期刊
NANO LETTERS
卷 16, 期 9, 页码 5365-5372出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.6b01434
关键词
Li-S,battery; biomimetic; ant-nest structure; high sulfur radio
类别
资金
- Advanced Battery Materials Research (BMR) program from U.S. Department of Energy (U.S. DOE)
The lithium sulfur,(Li-S) rechargeable bat-tery has the benefit of high gravimetric energy density and low cost. Significant research currently focuses on increasing the sulfur loading and sulfur/inactive-materials ratio, to improve life and capacity. Inspired by nature's ant-nest structure, this research results in a novel Li-S electrode that is designed to meet both goals. With only three simple manufacturing friendly steps, which include slurry :ball-milling, doctor-blade based laminate casting, and the use of the sacrificial method with water to dissolve away table salt, the ant-nest design has been successfully recreated in an Li-S electrode. The efficient capabilities of the ant-nest structure are adopted to facilitate fast ion transportation, sustain polysulfide dissolution, and assist efficient precipitation. High cycling stability in the Li-S batteries, for practical applications, has been achieved with up to 3 mg.cm(-2) sulfur loading. Li-S electrodes with up to a 85% sulfur ratio have also been achieved for the efficient design of this novel ant-nest structure
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