期刊
ENERGY & ENVIRONMENTAL SCIENCE
卷 16, 期 8, 页码 3240-3301出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/d3ee01344h
关键词
-
Manganese-based materials are considered as promising cathode materials for zinc-ion batteries. This review focuses on the modification strategies that can significantly change the electronic structure of these materials, and proposes a top-down methodology for electrochemical performance optimization. The comparison of different modification methods and evaluation of their applicability and economy are also discussed.
Manganese-based materials are considered as one of the most promising energy storage cathode materials for zinc-ion batteries (ZIBs). To achieve major breakthroughs in commercialization, optimizing their poor inherent performance through various modification methods has attracted extensive attention. The previous reviews have mainly focused on the improvement of electrochemical performance and specific means but lack a discussion of the common internal mechanisms that various regulatory strategies can bring about significant changes in the electronic structure, which is insufficient to provide in-depth guidance and reference for electrochemical performance optimization of manganese-based materials. Herein, by summarizing the contribution of almost all modification strategies to the significant changes in the electronic structure, this review discloses that electronic structure regulation can be used as a general means to optimize the intrinsic properties and proposes a top-down electrochemical performance optimization methodology, which provides comprehensive suggestions for the optimization of manganese-based material performance. Notably, the electronic structure regulation effects of different modification methods are thoroughly compared, and their applicability and economy are evaluated, which is expected to further accelerate the commercialization of manganese-based ZIBs.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据