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Article
Chemistry, Physical
Gang Ni et al.
Summary: In this study, hybrid Zn/K batteries with Berlin green (FeHCF) cathode and aqueous KCF3SO3/Zn(CF3SO3)2 electrolyte were fabricated using fire-retardant triethyl phosphate (TEP) as a co-solvent. The addition of TEP suppresses water decomposition, increases the Coulombic efficiency, and prevents Zn displacement of FeHCF while inhibiting its surface reduction and decomposition by reducing water activity. Moreover, TEP suppresses dendrite growth and parasitic reactions on the Zn anode. These positive effects significantly improve the cycle performance of hybrid batteries.
MATERIALS TODAY ENERGY
(2023)
Article
Green & Sustainable Science & Technology
Junmin Ge et al.
Summary: Aqueous potassium-ion batteries have emerged as a more sustainable technology to complement lithium-ion counterparts. Ge et al. engineer the surface of a potassium manganese hexacyanoferrate cathode material, achieving unprecedented electrochemical performance in full K-ion cells.
NATURE SUSTAINABILITY
(2022)
Article
Chemistry, Multidisciplinary
Fangwang Ming et al.
Summary: This work proposes a hybrid electrolyte induced by the salting-in effect as an effective strategy to achieve a highly reversible zinc anode with good stability and compatibility. By altering the solvation structure and reducing parasitic side reactions, this electrolyte ensures a stable zinc anode with excellent cycling stability.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2022)
Article
Chemistry, Physical
Yunpo Sun et al.
Summary: This work proposes a cost-effective water/ethanol hybrid electrolyte that solves the issues of zinc corrosion and dendrite growth in zinc-ion batteries, resulting in high capacity, superior rate capability, and extremely stable cycling performance.
ENERGY STORAGE MATERIALS
(2022)
Article
Materials Science, Multidisciplinary
Xin-Fei Wu et al.
Summary: This work presents a facile carbonization method to prepare sulfur-doped amorphous carbon microspheres (S-CM-700) with hierarchical structure and modulated defects concentration for potassium storage. The S-CM-700 exhibits optimal performance, including high reversible capacity, excellent rate property, and remarkable durability. The study also reveals that the potassium storage can be enhanced by regulating the defect level, layer spacing, and the content of sulfur-doping.
Article
Chemistry, Multidisciplinary
Qiu Zhang et al.
Summary: By introducing halogen ions, the challenges of dendritic growth and hydrogen evolution reaction in zinc metal batteries can be overcome. Designing an electrolyte composed of zinc acetate and ammonium halide can form a halogenated Zn2+ solvation structure, achieving high coulombic efficiency and suppressing dendritic growth.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2022)
Review
Electrochemistry
Shen Qiu et al.
Summary: This review introduces the recent progress of Prussian blue analogues for aqueous monovalent ion batteries, including metal ions of Li+, Na+, K+, and non-metal ions of H+ and NH4+.
ELECTROCHEMICAL ENERGY REVIEWS
(2022)
Review
Chemistry, Multidisciplinary
Haocong Yi et al.
Summary: This review discusses the structure/property correlations and optimization strategies of Prussian blue analogue (PBA) materials as host frameworks for various charge-carrier ions in energy storage/conversion applications. The prospects for further applications of PBA materials in different types of batteries are summarized, with extra attention given to the selection of anode materials and electrolytes for practical implementation. This work aims to provide a comprehensive understanding of PBA materials and to guide future research and development of PBA electrodes.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Multidisciplinary Sciences
Wei Sun et al.
Summary: The study presents a zinc-O-2/zinc peroxide chemistry that operates through a 2e(-)/O-2 process in nonalkaline aqueous electrolytes, allowing highly reversible redox reactions in zinc-air batteries. This innovative ZnO2 chemistry, enabled by water-poor and zinc ion (Zn2+)-rich inner Helmholtz layer, shows superior reversibility and stability compared to alkaline zinc-air batteries.
Review
Chemistry, Multidisciplinary
Jianping Yan et al.
Summary: This review discusses the design strategies and challenges of high-voltage rechargeable zinc-ion batteries (ZIBs), introduces recent advances in high-voltage cathode materials, and explores strategies to increase cathode operating voltage and factors influencing voltage in redox reactions.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Engineering, Environmental
Yuming Xi et al.
Summary: In this study, a bottom-up method for the rapid and efficient preparation of NaxMn[Fe(CN)(6)](y) with low defect and high sodium content was proposed by combining homogeneous rapid precipitation in a microreactor and subsequent thermal aging treatment. The key to successful bottom-up synthesis was enhancing the aggregation-mediated growth of building blocks, which decouples nucleation and growth under high supersaturation to obtain uniform building blocks. The as-prepared MnHCF exhibited high capacity, excellent rate performance, and satisfactory cyclic retention due to its high crystallinity, with a capacity retention of 76% for 100 cycles at a current density of 150 mAg(-1).
CHEMICAL ENGINEERING JOURNAL
(2021)
Article
Chemistry, Physical
Qian Li et al.
Summary: A unique dual-ion battery based on zinc hexacyanoferrate cathode and zinc metal anode was developed, showing outstanding rate performance and cycling life.
ENERGY STORAGE MATERIALS
(2021)
Article
Nanoscience & Nanotechnology
Tong Cao et al.
Summary: Research focuses on obtaining less water and low defect KMHCF material as the cathode of A-ZIBs by controlling the synthesis process, showing excellent cycling stability and discharge capacity. The study also found that the KMHCF electrode undergoes a phase transition process when activated by a small current density, forming a new stable phase to participate in subsequent electrochemical reactions.
ACS APPLIED MATERIALS & INTERFACES
(2021)
Article
Chemistry, Physical
Wenjun Deng et al.
Summary: This study reports a K2MnFe(CN)6 cathode achieving a very stable capacity in a ZIB, attributed to its gradual transformation to a more stable K2Zn3[Fe(CN)6](2) phase induced by Zn2+ insertion. The mechanism involves lattice distortion and formation of wider channels for highly stable storage and release of zinc ions, providing new insights into the evolution of PBAs in ZIBs.
ADVANCED ENERGY MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Yinxiang Zeng et al.
Summary: A template-engaged ion exchange approach was developed for synthesizing Co-substituted Mn-rich PBA hollow spheres, which showed efficient zinc ion storage properties with high capacity, decent rate capability, and prolonged cycle life.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Multidisciplinary
Yun Tang et al.
ADVANCED FUNCTIONAL MATERIALS
(2020)
Review
Chemistry, Physical
Shude Liu et al.
ADVANCED ENERGY MATERIALS
(2020)
Article
Chemistry, Physical
Meng Huang et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2020)
Review
Chemistry, Physical
Lauren E. Blanc et al.
Review
Chemistry, Physical
Hongfei Li et al.
Article
Energy & Fuels
Liwei Jiang et al.
Review
Chemistry, Physical
Jianhang Huang et al.
Review
Chemistry, Multidisciplinary
Lidan Xing et al.
ACCOUNTS OF CHEMICAL RESEARCH
(2018)
Review
Chemistry, Multidisciplinary
Ming Song et al.
ADVANCED FUNCTIONAL MATERIALS
(2018)
Article
Chemistry, Multidisciplinary
Qiang Zhang et al.
Article
Chemistry, Physical
Ke Lu et al.
JOURNAL OF POWER SOURCES
(2016)
Article
Chemistry, Physical
Niccolo Peruzzi et al.
JOURNAL OF SOLUTION CHEMISTRY
(2015)
Article
Chemistry, Physical
Leyuan Zhang et al.
ADVANCED ENERGY MATERIALS
(2015)