期刊
ORGANIC LETTERS
卷 18, 期 3, 页码 436-439出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.5b03476
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资金
- Spanish Ministry for Economy and Competitiveness [CTQ2011-25027, CTQ2013-50105-EXP]
- Spanish Ministry for Economy and Competitiveness (Severo Ochoa Excellence Accreditation) [SEV-2013-0319]
- ICIQ Summer Fellow Programme
- Cellex-ICIQ Program
- ICREA Funding Source: Custom
Conditions for an attractive and productive protocol for the position-selective intramolecular C-H amination of aliphatic groups (Hofmann-Loftier reaction) are reported employing sulfonimides as nitrogen sources. N-Iodosuccinimide is the only required promoter for this transformation, which is conveniently initiated by visible light. The overall transformation provides pyrrolidines under mild and selective conditions as demonstrated for 17 different substrates.
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