4.6 Article

Turing Patterns in Forced Open Two-Side-Fed-Reactor

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ADVANCED THEORY AND SIMULATIONS
卷 6, 期 9, 页码 -

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WILEY-V C H VERLAG GMBH
DOI: 10.1002/adts.202300091

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nonlinear dynamics; pattern formation; reaction-diffusion

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The mechanism proposed by Turing for reaction-diffusion systems is widely used to explain pattern formation in various fields. The persistence of patterns in changing environments is crucial in many natural cases. Experimental studies of these phenomena can be carried out using specially designed chemical systems, such as two-side-fed open gel reactors. By testing the effect of time-periodic boundary conditions on the dynamics of Turing patterns, this configuration allows for a better understanding of pattern formation in altering environments. Numerical simulations based on realistic chemistry and a 2D reactor description can reproduce feeding from boundaries and concentration gradients, revealing two regimes, spatiotemporal oscillations and pulsating spot patterns, with the possibility of a mixed-mode pattern. The findings suggest that periodic feeding can effectively control pattern formation in chemical systems.
The mechanism suggested by Turing for reaction-diffusion systems is widely used to explain pattern formation in biology and in many other areas. The persistence of patterns in altering environments is an important property in many natural cases. The experimental study of these phenomena can be done in chemical systems using appropriately designed reactors, e.g., in two-side-fed open gel reactors. This configuration allows for testing the effect of time-periodic boundary conditions that generate periodic feeding of chemicals on the dynamics of Turing patterns. The numerical approach is based on a chemically realistic mechanism and a 2D description of the reactor that reproduces the feeding from the boundaries and the corresponding concentration gradients. Depending on the amplitude and the frequency of the forcing, two basic regimes are observed, spatiotemporal oscillations and pulsating spot pattern. In between them, a mixed-mode pattern can also develop. Spot patterns can survive large amplitude forcing. The dynamics of the spot pulsation are analyzed in detail, considering the effect of the tanks and the chemical gradients that localize the patterns. These findings suggest that periodic feeding effectively controls pattern formation in chemical systems.

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