期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 357, 期 6, 页码 1199-1203出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201400739
关键词
amides; N-heterocyclic carbenes; organic catalysis; oxidation; oxidative amidation
资金
- DST, SERB, New Delhi [SB/FT/CS-108/2012]
The N-heterocyclic carbene (NHC)-catalyzed oxidative amidation of aromatic aldehydes with amines in the presence of N-bromosuccinimide (NBS) as an oxidant has been developed for the synthesis of amides. This amidation strategy is tolerant to both the electronic and the steric nature of the aryl aldehydes employed. The present methodology was extended to chiral amino acid derivatives to generate the corresponding amides in good yields and excellent ee values (> 98%).
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