期刊
ORGANIC LETTERS
卷 18, 期 16, 页码 3940-3943出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.6b01575
关键词
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资金
- 973 Program [2012CB725302]
- National Natural Science Foundation of China [21390400, 21272180, 21302148]
- Research Fund for the Doctor-al Program of Higher Education of China [20120141130002]
- Ministry of Science and Technology of China [2012YQ120060]
A highly regio- and stereoselective oxysulfonylation of allenes was developed that provided direct access to 2-sulfonyl allylic alcohols in good yields. By means of dioxygen activation, selective difunctionlization of allenes could be successfully achieved under mild metal-free conditions. Preliminary mechanistic investigation disclosed that this transformation probably goes through a radical process.
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