期刊
PHYSICAL CHEMISTRY CHEMICAL PHYSICS
卷 18, 期 36, 页码 24825-24829出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cp04525a
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资金
- EPSRC [EP/K006851/1, EP/K031511/1]
- EPSRC [EP/K031511/1, EP/K006851/1] Funding Source: UKRI
- Engineering and Physical Sciences Research Council [EP/K031511/1, EP/K006851/1] Funding Source: researchfish
Graphitic carbon nitride (g-C3N4) synthesised from a urea precursor is an excellent CO2 reduction photocatalyst using [Co(bpy)(n)](2+) as a co-catalyst. A five-fold increase in activity for the highly polymerised urea derived g-C3N4 is achieved compared to alternative precursors. Transient absorption, time-resolved and steady-state emission studies indicate that the enhanced activity is related to both an increased driving force for photoelectron transfer and a greater availability of photogenerated charges.
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