期刊
ORGANIC LETTERS
卷 18, 期 24, 页码 6416-6419出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b03314
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-
资金
- CSIR [02/(0155)/13/EMR-II]
- CSIR, India
A novel Ru-catalyzed oxidative double annulation of heteroarenes with symmetrical and unsymmetrical alkynes is reported. A general method for the unsymmetrical annulation of heteroarenes with two distinct alkynes is showcased for the first time. Methylphenyl sulfoximine (MPS) plays an important role in the annulations of heteroarenes and allows the construction of structurally complex pi-conjugated heteroarene-fused polycyclic amide skeletons via the formation of multiple C-C and C-N bonds in a single operation. The reaction exhibits excellent substrate scope and tolerates a wide range of functional groups.
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