4.8 Article

Induced Fission of 240Pu within a Real-Time Microscopic Framework

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PHYSICAL REVIEW LETTERS
卷 116, 期 12, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.116.122504

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资金

  1. U.S. Department of Energy (DOE) [DE-FG02-97ER41014]
  2. Polish National Science Center (NCN) [UMO-2013/08/A/ST3/00708, UMO-2012/07/B/ST2/03907]
  3. U.S. Department of Energy through an Early Career Award of the LANL/LDRD Program
  4. DOE Office of Science [DE-AC05-00OR22725]
  5. Office of Science of the U.S. Department of Energy [DE-AC02-05CH11231]

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We describe the fissioning dynamics of Pu-240 from a configuration in the proximity of the outer fission barrier to full scission and the formation of the fragments within an implementation of density functional theory extended to superfluid systems and real-time dynamics. The fission fragments emerge with properties similar to those determined experimentally, while the fission dynamics appears to be quite complex, with many excited shape and pairing modes. The evolution is found to be much slower than previously expected, and the ultimate role of the collective inertia is found to be negligible in this fully nonadiabatic treatment of nuclear dynamics, where all collective degrees of freedom (CDOF) are included (unlike adiabatic treatments with a small number of CDOF).

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