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Long-term heat-storage materials based on λ-Ti3O5 for green transformation (GX)

CHEMICAL COMMUNICATIONS (2023)

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Article Chemistry, Multidisciplinary

Direct Synthesis of Metastable λ-Phase Ti3O5 Films on LaAIO3 (110) Substrates at High Temperatures

Kohei Yoshimatsu et al.

Summary: High-quality metastable lambda-phase trititanium pentoxide (λ-Ti3O5) films were grown at very high temperatures via pulsed-laser deposition, directly on the substrate surface without transient layers. The monoclinic lambda-Ti3O5 films obtained were nearly single-domain with less than 1% rotational domains on pseudocubic LaAlO3 substrates. The successful synthesis of these films enables the utilization of their rich functionalities.

CRYSTAL GROWTH & DESIGN (2022)

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Article Chemistry, Physical

First-Principles Investigation of Electronic Properties and Phase Transition of Ti3O5

Stefan Juetten et al.

Summary: In this study, the electronic ground state and phase transition mechanism of trititanium pentoxide were comprehensively investigated using the new r(2)SCAN-D3 method. The study found that the r(2)SCAN-D3 method demonstrates good performance in both computational efficiency and accuracy. The inclusion of dispersion interactions is essential for obtaining correct energy differences between the phases. This method is recommended for high-throughput investigations of heat storage materials.

JOURNAL OF PHYSICAL CHEMISTRY C (2022)

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Article Materials Science, Multidisciplinary

Could λ-Ti3O5 with lamellar and channel microstructure characteristics determine the excellent properties of LIBs? The first-principles study of λ-Ti3O5 lithiation mechanism

Danmin Peng et al.

Summary: This study investigates the influence of microstructure characteristics on the electrochemical properties of lambda-Ti3O5 as an electrode material for Li-ion batteries. DFT simulations reveal that lambda-Ti3O5 exhibits good stability during lithiation, but its microstructure has a relatively small impact on Li-ion diffusion performance.

MATERIALS TODAY COMMUNICATIONS (2022)

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Review Chemistry, Physical

Realistic pathways to decarbonization of building energy systems

Srinivas Garimella et al.

Summary: This paper discusses the impact of rapid electrification on the decarbonization of the energy sector and emphasizes the role of the electricity grid. The challenges in the building energy sector and potential solutions are also discussed. The study finds that a significant reduction in building energy usage and carbon emissions can be achieved through the adoption of carbon-free thermal energy and efficient management technologies.

JOULE (2022)

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Article Engineering, Environmental

Intelligent coating based on metal-insulator transitional Ti3O5 towards fire sensing and protection

Shuai Zhang et al.

Summary: With the acceleration of urbanization, energy-efficient, comfortable, and lightweight materials have been widely used. This paper develops a sensitive and durable fire alarm intelligent coating strategy based on a metal-insulator transitional Ti3O5, and elucidates its atomic and electronic structure. The coating demonstrates a sensitive fire response time and excellent response repeatability, as well as remarkable flame retardancy, smoke suppression, and weatherability.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Materials Science, Multidisciplinary

Pressure effect on long-term heat storage ceramics based on Mg-substituted λ-Ti3O5

Shin-ichi Ohkoshi et al.

Summary: This study reports a new type of heat-storage material, a ceramic that can store latent heat for a prolonged period and release heat by applying pressure. The Mg-substituted trititanium pentoxide undergoes a phase transition under pressure, allowing for temperature control of the heat storage. This material exhibits high heat storage capacity and is suitable for storage of waste heat from industries and power plants, making it effective for sustainable reuse of wasted heat energy.

MATERIALS ADVANCES (2022)

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Article Materials Science, Multidisciplinary

Selection rule for the photoinduced phase transition dominated by anisotropy of strain in Ti3O5

Takuo Saiki et al.

Summary: The relation between crystal orientation and the direction of light polarization or wave vector is important in photoinduced phase transitions, but there is a lack of experimental studies in this direction. Ti3O5 undergoes a structural phase transition involving the migration of Ti and O ions, and its nanocrystals exhibit persistent photoinduced phase transitions. We found that the occurrence of photoinduced phase transitions in a single crystal of this compound significantly depends on the orientation of the irradiated plane, which is determined by the anisotropy of the strain associated with the phase transition.

PHYSICAL REVIEW B (2022)

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Article Chemistry, Multidisciplinary

Direct Synthesis of Metastable lambda-Phase Ti3O5 Films on LaAIO(3) (110) Substrates at High Temperatures

Kohei Yoshimatsu et al.

Summary: High-quality metastable lambda-phase trititanium pentoxide films were successfully grown on substrates via pulsed-laser deposition at very high growth temperature. These films directly formed on substrates without any detectable transient layers, containing almost single domains with very low fraction of rotational domains. The successful synthesis of these metastable films enables the utilization of their rich functionalities.

CRYSTAL GROWTH & DESIGN (2022)

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Article Multidisciplinary Sciences

Strain wave pathway to semiconductor-to-metal transition revealed by time-resolved X-ray powder diffraction

C. Mariette et al.

Summary: Researchers have used femtosecond powder X-ray diffraction to study the transition from semiconductor to metal in Ti3O5 nanocrystals, finding that strain waves and electronic precursor phenomena determine the transformation pathway. The study demonstrates that in nanocrystals, picosecond switching occurs simultaneously with the propagating acoustic wavefront.

NATURE COMMUNICATIONS (2021)

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Article Metallurgy & Metallurgical Engineering

Progress in Ti3O5: Synthesis, properties and applications

Peng-fei Zhao et al.

Summary: Research on the crystal structure, physical, chemical, and phase transition properties of trititanium pentoxide (Ti3O5) has been ongoing since the 1950s, with different crystalline forms exhibiting various properties. Of particular interest are the reversible phase transitions between lambda- and beta-Ti3O5, which have potential applications in energy and data storage. Recent advancements have also shown Ti3O5 materials performing well in trace detection, microwave absorption, and virus adsorption, expanding their application fields.

TRANSACTIONS OF NONFERROUS METALS SOCIETY OF CHINA (2021)

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Article Chemistry, Physical

Ti3O5 nanofilm on carbon nanotubes by pulse laser deposition: Enhanced electrochemical performance

Peng Sun et al.

Summary: A pulsed laser deposition process was developed to grow Ti3O5 nanofilm on highly conductive carbon nanotube networks under vacuum condition, resulting in a high specific capacitance of 445.7F g(-1) at 1 A g(-1) for the Ti3O5@CNTs/Ni hybrid composite. Density functional theory calculations showed that combining Ti3O5 and CNTs can improve the conductivity of the composites by increasing the number of near-conduction bands, enhancing the electrochemical activity.

APPLIED SURFACE SCIENCE (2021)

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Article Chemistry, Physical

A Study on the Characteristic and Antibacterial Activity of Ti3Ox Thin Films

Endrika Widyastuti et al.

Summary: The study successfully synthesized Ti3Ox thin films using the HiPIMS method without the need for post-annealing, showing excellent photocatalytic and antibacterial activity, with two co-existing phases.

CATALYSTS (2021)

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Article Materials Science, Multidisciplinary

Electron-phonon interaction in TinO2n-1 using first-principles calculations

S. Vahid Hosseini et al.

Summary: The present study investigated the electronic, phonon, and electron-phonon interactions of titanium suboxide structures using density-functional theory. The mechanism of superconductivity in these materials appears to be phonon mediated, possibly with participation of paramagnetic spin fluctuations. Pressure influences the superconducting transition temperature (TC) of cubic TiO and Ti4O7 through this mechanism.

PHYSICAL REVIEW B (2021)

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Article Materials Science, Multidisciplinary

Preparing high purity λ-Ti3O5 and Li/λ-Ti3O5 as high-performance electromagnetic wave absorbers

Xiankai Fu et al.

Summary: This paper introduces a new candidate material, lambda-Ti3O5, for microwave absorption. It explains that Li has the strongest stabilizing effect on lambda-Ti3O5, and both lambda-Ti3O5 and Li/lambda-Ti3O5 exhibit good microwave absorption properties. Additionally, a strategy using the number of states of the micro-electric field to predict microwave absorption properties of materials is proposed.

JOURNAL OF MATERIALS CHEMISTRY C (2021)

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Article Materials Science, Multidisciplinary

Evidence for bandwidth-control metal-insulator transition in Ti3O5

Xian-Kai Fu et al.

COMPUTATIONAL MATERIALS SCIENCE (2020)

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Article Physics, Applied

Non-metallic electrical transport properties of a metastable λ-Ti3O5 thin film epitaxially stabilized on a pseudobrookite seed layer

Hao Chen et al.

APPLIED PHYSICS LETTERS (2020)

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Article Electrochemistry

One-step electrochemical deposition of thin film titanium suboxide in basic titanyl sulfate solution at room temperature

Zeliha Ertekin et al.

JOURNAL OF SOLID STATE ELECTROCHEMISTRY (2020)

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Article Chemistry, Physical

Synthesis of nanoscale lambda-Ti3O5 via a PEG assisted sol-gel method

Yu Cai et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2020)

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Article Multidisciplinary Sciences

Long-term heat-storage ceramics absorbing thermal energy from hot water

Yoshitaka Nakamura et al.

SCIENCE ADVANCES (2020)

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Article Materials Science, Multidisciplinary

Structural, magnetic, transport, and thermoelectric properties of the pseudobrookite AlTi2O5-Ti3O5 system

Ryusei Takahama et al.

PHYSICAL REVIEW MATERIALS (2020)

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Article Chemistry, Physical

Synthesis of λ-Ti3O5 nanocrystals using a block copolymer

Y. Araki et al.

MATERIALS TODAY ENERGY (2020)

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Article Chemistry, Physical

Phase evolution and formation of λ phase in Ti3O5 induced by magnesium doping

Mingzhe Wang et al.

JOURNAL OF ALLOYS AND COMPOUNDS (2019)

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Article Multidisciplinary Sciences

Low-pressure-responsive heat-storage ceramics for automobiles

Shin-ichi Ohkoshi et al.

SCIENTIFIC REPORTS (2019)

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Article Physics, Multidisciplinary

First-principles investigation on elastic, electronic, and optical properties of Ti3O5

Fu Xian-Kai et al.

ACTA PHYSICA SINICA (2019)

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Theoretical prediction of a charge-transfer phase transition

Hiroko Tokoro et al.

SCIENTIFIC REPORTS (2018)

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Article Materials Science, Multidisciplinary

Dielectric and optical constants of λ-Ti3O5 film measured by spectroscopic ellipsometry

Fumiyoshi Hakoe et al.

MATERIALS LETTERS (2017)

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Article Materials Science, Multidisciplinary

Self-induced preparation of Ti3O5 nanorods by chemical vapor deposition

Wenqian Qi et al.

VACUUM (2017)

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Article Physics, Applied

Stabilization of microcrystal λ-Ti3O5 at room temperature by aluminum-ion doping

Zujia Shen et al.

APPLIED PHYSICS LETTERS (2017)

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Article Chemistry, Physical

Time-Resolved X-Ray Powder Diffraction Study of Photoinduced Phase Transitions in Ti3O5 Nanoparticles

Kelin R. Tasca et al.

CHEMPHYSCHEM (2017)

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Electronic structure and correlation in β-Ti3O5 and λ-Ti3O5 studied by hard x-ray photoelectron spectroscopy

Keisuke Kobayashi et al.

PHYSICAL REVIEW B (2017)

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Innovative carbon-free low content Pt catalyst supported on Mo-doped titanium suboxide (Ti3O5-Mo) for stable and durable oxygen reduction reaction

Reza Alipour Moghadam Esfahani et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2017)

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Preparation and oxygen sensing properties of Ti3O5 submicron rods

Xiaoyan Zhang et al.

MICRO & NANO LETTERS (2016)

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Fabrication of nanocrystalline λ-Ti3O5 with tunable terahertz wave transmission properties across a temperature induced phase transition

Qiwu Shi et al.

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Cathodic electrochemical deposition of Magneli phases TinO2n-1 thin films at different temperatures in acetonitrile solution

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Preparation and characterization of λ-Ti3O5 by carbothermal reduction of TiO2

Guoqing Chai et al.

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Ab initio study of the low-pressure phases of Ti3O5

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New metastable phases in a trititanium pentoxide compound

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MATERIALS RESEARCH EXPRESS (2015)

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Single-shot time resolved study of the photo-reversible phase transition induced in flakes of Ti3O5 nanoparticles at room temperature

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CHEMICAL PHYSICS LETTERS (2014)

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Electronic, magnetic and optical properties of beta-Ti3O5 and lambda-Ti3O5: A density functional study

Rui Liu et al.

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Hierarchically Porous Monoliths Based on N-Doped Reduced Titanium Oxides and Their Electric and Electrochemical Properties

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Preparation and Optical Storage Properties of λ-Ti3O5 Powder

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Selective Preparation of Macroporous Monoliths of Conductive Titanium Oxides TinO2n-1 (n=2, 3, 4, 6)

Atsushi Kitada et al.

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First-principles study of thermal properties and phase transition between β-Ti3O5 and λ-Ti3O5

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