期刊
NANO LETTERS
卷 16, 期 3, 页码 1554-1559出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.5b03954
关键词
2D materials; transition metal dichalcogenides; molybdenum disulfide; quantum confined Stark effect; electrical control; exciton polarizability
类别
资金
- Deutsche Forschungsgemeinschaft (DFG) through TUM International Graduate School of Science and Engineering (IGSSE)
- German Excellence Initiative via Nano-systems Initiative Munich
- PhD programme ExQM of the Elite Network of Bavaria
- Technische Universitat Munchen - Institute for Advanced Study - German Excellence Initiative
- Alexander von Humboldt Foundation
We demonstrate electrical control of the A-exciton inter band transition in mono- and few-layer MoS2 crystals embedded into photocapacitor devices via the DC Stark effect. Electric field dependent low-temperature photoluminescence spectroscopy reveals a significant tuneability of the A-exciton transition energy up to similar to 16 meV from which we extract the mean DC exciton polarizability <(beta) over bar (N)> = (0.58 +/- 0.25) x 10(-8) Dm V-1. The exciton polarizability is shown to be layer-independent, indicating a strong localization of both electron and hole wave functions in each individual layer.
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