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Article
Chemistry, Multidisciplinary
Jun Pan et al.
Summary: A solvated double-layer quasi-solid polymer electrolyte (SDL-QSPE) is designed to improve stability and Na+ conductivity in polymer-based sodium-ion batteries. The SDL-QSPE, laminated with cathode- and anode-facing polymer electrolyte, exhibits enhanced cycle performance and high Coulombic efficiency. The interfacial evolution is analyzed through theoretical calculations and 3D X-ray microtomography.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2023)
Article
Chemistry, Multidisciplinary
Xianming Xia et al.
Summary: The authors developed an artificial heterogeneous interphase (Na@Na2Se/V) on the surface of sodium metal, which exhibits excellent ionic conductivity and mechanical properties. This interphase layer promotes homogeneous sodium deposition without dendrite formation, resulting in outstanding cycling life and electrochemical performance in carbonate-based electrolyte.
ADVANCED MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Xuyang Liu et al.
Summary: The FEIE electrolyte provides intrinsic safety and eliminates fire hazards for SMBs, while significantly improving sodium deposition and cycling stability. Usage of functional molecules with amphiphilicity extends the possibility of applying immiscible agents in battery electrolytes.
ADVANCED FUNCTIONAL MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Yixian Wang et al.
Summary: A new intermetallic compound NST-Na, fabricated through repeated cold rolling and folding, demonstrates outstanding electrochemical performance and stability. The thermodynamically stable face-centered-cubic structure of NST-Na allows for high efficiency in commonly used electrolytes, contributing to improved energy storage efficiency in sodium-metal batteries.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Yu Jiang et al.
Summary: Metallic Na (K) is a promising anode material for Na-metal and K-metal batteries, but the growth of Na (K) dendrites affects their stability. This study introduces a heterogeneous interface layer to improve the performance of the batteries, resulting in enhanced lifespan, capacity, energy density, and power density.
ADVANCED MATERIALS
(2022)
Review
Chemistry, Multidisciplinary
Tian Wang et al.
Summary: This review focuses on supporting the stability of working Na metal anodes through artificial interface engineering, emphasizing the importance of interface engineering in SMBs. Recent research on enhancing the interface between Na metal and electrolytes using an artificial interface layer is summarized, and prospects for interphase chemistry for Na metal anodes are provided.
Article
Chemistry, Multidisciplinary
Qianzheng Jin et al.
Summary: A novel metallic sodium/sodium-tin alloy foil anode (Na/NaSn) with 3D interpenetrated network and porous structure is prepared, which allows for uniform sodium deposition at high areal capacity and exhibits excellent electrochemical performance.
Article
Chemistry, Physical
Mengyang Xu et al.
Summary: A strategy of in situ forming a protective layer to suppress dendrite growth on sodium metal has been developed, leading to enhanced cyclic stability of sodium metal batteries. The design of a NaF-rich solid electrolyte interface prevents continuous electrolyte depletion during charge/discharge cycles and contributes to the high performance of the batteries.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Qifei Li et al.
Summary: Zinc-ion batteries, especially quasi-solid-state ZIBs, are important in energy storage devices due to abundant zinc reserve, low cost, high safety, and high theoretical capacity. This study presents a microwave-assisted hydrothermal method to prepare pre-potassiated hydrated vanadium pentoxide (KHVO) cathode material, which exhibits high electrochemical properties and superior zinc storage performance.
CHINESE CHEMICAL LETTERS
(2022)
Article
Chemistry, Physical
Zheng Luo et al.
Summary: Metallic sodium with high specific capacity is a promising material for electrical energy storage. However, the uncontrollable growth of dendrites hampers its practical application. In this study, an artificial interlayer composed of NaBr/Na3P nanocrystallines is constructed to control the Na diffusion behavior and suppress dendrite growth. The interlayer eliminates diffusion barriers and ensures fast Na+ transport, leading to a dendrite-free sodium anode with improved stability and performance.
Article
Chemistry, Multidisciplinary
Dongjun Li et al.
Summary: An artificial solid electrolyte interphase (SEI) layer consisting of an alloy and a solid electrolyte is constructed on the surface of sodium/potassium anode through an in situ reaction, leading to uniform deposition and improved cycle life and safety of the battery. This method combines the properties of high ionic conductivity, electronic insulation, and interfacial stability, providing important insights into the design principles of stable SEI layers for high-energy-density metal batteries.
Article
Multidisciplinary Sciences
Chuanlong Wang et al.
Summary: This study proposes a specific electrolyte formulation for low-temperature operation of non-aqueous sodium-based batteries, which exhibits thermal stability and enables a stable electrode|electrolyte interface at extremely low temperatures. Through a series of experiments and calculations, the mechanisms behind the efficient electrochemical performance at low temperatures are revealed.
NATURE COMMUNICATIONS
(2022)
Article
Electrochemistry
Jia-Lin Yang et al.
Summary: The research aims to convert spent anode graphite into cathode material for dual-ion batteries through a two-step treatment, achieving comparable performance to commercial graphite with high reversible capacity and improved cycling performance, demonstrating significant environmental and economic benefits.
Review
Chemistry, Physical
Huaming Yu et al.
Summary: Aqueous zinc-ion batteries (ZIBs) have gained attention as promising candidates for aqueous metal batteries due to their superior safety, low cost, and environmentally friendly characteristics. However, the role of water in the batteries is a double-edged sword, as it can boost the diffusion kinetics of zinc ions but also lead to hydrogen evolution reactions, dendrites growth, and surface passivation at the unstable interface.
Article
Chemistry, Physical
Xianming Xia et al.
Summary: This study designs a high-performance sodium anode by introducing an artificial VN interlayer on the sodium metal surface to regulate sodium nucleation and deposition behaviors, achieving uniform sodium deposition and extended cycling lifespan.
NANOSCALE HORIZONS
(2022)
Article
Electrochemistry
Ai-Long Chen et al.
Summary: A novel Li+ flux distributor achieved by placing PVDF/PMMA composite nanofiber interlayer on a current collector induces uniform lithium deposition to mitigate dendrite growth, improving the stability of lithium metal batteries. Experimental results show that the design enables molecular-level uniform Li nucleation, leading to high cycling stability and increased rate capacity.
Article
Chemistry, Multidisciplinary
Shuo Zhao et al.
Summary: A novel bifunctional cation additive TBA(+) is introduced in this study to enhance the cycling stability and Coulombic efficiency of aprotic Na-O-2 batteries. Experimental results show that the addition of TBA(+) improves the rate capability of the batteries.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Multidisciplinary
Xianghua Zhang et al.
Summary: Mesoporous carbon nanosheet-assembled flowers exhibit high potassium storage capacity, excellent rate performance, and superior long cycle capability, mainly due to their large surface area and reasonable pore volume.
CHINESE CHEMICAL LETTERS
(2021)
Article
Chemistry, Multidisciplinary
Hai Yang et al.
Summary: The study demonstrates that Na2Te/K2Te can improve Na+/K+ transport and suppress dendrite formation, offering a promising way to stabilize sodium (potassium)-metal anodes.
ADVANCED MATERIALS
(2021)
Article
Engineering, Environmental
Tiefeng Liu et al.
Summary: Recent research has focused on the interphase engineering chemistries of sodium metal anodes in batteries, highlighting advancements in addressing issues such as undesired dendrite growth and unstable solid electrolyte interphase. Understanding the critical role of a healthy SEI formed on the surface of sodium metal and implementing strategies to construct stable interphases can enhance the electrochemical stability of the anode.
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Chemistry, Multidisciplinary
Xiangsi Liu et al.
Summary: The recent applications of solid-state nuclear magnetic resonance (ssNMR) and magnetic resonance imaging (MRI) techniques in Li/Na batteries are reviewed, emphasizing the importance of investigating battery materials structure, solid electrolyte interfaces, and in situ research.
ADVANCED MATERIALS
(2021)
Review
Chemistry, Physical
Muhammad Kashif Aslam et al.
Summary: With the increasing diversity of electronic/electric appliances and large-scale energy storage systems, there is a growing demand for high-energy-density based device technology. However, metal batteries face challenges such as high anode reactivity, dendritic growth, and safety risks, with dendrite growth being a particularly severe issue.
Article
Physics, Applied
Hongcai Gao et al.
Summary: This study demonstrates an all-solid-state lithium battery based on a polymer-in-salt electrolyte, which features a wide electrochemically stable window, high ionic conductivity, increased lithium-ion transference number, and suppressed dendrite growth from the lithium-metal anode. Additionally, a stable interphase formed between the lithium-metal anode and the polymer-in-salt electrolyte can restrain uncontrolled parasitic reactions.
ENERGY MATERIAL ADVANCES
(2021)
Review
Nanoscience & Nanotechnology
Ying Wu et al.
Summary: This review systematically explores the rational design strategies for integrating porous carbon matrix with adsorption-catalysis agents in room-temperature sodium-sulfur batteries, as well as summarizes the multistep reaction mechanism and future prospects for the development of these batteries.
Review
Electrochemistry
Yan-Fang Zhu et al.
Summary: This review highlights recent advances in spinel engineering on layered oxide cathodes for enhancing Na+ transport kinetics and providing structural stability to achieve high-performance SIBs.
Article
Chemistry, Physical
Pan Xu et al.
Summary: Phosphorizing treatment was used to create a sodiophilic phosphorized copper mesh as a current collector for metallic sodium hosting, resulting in improved electrodeposition efficiency and behavior for sodium plating/stripping.
JOURNAL OF MATERIALS CHEMISTRY A
(2021)
Review
Chemistry, Multidisciplinary
Qifei Li et al.
Summary: This review comprehensively analyzes the recent development of metal phosphides (MPs) as anode materials for sodium-ion batteries (SIBs), including synthesis methods, advanced modification strategies, electrochemical performance, and sodium storage mechanism. Several research emphases for overcoming challenges and promoting the commercial application of emerging MPs anodes for SIBs are also pointed out.
Review
Nanoscience & Nanotechnology
Yue Gong et al.
Summary: MXenes are a rapidly growing family of 2D materials, and their composition, morphology, structure, surface chemistry, and structural configuration directly affect their electrochemical performance, significantly impacting the storage performance of devices like transistors. The work function and bandgap of MXenes can be controlled by tailoring their structure and surface functional groups, making them important in various storage applications. Researchers are striving to develop novel MXenes and improve their applications, with the aim of enhancing their effectiveness in high-density data storage applications.
Article
Chemistry, Multidisciplinary
Xueying Zheng et al.
Summary: This study demonstrates the development of a high-voltage Na/Na3V2(PO4)(2)O2F battery that can withstand temperatures as low as -30 degrees Celsius and fast charging up to 30C. By utilizing a weakly solvated electrolyte and a biphasic artificial SEI, the researchers have successfully achieved low-temperature and fast-charging performances for sodium metal batteries. The design strategy highlights the importance of de-solvation and SEI control in overcoming kinetic barriers under extreme conditions.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
Review
Chemistry, Multidisciplinary
Min Fan et al.
Summary: The article summarizes the recent progress of recycling spent LIBs, especially focusing on green innovations. The sustainability of the recycling process has become an important factor in the field.
Article
Chemistry, Multidisciplinary
Xin-Bing Cheng et al.
Summary: Lithium-ion batteries have been successful in portable electronics and electric vehicles, but face challenges in terms of sustainable development, requiring innovation in material chemistry and safety performance, as well as the importance of battery recycling for a sustainable society.
Article
Chemistry, Multidisciplinary
Bing Sun et al.
ADVANCED MATERIALS
(2020)
Article
Chemistry, Multidisciplinary
Phung M. L. Le et al.
ADVANCED FUNCTIONAL MATERIALS
(2020)
Article
Chemistry, Physical
Xueying Zheng et al.
Article
Chemistry, Physical
Vipin Kumar et al.
ENERGY STORAGE MATERIALS
(2020)
Article
Chemistry, Physical
Shiyang Wang et al.
Article
Chemistry, Physical
Xueying Zheng et al.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2019)
Article
Chemistry, Physical
Huajun Tian et al.
Article
Chemistry, Physical
Yang Zhao et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2019)
Article
Chemistry, Multidisciplinary
Shiyang Wang et al.
CHEMICAL COMMUNICATIONS
(2019)
Article
Multidisciplinary Sciences
Yu Gu et al.
NATURE COMMUNICATIONS
(2018)
Article
Chemistry, Physical
Alexander Bauer et al.
ADVANCED ENERGY MATERIALS
(2018)
Article
Multidisciplinary Sciences
Snehashis Choudhury et al.
NATURE COMMUNICATIONS
(2017)
Article
Chemistry, Physical
Lukas Lutz et al.
CHEMISTRY OF MATERIALS
(2017)
Article
Nanoscience & Nanotechnology
Juan Zhang et al.
ACS APPLIED MATERIALS & INTERFACES
(2015)
