期刊
NANO LETTERS
卷 16, 期 4, 页码 2851-2859出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.6b00712
关键词
Nanoferroics; organic crystallization; materials design; and multifuctionality
类别
资金
- Army Research Office - Young Investigator Program [W911NF-15-1-0610]
- U.S. Department of Energy-Basic Energy Sciences Award [DE-SC0014902]
- Department of Energy (DOE), Office of Science, Basic Energy Science (BES) [DE-SC0010307]
- U.S. Department of Energy (DOE) [DE-SC0010307, DE-SC0014902] Funding Source: U.S. Department of Energy (DOE)
Organic charge-transfer superstructures are enabling new interfacial electronics, such as organic thermoelectrics, spin-charge converters, and solar cells. These carbon-based materials could also play an important role in spin-based electronics due to their exceptionally long spin lifetime. However, to explore these potentials a coherent design strategy to control interfacial charge-transfer interaction is indispensable. Here we report that the control of organic crystallization and interfacial electron coupling are keys to dictate external stimuli responsive behaviors in organic charge-transfer superstructures. The integrated experimental and computational study reveals the importance of chemically driven interfacial coupling in organic charge-transfer superstructures. Such degree of engineering opens up a new route to develop a new generation of functional charge-transfer materials, enabling important advance in all organic interfacial electronics.
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