期刊
ORGANIC LETTERS
卷 18, 期 13, 页码 3294-3297出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b01611
关键词
-
资金
- National Institutes of Health [F32-GM112454, R01-GM069559]
The development of. Rh(III)-catalyzed C-H conjugate addition/cyclization reactions that provide access to synthetically useful fused bi- and tricyclic nitrogen heterocycles is reported. A broad scope of C-H functionalization substrates and electrophilic olefin coupling partners is effective, and depending on the nature of the directing group, cyclic imide, amide, or heteroaromatic products are obtained. An efficient synthesis of a pyrrolophenanthridine alkaloid natural product, oxoassoanine, highlights the utility of this method.
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