期刊
CATALYSIS SCIENCE & TECHNOLOGY
卷 6, 期 8, 页码 2560-2564出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cy02072g
关键词
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资金
- EPSRC [EP/K036548/1, EP/K014706/1]
- Royal Society
- European Union [604307]
- EPSRC [EP/K036548/2] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/K036548/1, EP/K036548/2, EP/K014706/1] Funding Source: researchfish
Mesopore incorporation into ZSM-5 enhances the dispersion of Pd nanoparticles throughout the hierarchical framework, significantly accelerating m-cresol conversion relative to a conventional microporous ZSM-5, and dramatically increasing selectivity towards the desired methylcyclohexane deoxygenated product. Increasing the acid site density further promotes m-cresol conversion and methylcyclohexane selectivity through efficient dehydration of the intermediate methylcyclohexanol.
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