期刊
PLASMA PROCESSES AND POLYMERS
卷 14, 期 6, 页码 -出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/ppap.201600081
关键词
ammonia; dielectric barrier discharges (DBD); ferroelectric PZT pellets; nitrogen conversion; packed-bed reactor
资金
- Junta de Andalucia [P12-2265MO]
- MINECO-CSIC through the EU regional fund project RECUPERA
Plasma reactions offer an attractive alternative route for the synthesis of a variety of valuable chemical compounds. Here we investigate the parameters that determine the efficiency of ammonia synthesis in a ferroelectric packed bed dielectric barrier discharge (DBD) reactor. The effects of varying the operating frequency, the size of the ferroelectric pellets and the inter-electrode distance have been systematically studied. Under optimised conditions nitrogen conversions in excess of 7% were achieved, higher than those previously obtained using DBD reactors. These findings are discussed with respect to variations in the electrical characteristics of the reactor under operating conditions and in the light of emission spectra obtained as a function of reactant flow rates. These encouraging results signpost future developments that could very substantially improve the efficiency of ammonia synthesis by means of DBD technology.
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