期刊
POLYMER
卷 82, 期 -, 页码 105-113出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.polymer.2015.11.045
关键词
Superhydrophobic; Tunable wettability; Controllable structures; Antifouling; Oil-water separation
资金
- National Young Top Talents Plan of China [2013042]
- National Science Foundation of China [51175066]
- FANEDD [201164]
- New Century Excellent Talents in University [NCET-12-0704]
- Provincial New Century Excellent Talent [1251-NCET-007]
- Science Foundation for Distinguished Young Scholars of Heilongjiang Province [JC201403]
Novel superhydrophobic electrospun poly(vinylidene fluoride) (PVDF) membranes with controllable structure and tunable wettability have been achieved through incorporating ZnO nanoparticles and ammonia treatment for PVDF and/or post-chemical treatment on polymer membrane. The maximum WCA (171 +/- 1.5 degrees) of the electrospun membrane can be achieved under the condition of adding 8 wt.% ZnO. The controllable micro/nano-structures grown on the electrospun fibers can be regulated by the nano-ZnO loading. The tunable wettability from hydrophobic to superhydrophobic or from superoleophilic to superamphiphobic can be realized through modifying PVDF membranes with aqueous ammonia solution and incorporating 1H,1H,2H,2H-perfluorodecyltriethoxysilane. Moreover, these superhydrophobic membranes also demonstrated excellent durability, anti-fouling property and oil-water separation ability after dozens of cycles. These promising PVDF nanocomposite membranes with controllable structure and tunable wettability have the potential values in large-scale application of filtration, oil-water separation and antifouling. (C) 2015 Elsevier Ltd. All rights reserved.
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