Degradation of Polylactic Acid Polymer and Biocomposites Exposed to Controlled Climatic Ageing: Mechanical and Thermal Properties and Structure

This paper deals with the study of the degradation of polylactic acid (PLA) material structures and biocomposite systems with a PLA matrix containing ground natural particulate waste fillers, buckwheat husks and egg shells. Waste fillers were used without difficult cleaning operations to describe the effect of the raw waste material on PLA. Biocomposites with raw waste materials are increasingly coming to the forefront in car interiors and packaging products. The prepared material systems were exposed to controlled climatic ageing simulating long-term solar radiation and cyclic outdoor conditions. The degradation of the biocomposite systems was evaluated via thermal (differential scanning calorimetry) and mechanical properties (tensile and flexural tests, Charpy impact toughness). In addition to evaluating the degradation of the material structures using standardized tests, the influence and effect of controlled climatic ageing was visually assessed using SEM images (electron microscopy) of the surfaces and fracture surfaces of the test specimens.

Automated summary

This paper investigates the degradation of biocomposite materials with a PLA matrix containing ground natural waste fillers. The degradation of the material systems was evaluated through thermal and mechanical properties tests, as well as visual assessment using SEM images of the surfaces and fracture surfaces of the test specimens under controlled climatic aging.