The first enantioselective total syntheses of six natural and two proposed meroterpenoids from Psoralea corylifolia have been achieved in 7-9 steps from 2-methylcyclohexanone. These synthetic approaches offer a high level of flexibility, stereodivergent fashion, and short route, providing a potential platform for the preparation of various this-type meroterpenoids and their pseudo-natural products.
The first enantioselective total syntheses of six natural and two proposed meroterpenoids isolated from Psoralea corylifolia have been achieved in 7-9 steps from 2-methylcyclohexanone. The current synthetic approaches feature a high level of synthetic flexibility, stereodivergent fashion and short synthetic route, thereby providing a potential platform for the preparation of numerous this-type meroterpenoids and their pseudo-natural products.
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