidic fuel cell to produce high power density at minimal cost

Caue A. Martins et al.

CHEMICAL COMMUNICATIONS (2018)

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Article Chemistry, Multidisciplinary

Electrochemical Oxidation of 5-Hydroxymethylfurfural to 2,5-Furandicarboxylic Acid (FDCA) in Acidic Media Enabling Spontaneous FDCA Separation

Stephen R. Kubota et al.

CHEMSUSCHEM (2018)

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Article Electrochemistry

Continuous electrochemical oxidation of biomass derived 5-(hydroxymethyl)furfural into 2,5-furandicarboxylic acid

R. Latsuzbaia et al.

JOURNAL OF APPLIED ELECTROCHEMISTRY (2018)

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Review Chemistry, Physical

Recent Advances in C-H Functionalization Using Electrochemical Transition Metal Catalysis

Cong Ma et al.

ACS CATALYSIS (2018)

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Article Chemistry, Physical

Nitrogen-promoted molybdenum dioxide nanosheets for electrochemical hydrogen generation

Junqing Yan et al.

JOURNAL OF MATERIALS CHEMISTRY A (2018)

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Article Chemistry, Multidisciplinary

Ultrathin Sulfur-Doped Graphitic Carbon Nitride Nanosheets As Metal-Free Catalyst for Electrochemical Sensing and Catalytic Removal of 4-Nitrophenol

Chellakannu Rajkumar et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2018)

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Article Chemistry, Physical

Complete electron economy by pairing electrolysis with hydrogenation

Rebecca S. Sherbo et al.

NATURE CATALYSIS (2018)

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Article Chemistry, Physical

Solar energy-driven lignin-first approach to full utilization of lignocellulosic biomass under mild conditions

Xuejiao Wu et al.

NATURE CATALYSIS (2018)

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Article Chemistry, Multidisciplinary

MnCo2O4 spinel supported ruthenium catalyst for air-oxidation of HMF to FDCA under aqueous phase and base-free conditions

Dinesh Kumar Mishra et al.

GREEN CHEMISTRY (2017)

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Article Chemistry, Multidisciplinary

Visible-Light-Driven Valorization of Biomass Intermediates Integrated with H2 Production Catalyzed by Ultrathin Ni/CdS Nanosheets

Guanqun Han et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2017)

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Article Chemistry, Physical

The path towards sustainable energy

Steven Chu et al.

NATURE MATERIALS (2017)

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Review Multidisciplinary Sciences

Combining theory and experiment in electrocatalysis: Insights into materials design

Zhi Wei Seh et al.

SCIENCE (2017)

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Article Chemistry, Multidisciplinary

A Modular Flow Design for the meta-Selective C-H Arylation of Anilines

Hannes P. L. Gemoets et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017)

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Article Chemistry, Multidisciplinary

Electrocatalytic Synthesis of Ammonia at Room Temperature and Atmospheric Pressure from Water and Nitrogen on a Carbon-Nanotube-Based Electrocatalyst

Shiming Chen et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2017)

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Article Chemistry, Multidisciplinary

Simultaneous H2 Generation and Biomass Upgrading in Water by an Efficient Noble-Metal-Free Bifunctional Electrocatalyst

Bo You et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2016)

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Review Chemistry, Multidisciplinary

Heterogeneously Catalyzed Hydrothermal Processing of C5-C6 Sugars

Xingguang Zhang et al.

CHEMICAL REVIEWS (2016)

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Article Chemistry, Multidisciplinary

A General Strategy for Decoupled Hydrogen Production from Water Splitting by Integrating Oxidative Biomass Valorization

Bo You et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2016)

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Article Chemistry, Physical

Electrocatalytic Conversion of Furanic Compounds

Youngkook Kwon et al.

ACS CATALYSIS (2016)

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Article Chemistry, Physical

P doped molybdenum dioxide on Mo foil with high electrocatalytic activity for the hydrogen evolution reaction

Xiao Xie et al.

JOURNAL OF MATERIALS CHEMISTRY A (2016)

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Article Chemistry, Physical

Interfacial effects on the catalysis of the hydrogen evolution, oxygen evolution and CO2-reduction reactions for (co-)electrolyzer development

Juan Herranz et al.

NANO ENERGY (2016)

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Article Polymer Science

Bio-based alternatives in the synthesis of aliphatic-aromatic polyesters dedicated to biodegradable film applications

Nicolas Jacquel et al.

POLYMER (2015)

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Article Chemistry, Physical

Recent Advances in the Catalytic Synthesis of 2,5-Furandicarboxylic Acid and Its Derivatives

Zehui Zhang et al.

ACS CATALYSIS (2015)

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Article Chemistry, Multidisciplinary

Electrocatalytic oxidation of 5-hydroxymethylfurfural to 2,5-furandicarboxylic acid on supported Au and Pd bimetallic nanoparticles

David J. Chadderdon et al.

GREEN CHEMISTRY (2014)

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Article Chemistry, Multidisciplinary

Efficient Reduction of CO2 to CO with High Current Density Using in Situ or ex Situ Prepared Bi-Based Materials

Jonnathan Medina-Ramos et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2014)

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Article Chemistry, Applied

Oxidation of biomass derived 5-hydroxymethylfurfural using heterogeneous and electrochemical catalysis

Koteswara Rao Vuyyuru et al.

CATALYSIS TODAY (2012)

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Review Chemistry, Multidisciplinary

Conversion of biomass to selected chemical products

Pierre Gallezot

CHEMICAL SOCIETY REVIEWS (2012)

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Article Chemistry, Multidisciplinary

On the mechanism of selective oxidation of 5-hydroxymethylfurfural to 2,5-furandicarboxylic acid over supported Pt and Au catalysts

Sara E. Davis et al.

GREEN CHEMISTRY (2012)

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Article Chemistry, Physical

Trends in activity for the water electrolyser reactions on 3d M(Ni,Co,Fe,Mn) hydr(oxy)oxide catalysts

Ram Subbaraman et al.

NATURE MATERIALS (2012)

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Review Multidisciplinary Sciences

Valorization of Biomass: Deriving More Value from Waste

Christopher O. Tuck et al.

SCIENCE (2012)

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Review Chemistry, Multidisciplinary

Ionic Liquid-Mediated Formation of 5-Hydroxymethylfurfural-A Promising Biomass-Derived Building Block

Malgorzata E. Zakrzewska et al.

CHEMICAL REVIEWS (2011)

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Article Multidisciplinary Sciences

Future CO2 Emissions and Climate Change from Existing Energy Infrastructure

Steven J. Davis et al.

SCIENCE (2010)

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Article Engineering, Chemical

Biomass-Derived Platform Chemicals: Thermodynamic Studies on the Conversion of 5-Hydroxymethylfurfural into Bulk Intermediates

Sergey P. Verevkin et al.

INDUSTRIAL & ENGINEERING CHEMISTRY RESEARCH (2009)

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Article Physics, Multidisciplinary

Scaling properties of adsorption energies for hydrogen-containing molecules on transition-metal surfaces

F. Abild-Pedersen et al.

PHYSICAL REVIEW LETTERS (2007)

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Article Multidisciplinary Sciences

Phase modifiers promote efficient production of hydroxymethylfurfural from fructose

Yuriy Roman-Leshkov et al.

SCIENCE (2006)

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Article Electrochemistry

Trends in the exchange current for hydrogen evolution

JK Norskov et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2005)

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Article Chemistry, Physical

Origin of the overpotential for oxygen reduction at a fuel-cell cathode

JK Norskov et al.

JOURNAL OF PHYSICAL CHEMISTRY B (2004)

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