期刊
SCIENCE
卷 352, 期 6286, 页码 697-701出版社
AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/science.aad9521
关键词
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资金
- European Union Marie Curie Postdoctoral Fellowship
- European Research Council
- Engineering and Physical Sciences Research Council (EPSRC)
- Medical Research Council
- BBSRC [BB/L014181/1] Funding Source: UKRI
- EPSRC [EP/K03927X/1, EP/K035746/1] Funding Source: UKRI
- Biotechnology and Biological Sciences Research Council [BB/L014181/1] Funding Source: researchfish
- Engineering and Physical Sciences Research Council [EP/K035746/1, EP/K03927X/1, 1245296] Funding Source: researchfish
The preparation of colloidally stable, self-assembled materials with tailorable solid or hollow two-dimensional (2D) structures represents a major challenge. We describe the formation of uniform, monodisperse rectangular platelet micelles of controlled size by means of seeded-growth methods that involve the addition of blends of crystalline-coil block copolymers and the corresponding crystalline homopolymer to cylindrical micelle seeds. Sequential addition of different blends yields solid platelet block comicelles with concentric rectangular patches with distinct coronal chemistries. These complex nano-objects can be subject to spatially selective processing that allows their disassembly to form perforated platelets, such as well-defined hollow rectangular rings. The solid and hollow 2D micelles provide a tunable platform for further functionalization and potential for a variety of applications.
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