Fit-for-Use Nanofibrillated Cellulose from Recovered Paper

The cost-effective implementation of nanofibrillated cellulose (CNF) at industrial scale requires optimizing the quality of the nanofibers according to their final application. Therefore, a portfolio of CNFs with different qualities is necessary, as well as further knowledge about how to obtain each of the main qualities. This paper presents the influence of various production techniques on the morphological characteristics and properties of CNFs produced from a mixture of recycled fibers. Five different pretreatments have been investigated: a mechanical pretreatment (PFI refining), two enzymatic hydrolysis strategies, and TEMPO-mediated oxidation under two different NaClO concentrations. For each pretreatment, five high-pressure homogenization (HPH) conditions have been considered. Our results show that the pretreatment determines the yield and the potential of HPH to enhance fibrillation and, therefore, the final CNF properties. These results enable one to select the most effective production method with the highest yield of produced CNFs from recovered paper for the desired CNF quality in diverse applications.

Automated summary

This paper investigates the influence of various production techniques on the morphological characteristics and properties of nanofibrillated cellulose (CNF) produced from a mixture of recycled fibers. The results show that the pretreatment determines the yield and the potential of high-pressure homogenization (HPH) to enhance fibrillation, thus determining the final CNF properties. This enables effective selection of the most suitable production method to obtain high yield and desired CNF quality for diverse applications.