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Article
Chemistry, Physical
Ping Xiao et al.
Summary: By utilizing γ-butyrolactone (GBL) as an organic solvent, the deposition behavior and performance of Zn anodes can be regulated, allowing for improved electrochemical performance under high current densities and large areal capacities due to reduced dendrite growth and enhanced reaction reversibility. The strong interactions between GBL molecules and Zn2+ and Zn slab were confirmed by DFT calculations, and the preferential adsorption of GBL at the Zn/electrolyte interface was highlighted through Raman spectra analysis. Electrochemical tests demonstrated the effectiveness of this strategy, achieving a supporting current density of 30 mA cm(-1) and a cycle life of 5000 h for the Zn anode using GBL.
ACS ENERGY LETTERS
(2023)
Article
Chemistry, Physical
Shengda D. Pu et al.
Summary: Rechargeable aqueous zinc batteries offer low cost, safety, and good cycling capacity, largely due to the water-compatible Zn-metal anode. However, Zn anodes corrode in aqueous electrolytes. This study successfully decouples and quantifies the aging-induced contributions toward anode degradation in mildly acidic aqueous electrolytes, demonstrating that the physical screening effect of evolved gases is the bigger contributor to the efficiency loss of these batteries.
Review
Electrochemistry
Zixuan Li et al.
Summary: Rechargeable aqueous zinc-ion batteries are promising candidates for next-generation energy storage due to their high theoretical capacity, low cost, safety, and environmental friendliness. However, the physical and chemical instability of the zinc anode hinders the electrochemical performance. Regulating the electrolyte can improve the performance of the zinc anode, making it important to gain an in-depth understanding of the electrolyte-dependent regulation mechanisms.
Article
Multidisciplinary Sciences
Yujing Liu et al.
Summary: In this study, self-assembled monolayers (SAMs) were utilized to control electrolyte degradation and solid-electrolyte interphase (SEI) formation in lithium metal batteries (LMBs), resulting in improved cycling performance and lifespan.
Review
Chemistry, Multidisciplinary
Yanyan Wang et al.
Summary: This review provides an overview of advanced electrolyte strategies for optimizing zinc-ion batteries, including improving the compatibility between cathode materials and electrolytes, inhibiting anode corrosion and dendrite growth, extending electrochemical stability windows, enabling wearable applications, and enhancing temperature tolerance. The underlying scientific mechanisms, electrolyte design principles, and recent progress are presented to enhance understanding and inspiration for readers.
Article
Chemistry, Physical
Tian Chen Li et al.
Summary: Adding carbonyl-containing organic solvents can enhance the reversibility of zinc-ion batteries and improve their cycling stability and capacity retention.
ADVANCED ENERGY MATERIALS
(2022)
Article
Chemistry, Physical
Hao Zhang et al.
Summary: The practical application of aqueous Zn-ion batteries has been hindered by poor reversibility of Zn anode due to dendritic growth and interfacial parasitic reaction. A novel stable Zn anode was successfully designed by incorporating hydrophilic graphene quantum dots (GQDs), leading to improved performance and extended lifespan of Zn-ion batteries.
Article
Green & Sustainable Science & Technology
Daliang Han et al.
Summary: Aqueous zinc batteries are safer than lithium-ion batteries, but their anodes are susceptible to dendrite failure and side reactions. The authors demonstrate a low-cost electrolyte that involves hydrate salt and organic solvent, proving to be non-flammable. The zinc battery cell delivers excellent performance even at low temperatures of -30 degrees Celsius.
NATURE SUSTAINABILITY
(2022)
Article
Chemistry, Multidisciplinary
Yinxiang Zeng et al.
Summary: The study developed a 3D multifunctional host consisting of N-doped carbon fibers embedded with Cu nanoboxes for stable Zn-metal anodes. The host's structure alleviates volume change during cycling and enables uniform and dense Zn deposition, resulting in high Coulombic efficiency and long cycling life for the electrode.
ADVANCED MATERIALS
(2022)
Article
Chemistry, Multidisciplinary
Fangwang Ming et al.
Summary: This work proposes a hybrid electrolyte induced by the salting-in effect as an effective strategy to achieve a highly reversible zinc anode with good stability and compatibility. By altering the solvation structure and reducing parasitic side reactions, this electrolyte ensures a stable zinc anode with excellent cycling stability.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2022)
Article
Multidisciplinary Sciences
Huan Yu et al.
Summary: We developed a three-dimensional hybrid fiber host for high-performance Zn metal batteries, which enables homogeneous Zn deposition on the interior and exterior surfaces of the hollow fibers.
Article
Chemistry, Multidisciplinary
Jing Xu et al.
Summary: The introduction of silk fibroin (SF) as an electrolyte additive for aqueous zinc-ion batteries can form a stable and self-healable protective film, which promotes homogeneous zinc deposition and suppresses parasitic reactions, leading to improved cycle life of the batteries.
Article
Chemistry, Physical
Hefei Fan et al.
Summary: The introduction of a negatively charged protection layer on the zinc anode improves cycle stability and Coulombic efficiency by suppressing dendrite growth and hydrogen evolution. The protective layer also acts as a physical barrier and manipulates the local electrolyte structure to mitigate passivation on the anode surface.
Article
Chemistry, Multidisciplinary
Xiaofeng He et al.
Summary: The study introduces a concept of constructing an anion concentration gradient-assisted solid-electrolyte interphase for metal anodes, which enhances ionic conductivity and suppresses dendritic growth and side reactions. This new approach enables stable plating/stripping of zinc metal and shows improved cycling stability in various types of batteries and supercapacitors.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2022)
Article
Chemistry, Multidisciplinary
Dongdong Wang et al.
Summary: N-methyl pyrrolidone (NMP) is developed as a bifunctional electrolyte additive to improve the electrochemical performance of Zn anode, protecting it from corrosion and facilitating uniform plating/stripping of Zn.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2022)
Article
Chemistry, Multidisciplinary
Peichao Zou et al.
Summary: In this study, a new solution structure of aqueous electrolyte was reported, which achieved a hydrophobic anode-electrolyte interface by adding a suitable diluent, and reduced passivation layer formation through the hydroxyl-ion-scavenging functionality, improving the reversibility and lifetime of zinc metal batteries.
Article
Chemistry, Physical
Yifei Geng et al.
Summary: Aqueous Zn ion batteries (AZIBs) are a promising electrochemical energy storage device. Additive engineering is an innovative and flexible technology that effectively solves the challenges faced by AZIBs cathode and anode. This review summarizes the effects of additive engineering on cathode and anode, as well as the influence on charge storage mechanism and kinetic characteristics of AZIBs.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Physical
Zhenghui Pan et al.
Summary: In this study, a 3D ZnOHF nanowire array interface was in-situ built on Zn foil through a hydrothermal method, and used as a Zn2+ ion modulation layer to guide the reversible and long-cycling Zn plating/stripping processes. The ZnOHF NWs@Zn anode demonstrated a low Zn nucleation overpotential, high Zn storage capacity, and excellent coulombic efficiency, and showed outstanding cycle stability.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Physical
Wenjing Deng et al.
Summary: The study proposes a simple strategy to achieve high reversibility of metallic zinc in rechargeable batteries by introducing the organic solvent DMA as an electrolyte additive, which controls water activity, replaces water in Zn2+ solvation sheath, and reshapes the hydrogen-bonding network of water. This strategy enables remarkable suppression of water-involved hydrogen evolution and severe corrosion, leading to uniform deposition of zinc and long cycling life in batteries.
ENERGY STORAGE MATERIALS
(2022)
Article
Chemistry, Physical
Qiang Hu et al.
Summary: This study investigates the corrosion mechanism of Zn metal in slightly acidic electrolytes and proposes a method for co-modification of the Zn anode using ZnO@Cu solid solution interface and TS additive. Experimental results show that the modified Zn anode exhibits low polarization and high cycling stability.
JOURNAL OF MATERIALS CHEMISTRY A
(2022)
Review
Chemistry, Physical
Zhehan Yi et al.
Summary: Zinc-ion batteries are considered promising candidates for next-generation energy storage systems due to their high safety, resource availability, and environmental friendliness. However, the instability of the Zn metal anode has hindered their reliable deployment, and efforts have been made to overcome this through electrode structure design, interface modification, and electrolyte/separator optimization. Understanding and categorizing these strategies based on their intrinsic mechanisms are important for the development of novel Zn metal anodes for ZIBs.
ADVANCED ENERGY MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Yang Yang et al.
Summary: The study successfully developed a Zn@ZnF2 electrode with a multi-functional protective layer by designing a 3D interconnected ZnF2 matrix on the surface of Zn foil. This electrode exhibits stable zinc deposition kinetics and good plating/stripping reversibility, showing potential for practical application in various battery systems.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Sailin Liu et al.
Summary: By tuning the solvation structure of the electrolyte and using fire-retardant triethyl phosphate as a cosolvent, the challenges of cathode dissolution, water reactivity, and zinc dendrites in aqueous zinc-ion batteries have been successfully addressed. The optimized electrolyte structure leads to high average Coulombic efficiency in Zn/Cu cells and enables over 1000 cycles at high current density.
ADVANCED FUNCTIONAL MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Jiahui Zhou et al.
Summary: By synthesizing a nitrogen-doped graphene oxide film on zinc foil, this study effectively suppresses hydrogen evolution reactions and passivation, improving the electrochemical performance of aqueous Zn-ion batteries. This research provides a new method for enhancing the application of high-specific-energy AZIBs.
ADVANCED MATERIALS
(2021)
Article
Chemistry, Multidisciplinary
Peng Sun et al.
Summary: The addition of glucose in ZnSO4 electrolyte can improve the performance of Zn ion batteries by suppressing Zn dendrite growth and side reactions, enhancing stability.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Multidisciplinary
Xiao Liu et al.
Summary: The study introduces a biphasic organic electrolyte to resolve the migration issue of redox molecules in electrochemical energy-storage devices, effectively inhibiting the shuttle effect. This method significantly prolongs the cycle life of lithium redox flow batteries and lithium-O-2 batteries.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2021)
Article
Chemistry, Physical
Shao-Jian Zhang et al.
Summary: The study introduces a simple method using ethylene diamine tetraacetic acid tetrasodium salt (Na(4)EDTA) to suppress the poor reversibility of the Zn anode in aqueous Zn-ion batteries, effectively inhibiting dendrite growth and hydrogen evolution. Additionally, the added EDTA promotes desolvation of Zn, prolonging the electrode lifespan.
ADVANCED ENERGY MATERIALS
(2021)
Review
Chemistry, Physical
Wenjing Lu et al.
Summary: This review highlights the challenges facing rechargeable aqueous zinc-based batteries (ZBBs) and the importance of rational anode design. It also summarizes the progress on mitigation strategies to suppress unwanted electrochemical reactions and provides in-depth illustrations of the relevant mechanisms behind these strategies. This perspective aims to offer comprehensive guidance for constructing high-performance and dendrite-free ZBBs.
ACS ENERGY LETTERS
(2021)
Review
Chemistry, Multidisciplinary
Libei Yuan et al.
Summary: Aqueous Zn-ion batteries have attracted significant attention for their safety, cost effectiveness, and environmental friendliness, but challenges at the Zn/electrolyte interphase, such as dendrite growth and side reactions, still need to be addressed. Research in interfacial engineering has become a growing area of interest, providing effective evaluation techniques and strategies for improvement.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
Article
Chemistry, Multidisciplinary
Yang Dong et al.
Summary: This study presents a non-concentrated aqueous electrolyte composed of 2m zinc trifluoromethanesulfonate and the organic dimethyl carbonate additive, which can stabilize the zinc electrochemistry and improve the coulombic efficiency of the zinc anode. Furthermore, this electrolyte can sustain stable operation of rechargeable aqueous zinc batteries when paired with various cathode materials. Rational electrolyte design with organic solvent additives could lead to the development of better aqueous batteries.
Review
Electrochemistry
Yingbo Li et al.
Summary: Rechargeable Zn-ion batteries (RZIBs) are promising energy storage systems for large-scale applications due to their high energy densities, low costs, environmental friendliness, and safety. Despite significant advancements, challenges remain and reported results often cannot be translated to industrial applications due to exaggeration under ideal testing conditions.
BATTERIES & SUPERCAPS
(2021)
Article
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Zhao Cai et al.
ENERGY STORAGE MATERIALS
(2020)
Article
Chemistry, Physical
Xiaotan Zhang et al.
ENERGY STORAGE MATERIALS
(2020)
Article
Chemistry, Multidisciplinary
Longsheng Cao et al.
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
(2020)
Review
Chemistry, Multidisciplinary
Tengsheng Zhang et al.
ENERGY & ENVIRONMENTAL SCIENCE
(2020)
Article
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Huibing He et al.
JOURNAL OF MATERIALS CHEMISTRY A
(2020)
Review
Chemistry, Multidisciplinary
Junnan Hao et al.
ENERGY & ENVIRONMENTAL SCIENCE
(2020)
Review
Chemistry, Physical
Lauren E. Blanc et al.
Article
Multidisciplinary Sciences
Jingxu Zheng et al.
Article
Electrochemistry
Keliang Wang et al.
JOURNAL OF THE ELECTROCHEMICAL SOCIETY
(2019)
Article
Chemistry, Multidisciplinary
Zhiming Zhao et al.
ENERGY & ENVIRONMENTAL SCIENCE
(2019)
Article
Spectroscopy
Wenwen Xu et al.
JOURNAL OF RAMAN SPECTROSCOPY
(2018)
Article
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Fei Wang et al.
Article
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Alan M. Hyde et al.
ORGANIC PROCESS RESEARCH & DEVELOPMENT
(2017)
Article
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Paula Navalpotro et al.
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
(2017)
Article
Engineering, Environmental
Shang Jiang et al.
CHEMICAL ENGINEERING JOURNAL
(2017)
Article
Nanoscience & Nanotechnology
Sang-Don Han et al.
ACS APPLIED MATERIALS & INTERFACES
(2016)
Article
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Kjell W. Schroder et al.
JOURNAL OF PHYSICAL CHEMISTRY LETTERS
(2015)
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Miao Wang et al.
Article
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Feng Xu et al.
JOURNAL OF PHYSICAL CHEMISTRY C
(2010)
Article
Spectroscopy
Xiaopeng Xuan et al.
JOURNAL OF RAMAN SPECTROSCOPY
(2007)
