4.7 Article

Enhancing the performances of EB-PVD TBCs via overlayer Al-modification

期刊

SURFACE & COATINGS TECHNOLOGY
卷 473, 期 -, 页码 -

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ELSEVIER SCIENCE SA
DOI: 10.1016/j.surfcoat.2023.130001

关键词

TBCs; EB-PVD; Bending properties; Oxidation resistance; CMAS corrosion

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In this study, an Al film was applied on the surface of EB-PVD TBCs and converted to alpha-Al2O3, which improved the lifespan of the TBCs. Alpha-Al2O3 had a toughening effect, enhanced high-temperature oxidation resistance, and prevented CMAS penetration and corrosion. Moreover, Al modification improved surface roughness and wetting resistance of the TBCs.
Thermal barrier coatings (TBCs) guarantee the service life of high-temperature alloy substrates under harsh service environments. Premature failure of TBCs due to coating fracture, high-temperature oxidation, and calcium oxide-magnesium oxide-aluminum oxide-silicon oxide (CMAS) corrosion, which significantly reduce their service lifespan. In this study, Al film was applied on the surface of EB-PVD TBCs using arc ion plating, and then converted it to alpha-Al2O3 by an in situ reaction between Al and ZrO2. The alpha-Al2O3 have toughening effect resulting in a higher bending resistance of EB-PVD TBCs. Because alpha-Al2O3 could seal the columnar inter-crystal gaps on the surface of EB-PVD TBCs, it reduced oxygen penetration, which enhanced the high-temperature oxidation resistance. CMAS reacted with alpha-Al2O3 to generate spinel and calcium-aluminum yellow feldspar compounds at 1350 degrees C, which prevented following CMAS penetration and corrosion. Furthermore, Al-modification reduced the surface roughness, which made Al-modified TBCs have better wetting resistance.

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