期刊
SCIENCE OF THE TOTAL ENVIRONMENT
卷 551, 期 -, 页码 51-56出版社
ELSEVIER
DOI: 10.1016/j.scitotenv.2016.02.026
关键词
Black carbon; Aerosol mixing states; Lensing effect; Radiative absorption; China
资金
- Fundamental Research Funds of Shandong University [2014QY001]
- Young Scholars Program of Shandong University [2015WLJH37]
- National Natural Science Foundation of China [41375126]
- Taishan Scholar Grand [ts20120552]
- Scientific Research Foundation for Returned Overseas Chinese Scholars of State Education Ministry [11460005451302]
- Swedish research funding agency Formas [214-2009-970]
- Swedish research funding agency STEM [35450-2]
The radiative absorption enhancement of ambient black carbon (BC), by light-refractive coatings of atmospheric aerosols, constitutes a large uncertainty in estimates of climate forcing. The direct measurements of radiative absorption enhancement require the experimentally-removing the coating materials in ambient BC-containing aerosols, which remains a challenge. Here, the absorption enhancement of the BC core by non-absorbing aerosol coatings was quantified using a two-step removal of both inorganic and organic matter coatings of ambient aerosols. The mass absorption cross-section (MAC) of decoated/pure atmospheric BC aerosols of 4.4 +/- 0.8 m(2)g(-1) was enhanced to 9.6 +/- 1.8 m(2)g(-1) at 678-nm wavelength for ambiently-coated BC aerosols at a rural Northern China site. The enhancement of MAC (E-MAC) rises from 1.4 +/- 0.3 in fresh combustion emissions to similar to 3 for aged ambient China aerosols. The three-week high-intensity campaign observed an average E-MAC of 2.25 +/- 0.55, and sulfates were primary drivers of the enhanced BC absorption. (C) 2016 Elsevier B.V. All rights reserved.
作者
我是这篇论文的作者
点击您的名字以认领此论文并将其添加到您的个人资料中。
推荐
暂无数据