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Article
Chemistry, Multidisciplinary
Jiahao Liu et al.
Summary: In this study, an acid-assisted confined self-assembly method (ACSA) was developed to prepare a two-dimensional mesoporous zincophilic sieve (2DZS) as the kinetic interface. The 2DZS interface effectively reduces the anodic polarization of sulfur-based aqueous zinc batteries (SZBs) at high current density, leading to improved lifespan and energy density.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2023)
Article
Chemistry, Multidisciplinary
Weiwei Zhang et al.
Summary: To fully utilize the potential of high energy Zn-S electrochemistry, the inefficiency and high reactivation energy barrier associated with sulfur cathodes in battery discharging and recharging need to be addressed. An experiment and theoretical prediction suggest that atomically dispersed Fe sites with Fe-N-4 coordination can serve as bidirectional electrocatalytic hotspots, enabling complete sulfur conversion and reducing the energy barrier of ZnS decomposition. The Fe sites facilitate sulfur and zinc polysulfide adsorption, leading to almost complete sulfur to ZnS conversion during discharge and reversible charging back to S during recharging.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Engineering, Environmental
Na Li et al.
Summary: This study demonstrates an in situ interfacial fabrication method of highly flexible MnO2@polyaniline core-shell nanowire film for high-rate and durable zinc energy storage. The hybrid cathode shows an impressive reversible capacity and improved rate and cycling performance, providing a new design approach for the development of flexible electronics.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Engineering, Environmental
Ge Chang et al.
Summary: A novel bifunctional electrolyte additive thiourea (TU) was introduced to improve the reaction kinetics and cycle stability of aqueous zinc-sulfur (Zn-S) battery. TU can undergo reversible redox reactions, enhancing the reversibility between ZnS and S and providing extra capacities. The mechanism of TU on the S@KB electrode was proposed, involving the interaction between TU intermediates and ZnS to weaken the Zn-S bonds and inhibit the formation of irreversible by-product. The S@KB electrode exhibited excellent cyclic performance with low decay rate of 0.11% per cycle after 300 cycles at 5 A/g.
CHEMICAL ENGINEERING JOURNAL
(2023)
Article
Electrochemistry
Yujin Kim et al.
Summary: This study investigated the impact of electrode loading levels on the electrochemical performance of lithium-ion batteries. The differences in performance were found to be related to varying internal resistances. The optimal loading level for commercial LiNi0.6-Co0.2Mn0.2O2 cathode materials was approximately 20 mg/cm2, which resulted in an areal capacity of 3.3 mAh/cm2.
ELECTROCHEMISTRY COMMUNICATIONS
(2023)
Article
Chemistry, Multidisciplinary
Hong Zhang et al.
Summary: In this study, a high-energy Zn-S system was designed with a high-capacity cathode and fast redox mediators, allowing for highly reversible conversion between sulfur and ZnS. The proposed redox electrocatalysis effect provides reliable insights into the tunable Zn-S chemistry, leading to improved performance in Zn-S cells.
Article
Chemistry, Physical
Junjie Shi et al.
Summary: The study introduces Ti3C2Tx MXenes with a two-dimensional (2D) layered structure and hydrophobic trifluoromethane sulfonate (OTf-) into AZIBs to address the low conductivity and poor stability issues of MoO3, resulting in exceptional high capacity and cycling life performance.
Article
Chemistry, Physical
Man Qi et al.
Summary: This study develops a high-performance flexible cathode for aqueous zinc-ion batteries. The cathode is prepared by electrodeposition and dipping methods, forming a three-dimensional interconnected structure of ultrathin MnO2 nanosheets on carbon cloth, coated with MXene for improved conductivity and active sites. The flexible cathode exhibits high charge storage performance, excellent cycling stability, and remarkable energy density, showing potential for application.
JOURNAL OF COLLOID AND INTERFACE SCIENCE
(2022)
Review
Chemistry, Multidisciplinary
Muhammad Sufyan Javed et al.
Summary: This review summarizes the advances in synthesis, properties, morphology, structure, and chemistry of MXenes for ZIBs. The recent developments in MXene-based electrodes and electrolytes are highlighted, along with strategies and challenges for enhancing the electrochemical performance of ZIBs. Future prospects for MXene-based ZIBs are also discussed.
Review
Chemistry, Multidisciplinary
Xinliang Li et al.
Summary: The diverse and tunable surface and bulk chemistry of MXenes have valuable and distinctive properties that can be utilized in various components of energy storage devices such as electrodes, electrolytes, and separators. They enhance stability and performance through ion storage, transfer regulation, steric hindrance, and electrocatalytic functions.
NATURE REVIEWS CHEMISTRY
(2022)
Article
Chemistry, Physical
Tiansheng Zhou et al.
Summary: In this study, a regulation strategy for uniform ZnS nucleation was proposed by introducing PEG-400 additive into the zinc ion battery, which improved the uneven conversion of sulfur-based cathode materials to S during the charge process. The modified solvation structure formed by this electrolyte allowed the formation of uniform and small ZnS particles, leading to enhanced battery performance.
MATERIALS TODAY ENERGY
(2022)
Article
Chemistry, Physical
Fan Zhao et al.
Summary: This study demonstrates the synthesis of the a-V2O5@Ti3C2Tx heterostructure for enhanced performance in rechargeable aqueous zinc-ion batteries. The heterostructure exhibits isotropic ion diffusion paths, plentiful ion storage sites, and excellent conductivity, resulting in excellent specific capacity and rate performance.
JOURNAL OF POWER SOURCES
(2022)
Article
Chemistry, Physical
Dongdong Liu et al.
Summary: By using a carbon-sheathed ZnS cathode and introducing iodinated thiourea as a redox mediator, the activation barrier was effectively reduced, leading to a high-performance Zn-S battery.
Article
Chemistry, Multidisciplinary
Ahmad Amiri et al.
Summary: This article introduces a freeze-resistant and multifunctional quasi-solid-state zinc-sulfur battery with high energy density and superior mechanical properties, which can be used under different climate conditions. Sulfur is deposited on activated carbon nanofibers using an electrostatic spray coating technique to form a load-bearing cathode. The use of an antifreezing hydrogel electrolyte addresses the strain issues of the structural energy storage device in extreme climates. The electrochemomechanical properties of the battery are also studied.
Article
Chemistry, Multidisciplinary
Zhao Xu et al.
Summary: This communication systematically illustrates the electrolyte chemistry in aqueous Zn-S batteries. Compared to Zn(AC)(2) and ZnSO4, Zn(OTF)(2) electrolyte shows better electrochemical performance due to the impact of larger CF3SO3- anions on the solvation shell structure of Zn2+. Moreover, a reversible capacity of 788 mA h g(-1) is obtained in concentrated Zn(OTF)(2) electrolyte (3 M) with higher retention due to higher Zn-nucleation overpotential and slower corrosion reactions.
CHEMICAL COMMUNICATIONS
(2022)
Review
Green & Sustainable Science & Technology
Sungjemmenla et al.
Summary: The increased demand for energy has led to the search for alternative energy storage devices. Post-Li-ion battery chemistries, such as sulfur-based batteries, have the potential to meet the market's demands for high energy density and low cost. However, the complex reaction chemistry of sulfur cathode and the increasing complexity with higher valency metal ions pose challenges to the development of sulfur cathode-based high-energy rechargeable batteries. This review provides a summary of the unique aspects of sulfur cathode and insights into the electrochemical performance of various metal-sulfur-based systems, aiming to accelerate the development of sulfur cathode for post-Li-ion batteries.
ADVANCED ENERGY AND SUSTAINABILITY RESEARCH
(2022)
Article
Nanoscience & Nanotechnology
Mangwei Cui et al.
Summary: This study addresses the limited specific capacity and Zn dendrites issues in traditional aqueous Zn-ion batteries by utilizing a conversion-type Zn-S battery and low-cost deep eutectic solvent (DES). The optimized electrolyte enables the symmetrical Zn battery to cycle stably for over 3920 hours, achieving an ultrahigh specific capacity of approximately 846 mA h g(S)(-1) and energy density of 259 W h kg(-1) at 0.5 A g(-1). The conversion chemistry of S and ZnS contributes to superior anti-self-discharge behavior, solving long-standing problems in conventional Zn-ion batteries.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Multidisciplinary
Xiaodong Zhu et al.
Summary: The manganese-vanadium hybrid K-V2C@MnO2 cathode, designed with MnO2 nanosheets uniformly formed on a V2CTX MXene surface, shows excellent electrochemical performance for aqueous ZIBs due to high conductivity, abundant active sites, and the synergistic reaction. It achieves a high specific capacity of 408.1 mAh g(-1) at 0.3 A g(-1) and maintains 119.2 mAh g(-1) at a high current density of 10 A g(-1) over 10000 cycles, outperforming almost all reported Mn-based cathodes in aqueous ZIBs.
Article
Chemistry, Multidisciplinary
Mian Li et al.
Summary: Experimental exploration of various halogen terminals on the surface of Ti3C2 MXenes showed that the presence of Br and I elements resulted in improved electrochemical performance for aqueous zinc ion batteries. The Lewis-acidic-melt etching route proved to be effective in tuning the surface chemistry of MXenes for expanding their potential applications.
Article
Chemistry, Multidisciplinary
Xinliang Li et al.
Summary: The study introduced a Nb2CTX host and achieved electro-oxidation of I- ions in MXene through electrodeposition strategy, thereby improving redox kinetics and duration. The aqueous Zn battery based on a Zn metal anode and ZnSO4 electrolyte showed outstanding performance, surpassing other aqueous MXenes and I-2-metal batteries.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Physical
Chunlong Dai et al.
Summary: High theoretical specific capacity zinc and sulfur are selected as the anode and cathode, with a strategy proposed to decouple charge carriers in anolyte and catholyte to simultaneously enhance the energy storage performance of flexible aqueous batteries. The new zinc-sulfur hybrid battery boasts ultrahigh theoretical specific capacity and volumetric energy density.
ADVANCED ENERGY MATERIALS
(2021)
Article
Nanoscience & Nanotechnology
Hiren K. Machhi et al.
Summary: The rechargeable aqueous zinc-iodine batteries (AZIBs) with a multipurpose sponge-like porous matrix of a metal-organic gel show superior electrochemical performance due to limited iodine diffusion, leading to high capacity retention and long-term stability even after 1500 cycles. Prototype flexible band-aid-type AZIBs also demonstrate promising performance in real-scale wearable applications.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Multidisciplinary
Ying Liu et al.
Summary: The research focuses on enhancing the performance of PANI cathode material in Zn-ion batteries using surface-engineered Ti3C2Tx MXene, which provides protons and maintains a low pH to suppress the instability of PANI, and improves performance through fast redox reactions and buffering of swelling/shrinking.
Review
Chemistry, Multidisciplinary
Haobo Dong et al.
Summary: The latest progress in polymer electrolytes for flexible ZIBs, particularly hydrogel electrolytes, is summarized in the article, along with discussions on relevant challenges, device configurations, and life cycle analysis. It is noted that most current polymer electrolytes emphasize electrochemical performance, with little consideration for mechanical behavior and interactions with electrode materials. Strategies to combine softness and strength, as well as the introduction of a ranking index to evaluate both electrochemical and mechanical properties, are discussed.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Chunlong Dai et al.
Summary: The cascade battery proposed in this study couples two sequential electrochemical reactions in a single battery, showing many advantages compared to traditional batteries. It integrates two batteries internally, eliminating the need for additional inactive connecting materials, can more fully utilize the inactive reaction chamber, and achieve a higher areal capacity even at low solid cathode loading.
ADVANCED MATERIALS
(2021)
Review
Chemistry, Multidisciplinary
Jiahao Liu et al.
Summary: This article focuses on constructing a theory-to-application methodology for aqueous sulfur-based batteries. Research reveals the complexity in the electrochemistry of aqueous sulfur-based batteries, which poses challenges and potential for future development. Further exploration in both theory and practice is needed for the future development direction.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2021)
Article
Chemistry, Multidisciplinary
Lian-Wei Luo et al.
Summary: This disposable aqueous primary battery chemistry utilizes environmentally benign sulfur cathode and Zn anode, showcasing high energy density and areal capacity under high mass loading conditions.
CHEMICAL COMMUNICATIONS
(2021)
Article
Chemistry, Multidisciplinary
Rahul Pai et al.
Summary: A facile strategy was presented to improve the electrochemical performance of lithium-sulfur batteries through surface functionalization between sulfur and Ti3C2Tz-MXene, resulting in higher sulfur loadings. The developed composite showed increased active area and effective trapping of lithium polysulfides, leading to enhanced cycle life and Coulombic efficiency. Ex situ studies revealed the nature of the LiPs-MXene interaction and the impact of surface functionalization on improved performance.
CELL REPORTS PHYSICAL SCIENCE
(2021)
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Yuwei Zhao et al.
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(2020)
Review
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Xinliang Li et al.
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(2020)
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Wei Li et al.
Review
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Tengsheng Zhang et al.
ENERGY & ENVIRONMENTAL SCIENCE
(2020)
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Keval K. Sonigara et al.
ADVANCED ENERGY MATERIALS
(2020)
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(2020)
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Minjie Shi et al.
CHEMICAL ENGINEERING JOURNAL
(2020)
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Jin Zhao et al.
Article
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Carmen C. Mayorga-Martinez et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2019)
Article
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Weizhai Bao et al.
ADVANCED ENERGY MATERIALS
(2018)
Article
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Yue Ma et al.
ACS SUSTAINABLE CHEMISTRY & ENGINEERING
(2018)
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Keval K. Sonigara et al.
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Qi Han et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2018)
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Jingwen Zhao et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2017)
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Meng Wang et al.
CHEMISTRY CENTRAL JOURNAL
(2011)