期刊
ORGANIC LETTERS
卷 18, 期 11, 页码 2548-2551出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b00819
关键词
-
资金
- 973 Project from the MOST of China [2013CB228102, 2015CB856600]
- NSFC [21431008]
Cross-coupling of polyfluoroarenes with aryl carbamates through the cleavage of both sp(2) C-O and C-H bonds is reported, The reaction conditions are simple, and only transition-metal catalysts and ligands are essential. Mechanistic studies indicated that Ni catalyst played an important role in activating C-O bond, while the Cu one in activating C-H Bond. The developed system proved to be effective for cross-coupling of terminal alkynes with aryl carbamates.
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