期刊
ACS CATALYSIS
卷 6, 期 5, 页码 2965-2981出版社
AMER CHEMICAL SOC
DOI: 10.1021/acscatal.6b00428
关键词
methane activation; methane valorization; heterogeneous catalysis; reaction mechanism; radical rebound mechanism; C-H bond activation; alkane functionalization
资金
- Dutch Science Foundation (NWO) through VIDI personal grant MetMOFCat
- Netherlands Center for Multiscale Catalytic Energy Conversion (MCEC), an NWO Gravitation programme - Ministry of Education, Culture and Science of the government of the Netherlands
In this Perspective, we highlight the main challenges to be addressed in the development of heterogeneous catalysts for the direct functionalization of methane. Along with our personal view on current developments in this field, we outline the main mechanistic, engineering, and catalyst design issues that have hampered implementation of new technologies and highlight possible paths to overcome these problems.
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