期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 357, 期 14-15, 页码 3033-3039出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.201500417
关键词
alkynes; allenes; [2+2+2] cycloaddition; imines; rhodium
资金
- Japan Society for the Promotion of Science (JSPS) [2646000104]
- Molecular Activation Directed toward Straightforward Synthesis from Ministry of Education, Culture, Sports, Science and Technology, Japan [23105501]
- [26293001]
- Grants-in-Aid for Scientific Research [26460001, 26293001] Funding Source: KAKEN
The rhodium(I)-catalyzed intramolecular [2+2+2] cycloaddition between allenes, alkynes, and imines has been developed. This cyclization proceeds via a strained azarhodacycle, giving a 5,7-fused cyclic amide or a tricyclic product containing an 8-azabicyclo[3.2.1] octane skeleton in high yield.
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