期刊
SCIENCE
卷 351, 期 6273, 页码 579-582出版社
AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/science.aad2212
关键词
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资金
- Air Force Office of Scientific Research award [FA9550-11-1-0275]
- Center for Bio-Inspired Energy Science (CBES), an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0000989-0002]
- Northwestern University
- NSF
- E. I. DuPont de Nemours Co.
- Dow Chemical Company
- state of Illinois
Unlike conventional inorganic materials, biological systems are exquisitely adapted to respond to their surroundings. Proteins and other biological molecules can process a complex set of chemical binding events as informational inputs and respond accordingly via a change in structure and function. We applied this principle to the design and synthesis of inorganic materials by preparing nanoparticles with reconfigurable surface ligands, where interparticle bonding can be programmed in response to specific chemical cues in a dynamic manner. As a result, a nascent set of transmutable nanoparticles can be driven to crystallize along multiple thermodynamic trajectories, resulting in rational control over the phase and time evolution of nanoparticle-based matter.
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