期刊
ORGANIC LETTERS
卷 18, 期 13, 页码 3298-3301出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b01619
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资金
- Deutsche Forschungsgemeinschaft [ME 776/17-2]
Relay metathesis enabled an improved access from (S)-citronellal to the marine trisnorguaiane (-)-clavukerin A. This hydroazulene was applied as an advantageously functionalized building block for the asymmetric synthesis of the sesquiterpene lactone osmitopsin and the proposed structure of 4,5-epoxyosmitopsin using a chemo-, regio-, and diastereoselective diepoxide opening as the key step.
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