期刊
CHEMICAL SOCIETY REVIEWS
卷 44, 期 10, 页码 3023-3035出版社
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cs00094g
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资金
- National Natural Science Funds for Excellent Young Scholars [21222608]
- Research Fund of the National Natural Science Foundation of China [21106099]
- Foundation for the Author of National Excellent Doctoral Dissertation of China [201251]
- Program for New Century Excellent Talents in University [NCET-12-0392]
- Program of Introducing Talents of Discipline to Universities [B06006]
Scientific interest in graphene as a catalyst and as a catalyst support in heterogeneous catalytic reactions has grown dramatically over the past several years. The present critical review summarizes the multiple roles of graphene in heterogeneous catalysis and highlights the influence of defects, heteroatom-containing functionalities, and graphene's two-dimensional structure on catalytic performance. We first discuss the role and advantages of graphene as a catalyst support, with emphasis on its interactions with the catalytic phases and the influence of mass transfer processes. We then clarify the origin of the intrinsic catalytic activity of graphene in heterogeneous catalytic reactions. Finally we suggest challenges and potential practical applications for graphene in industrial processes.
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