期刊
ORGANIC LETTERS
卷 18, 期 3, 页码 488-491出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b03533
关键词
-
资金
- National Natural Science Foundation of China [21462022]
A regio- and chemoselective oxidative cycloisomerization reaction of acyclic 1,5-diynols has been developed. The reaction proceeds under metal-free reaction conditions with high efficiency and broad functional group tolerance, which offers a general and straightforward access to benzo[b]fluorenones under metal-free conditions. The preliminary mechanistic studies revealed the possible involvement of a Meyer-Schuster rearrangement combined with an oxidative radical cyclization.
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