期刊
ORGANIC LETTERS
卷 18, 期 20, 页码 5356-5359出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b02711
关键词
-
资金
- National Natural Science Foundation of China [21474048, 21372114, 21672099]
The reductive single electron transfer (SET) umpolung amination of aldehyde-derived hydrazones has been developed through visible-light-promoted photoredox catalysis. The ideal transformation of hydrazones into the corresponding hydrazonamide through selective carbon-hydrogen (C-H) bond functionalization represents one of the most step- and atom-economical methods. This SET umpolung strategy features mild conditions and a remarkably broad substrate scope, offering an entirely new substrate class to direct C-H amination.
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