期刊
CHEMICAL COMMUNICATIONS
卷 59, 期 37, 页码 5579-5582出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d3cc01121f
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An organocatalytic photoinduced 1,2-carbofunctionalization strategy has been developed that enables regioselective and efficient 1,2-carboisothiocyanation of conjugated dienes without the need for exogenous photocatalysts or additives. The reaction is proposed to proceed through EDA complexation between the diene and TMSNCS.
An organocatalytic photoinduced 1,2-carbofunctionalization strategy for conjugated dienes has been developed. No exogenous photocatalyst or additives are required in this mild protocol and it allows for highly regioselective and efficient 1,2-carboisothiocyanation through the coupling of a diene, an alkyl radical and TMSNCS. The reaction is proposed to proceed through EDA complexation between the diene and TMSNCS.
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