期刊
ORGANIC & BIOMOLECULAR CHEMISTRY
卷 14, 期 29, 页码 7024-7027出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6ob01344a
关键词
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资金
- JSPS, Japan [25410054, 16K05783]
- Sumitomo Foundation [130325]
Skeletal reorganisation of benzofused spiro[3.3]heptanes has been achieved using rhodium(I) catalysts. The reaction of benzofused 2-(2-pyridylmethylene)spiro[3.3]heptanes proceeds via sequential C-C bond oxidative addition and beta-carbon elimination. On the other hand, benzofused spiro[3.3]heptan-2-ols undergo two consecutive beta-carbon elimination processes. In both cases, substituted naphthalenes are obtained.
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