期刊
ACS MACRO LETTERS
卷 5, 期 2, 页码 258-262出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsmacrolett.6b00004
关键词
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资金
- MRSEC program of the National Science Foundation [DMR 1121053]
- Dow Chemical Company through the Dow Materials Institute at UCSB
- NSF Graduate Research Fellowship
- Alexander von Humboldt Foundation
- PREM program of the National Science Foundation [DMR-1205194]
The development of an operationally simple, metal-free surface-initiated atom transfer radical polymerization (SI-ATRP) based on visible-light mediation is reported. The facile nature of this process enables the fabrication of well-defined polymer brushes from flat and curved surfaces using a benchtop setup that can be easily scaled to four-inch wafers. This circumvents the requirement of stringent air-free environments (i.e., glovebox), and mediation by visible light allows for spatial control on the micron scale, with complex three-dimensional patterns achieved in a single step. This robust approach leads to unprecedented access to brush architectures for nonexperts.
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