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First-Row Transition Metals for Catalyzing Oxygen Redox

SMALL (2023)

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Article Chemistry, Physical

CNTs/CNF-supported multi-active components as highly efficient bifunctional oxygen electrocatalysts and their applications in zinc-air batteries

Weiyuan Ding et al.

Summary: In this study, FeCo nanoparticles, MNx (M = Fe, Co), and FePx were embedded in porous and graphitized carbon nanotubes (CNTs)/carbon nanofiber (CNF) using electrospinning and chemical vapor deposition (CVD) techniques. The prepared FeCo@CoNx@FePx/C exhibited a high half-wave potential of 0.86 V in oxygen reduction reaction (ORR) and a low oxygen evolution reaction (OER) overpotential of 368 mV at 10 mAmiddotcm(-2). The assembled Zn-air battery (ZAB) showed a high energy efficiency of 65% at 20 mAmiddotcm(-2) and remained stable for 700 charge-discharge cycles. This work has important implications for the design of bifunctional electrocatalysts.

NANO RESEARCH (2023)

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Review Chemistry, Multidisciplinary

Advances in Spin Catalysts for Oxygen Evolution and Reduction Reactions

Haoyun Bai et al.

Summary: This review discusses the recent development of spin catalysts and explores the origins for the improved catalytic activity. Firstly, an introduction is given on the applications and advances in spin-related catalytic phenomena, followed by the fundamental principles of spin catalysts and magnetic fields-radical reactions. The spin-related catalytic performance reported in oxygen evolution/reduction reaction (OER/ORR) is systematically discussed, and general rules are summarized accordingly. Finally, the challenges and perspectives are provided.

SMALL (2023)

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Article Chemistry, Physical

Engineering Self-Supported Hydrophobic-Aerophilic Air Cathode with CoS/Fe3S4 Nanoparticles Embedded in S, N Co-Doped Carbon Plate Arrays for Long-Life Rechargeable Zn-Air Batteries

Lei Yan et al.

Summary: A hydrophobic-aerophilic strategy is developed to engineer the reaction kinetics at air cathodes by fabricating a self-supported air cathode based on CoS/Fe3S4 nanoparticles encapsulated in S, N co-doped carbon plate arrays (CoS/Fe3S4@SNCP). The in situ growth of bimetallic sulfides nanoparticles on the carbon plate arrays improves the intrinsic electrocatalytic activity and electron conduction of the air cathode. The hydrophobic-aerophilic surface repels water molecules and creates abundant solid-liquid-gas three-phase reaction interfaces, promoting the diffusion of reactive molecules/ions and oxygen adsorption.

ADVANCED ENERGY MATERIALS (2023)

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Review Chemistry, Physical

Research progress on the construction of synergistic electrocatalytic ORR/OER self-supporting cathodes for zinc-air batteries

Qi Liu et al.

Summary: In this review, the application of non-precious metal-based self-supporting electrodes in Zn-air batteries (ZABs) is systematically summarized. The basic structure and principle of ZABs, as well as a reasonable electrode preparation method, are introduced. The reaction mechanism is discussed for a deep understanding of the real active sites. The progress, challenges, and future directions of self-supporting electrodes in ZABs are presented.

JOURNAL OF MATERIALS CHEMISTRY A (2023)

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Article Chemistry, Physical

The OER/ORR activities of copper oxyhydroxide series electrocatalysts

Yilei Yue et al.

Summary: In this work, the OER/ORR electrocatalytic activity of all CuOOH series was investigated using the DFT method, and an improvement scheme was proposed. The results showed that pure CuOOH catalysts were inert towards OER/ORR, but their performances could be significantly improved by Co or Rh doping. This work revealed the OER/ORR performance of the CuOOH series, which will help us to understand and improve the OER/ORR performance of previous copper oxide electrocatalysts.

MOLECULAR CATALYSIS (2023)

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Article Chemistry, Physical

Structural design of supported electrocatalysts for rechargeable Zn-air batteries

Qian Lu et al.

Summary: This review summarizes the structural design of supported electrocatalysts using different types of supports, including carbon materials and transition metal compounds. The configuration and role of transition metal catalysts on carbon supports are discussed, as well as the synthesis strategies for achieving controllable preparation. Personal perspectives for developing more efficient bifunctional electrocatalysts in the future are also presented.

ENERGY STORAGE MATERIALS (2023)

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Article Chemistry, Physical

Advanced Zn-air batteries based on efficient and durable perovskite/dual-doped graphene bifunctional oxygen catalysts

Ziyi Shui et al.

Summary: Rechargeable Zn-air batteries are considered promising energy storage devices due to their high energy and power density, safety, and cost-effectiveness. However, the sluggish kinetics of the oxygen reaction during discharge and charge processes have hindered their practical application. In this study, LSFMO nanoparticles synthesized with a modified coprecipitation method exhibited high intrinsic activities. Furthermore, the synergic covalent coupling between N/S dual-doped reduced graphene and LSFMO significantly improved the oxygen reduction and evolution reaction capabilities of the LSFMO@NS-RGO hybrid material. The excellent results demonstrated that LSFMO@NS-RGO represents a new class of promising bifunctional catalysts for rechargeable Zn-air batteries.

JOURNAL OF ALLOYS AND COMPOUNDS (2023)

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Article Engineering, Electrical & Electronic

A Nanosized Manganese-Based Chalcogenide Composite for Enhanced Electrocatalytic OER

F. F. Alharbi et al.

Summary: The slow kinetics of water-splitting reaction and the need for improved oxygen evolution reaction (OER) electrocatalysts have been identified as major barriers to hydrogen production from water. This study investigates the effectiveness of inexpensive manganese bichalcogenide heterostructures and their equivalents, manganese oxide (MnO) and manganese sulfide (MnS), as electrocatalysts for water splitting. Various techniques such as powder X-ray diffraction (PXRD), Fourier transform infrared (FTIR) spectroscopy, and scanning electron microscopy (SEM) are employed to study these electrocatalysts. The results show that the MnS/MnO electrocatalyst exhibits remarkable efficiency and stability, outperforming other rare earth metal and Mn-based electrocatalysts under identical electrochemical conditions. The stability analysis indicates that the fabricated nanohybrids remain stable for 30 hours after 1000 cycles. This innovation provides a promising non-noble metal electrocatalyst for OER.

JOURNAL OF ELECTRONIC MATERIALS (2023)

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Article Chemistry, Multidisciplinary

A Fe Single Atom Seed-Mediated Strategy Toward Fe3C/Fe-N-C Catalysts with Outstanding Bifunctional ORR/OER Activities

Jiangwei Chang et al.

Summary: A Fe single atom seed-mediated strategy is reported for the fabrication of Fe3C species closely surrounded by Fe-N-4-C active sites with strong electronic interactions built between them. The compositionally-optimized Fe-N-C/Fe3C-op electrocatalyst shows a small voltage difference between the ORR half-wave and OER potential, making it one of the best bifunctional OER/ORR benchmarks. Assembled zinc-air batteries with Fe-N-C/Fe3C-op as the air cathode exhibit remarkable specific capacity and power density, along with excellent long-term durability. This work extends the methodology for modulating the activity of Fe-N-4-C atomic site, inspiring further exploration in the design of bifunctional oxygen electrocatalysts.

ADVANCED SCIENCE (2023)

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Review Chemistry, Multidisciplinary

Magnetoelectric Coupling for Metal-Air Batteries

Hengwei Wang et al.

Summary: Metal-air batteries are considered as a promising source of electrochemical energy due to their excellent characteristics and low cost. However, commercialization is hindered by slow kinetics, corrosion, and dendrite growth. The use of magnetic fields has shown promise in improving the performance of these batteries by enhancing mass transfer, charge transfer, and electrocatalysis.

ADVANCED FUNCTIONAL MATERIALS (2023)

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Article Chemistry, Multidisciplinary

Engineering the Electronic Structure of Single-Atom Iron Sites with Boosted Oxygen Bifunctional Activity for Zinc-Air Batteries

Zhijun Li et al.

Summary: Researchers have developed a new catalyst consisting of atomically dispersed iron atoms supported on a mesoporous nitrogen-doped carbon material. This catalyst exhibits remarkable activity for both oxygen reduction and evolution reactions in a wide pH range. The zinc-air battery assembled with this catalyst outperforms the traditional Pt/C+RuO2 counterpart in terms of power density, capacity, and cycling stability. These findings highlight the importance of electronic structure engineering of metal sites in catalytic activity.

ADVANCED MATERIALS (2023)

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Article Materials Science, Ceramics

High-performance MnO/N-rGO catalyst for half-cell and Zn-air batteries by photochemically assisted synthesis

Chenghong Sun et al.

Summary: The development of efficient cathode-side ORR catalysts is crucial for the practical application of fuel cells and ZABs. In this study, a facile and green photochemical method is used to synthesize MnO/N-rGO catalysts with highly catalytical activity and stability. The catalysts exhibit exciting ORR performance in alkaline media and outperform Pt/C-based GDE half-cell and Pt/C + RuO2-based ZABs in terms of overall performance and long-term durability. The synergistic effect between MnO nanoparticles and N-rGO support is the key factor contributing to their enhanced performance.

CERAMICS INTERNATIONAL (2023)

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Review Electrochemistry

Carbon-Based Electrodes for Advanced Zinc-Air Batteries: Oxygen-Catalytic Site Regulation and Nanostructure Design

Wenjie Shao et al.

Summary: In this review, the design and optimization methods of nanostructured carbon-based electrodes for advanced Zn-air batteries are comprehensively summarized. By tailoring the structure of carbon-based materials and oxygen catalytic centers, the performance of oxygen electrodes can be improved. Furthermore, recent progress in engineering flexible and high-power Zn-air batteries is briefly outlined, and the challenges and future perspectives on the rational design of nanostructured carbon-based oxygen electrodes are discussed.

ELECTROCHEMICAL ENERGY REVIEWS (2023)

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Review Chemistry, Physical

Lanthanum modified Fe3N/carbon foam as highly efficient electrode for zinc-air batteries

Minghui Wang et al.

Summary: Efficient electrocatalysts for ORR and OER are important for large-scale application of rechargeable zinc-air batteries. Iron-nitrogen-carbon materials exhibit excellent ORR catalytic activity, but have low OER performance. This study applies lanthanum (La) to enhance the OER electrocatalytic properties of Fe-N-C materials. The modified La-Fe3N carbon foam (La-Fe0.1:1/NFC) shows improved bi-functional electrocatalytic performance and high power density in a real zinc-air battery cell.

JOURNAL OF ALLOYS AND COMPOUNDS (2023)

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Review Chemistry, Multidisciplinary

Toward Excellence of Electrocatalyst Design by Emerging Descriptor-Oriented Machine Learning

Jianwen Liu et al.

Summary: Machine learning (ML) is a powerful tool for accelerating electrocatalyst design by learning from historic data without explicit programming. This review provides a summary of the application of ML in electrocatalyst design and tracks its progress and potential changes in different electrocatalytic reactions. The selection tactics for descriptors are identified as a current challenge.

ADVANCED FUNCTIONAL MATERIALS (2022)

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Article Chemistry, Multidisciplinary

Linker-Compensated Metal-Organic Framework with ElectronDelocalized Metal Sites for Bifunctional Oxygen Electrocatalysis

Yi Jiang et al.

Summary: This study proposes a linker compensation strategy to enhance the catalytic performance of metal-organic frameworks. By compensating the metal nodes, the performance of zinc-air batteries can be improved, resulting in higher current density and more stable voltage gap.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Article Chemistry, Multidisciplinary

Superdurable Bifunctional Oxygen Electrocatalyst for High-Performance Zinc-Air Batteries

Chenhui Zhou et al.

Summary: A Mn-doped RuO2 bimetallic oxide with atomic-scale dispersion of Mn atoms exhibits remarkable activity and super durability for both ORR and OER, providing a new catalyst design strategy for Zn-air batteries.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2022)

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Review Chemistry, Multidisciplinary

Recent Advances in ZIF-Derived Atomic Metal-N-C Electrocatalysts for Oxygen Reduction Reaction: Synthetic Strategies, Active Centers, and Stabilities

Chen Gao et al.

Summary: This review highlights the significance of exploring highly active and stable electrocatalysts with earth-abundant metal centers for the oxygen reduction reaction (ORR). The focus is on the synthetic strategies and design principles of metal-N-C (M-N-C) electrocatalysts derived from zeolite imidazolate framework (ZIF) for efficient ORR catalysis. The review discusses methods to improve intrinsic ORR activity, such as coordination structures, doping metal-free heteroatoms, and edge-hosted structures, as well as strategies to increase active site density, including formation of M-N complexes and porous structure design.

SMALL (2022)

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Article Multidisciplinary Sciences

Manipulating the oxygen reduction reaction pathway on Pt-coordinated motifs

Jiajun Zhao et al.

Summary: Controlling the coordination environment of Pt can manipulate the 2e(-) or 4e(-) reduction pathways, leading to controlled product selectivity and H2O2 generation rate during oxygen reduction.

NATURE COMMUNICATIONS (2022)

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Article Chemistry, Physical

Atomically Dispersed Fe-Co Dual Metal Sites as Bifunctional Oxygen Electrocatalysts for Rechargeable and Flexible Zn-Air Batteries

Yuting He et al.

Summary: This study presents atomically dispersed Fe-Co dual metal sites derived from Fe and Co codoped zeolitic imidazolate frameworks, showing excellent bifunctional catalytic activity for ORR and OER in alkaline media. The FeCo-NC catalyst exhibits outstanding stability and is integrated into an air electrode for fabricating rechargeable and flexible Zn-air batteries, achieving a high power density and long-cycle stability. This work offers a method to design and synthesize atomically dispersed multi-metal site catalysts for advanced electrocatalysis.

ACS CATALYSIS (2022)

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Review Nanoscience & Nanotechnology

Atomically Dispersed Transition Metal-Nitrogen-Carbon Bifunctional Oxygen Electrocatalysts for Zinc-Air Batteries: Recent Advances and Future Perspectives

Fang Dong et al.

Summary: This paper reviews the general principles for designing atomically dispersed M-N-C catalysts and presents strategies to enhance their bifunctional catalytic activity and stability. It also outlines the challenges and perspectives of using M-N-C catalysts for rechargeable zinc-air batteries.

NANO-MICRO LETTERS (2022)

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Article Chemistry, Physical

Modulation of pore-size in N, S-codoped carbon/Co9S8 hybrid for a stronger O2 affinity toward rechargable zinc-air battery

Qi Zheng et al.

Summary: Introducing porosity into the carbon structure enhances the electrocatalytic activity for oxygen reduction reaction by improving wetting property and interaction with O2. The NSC/Co9S8 sample with an average pore size of 200 nm showed the best catalytic activities and was used in rechargeable zinc-air batteries, demonstrating significantly improved durability and stability. This study showcases a versatile and clever strategy for regulating advanced electrocatalytic materials, enabling their integration into flexible, secure energy storage and conversion devices.

NANO ENERGY (2022)

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Review Electrochemistry

MOF/PCP-based Electrocatalysts for the Oxygen Reduction Reaction

Liang Tang et al.

Summary: The oxygen reduction reaction (ORR) is the fundamental reaction at the cathode of a fuel cell. Metal-organic frameworks (MOFs) or porous coordination polymers (PCPs) are considered the most promising catalytic material for the ORR due to their large specific surface area, high porosity, and tunable chemical structure. This review discusses the research progress and latest development of MOF/PCP applications as ORR catalysts, including the basic principles and the design rules of MOFs/PCPs as ORR catalysts.

ELECTROCHEMICAL ENERGY REVIEWS (2022)

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Article Chemistry, Physical

Regulation and mechanism study of the CoS2/Cu2S-NF heterojunction as highly-efficient bifunctional electrocatalyst for oxygen reactions

Wanqing Li et al.

Summary: The study focuses on designing and synthesizing a CoS2/Cu2S heterostructured composite that enhances the electronic transfer and interaction, leading to improved efficiency in oxygen reaction electrocatalysis. This heterostructure exhibits the lowest potential difference compared to commercial catalysts and shows great potential for application in rechargeable metal-solid batteries.

APPLIED CATALYSIS B-ENVIRONMENTAL (2022)

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Article Chemistry, Physical

Flower-like Mesoporous Carbon with Cobalt Sulfide Nanocrystalline as Efficient Bifunctional Electrocatalysts for Zn-Air Batteries

Haoran Zhou et al.

Summary: Transition-metal sulfides have gained attention for their efficient activity in rechargeable Zn-air batteries. This study successfully synthesized cobalt sulfide nanocrystalline electrocatalysts supported on hierarchically porous nanocarbon and demonstrated excellent bifunctional oxygen catalytic performance. The rechargeable Zn-air batteries assembled with the cobalt sulfide-based hierarchically porous electrocatalysts exhibited high peak power density and cycling stability.

CHEMCATCHEM (2022)

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Article Engineering, Environmental

Rechargeable sunlight-promoted Zn-air battery constructed by bifunctional oxygen photoelectrodes: Energy-band switching between ZnO/Cu2O and ZnO/CuO in charge-discharge cycles

Degang Bu et al.

Summary: This study successfully achieved low charge potential and high discharge potential in rechargeable Zn-air batteries by constructing highly efficient and stable bifunctional photoelectrodes. The investigation revealed the electrocatalytic mechanism involved, providing new insights for the development of other photo-assisted batteries.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Green & Sustainable Science & Technology

Research progress in transition metal oxide based bifunctional electrocatalysts for aqueous electrically rechargeable zinc-air batteries

Maria Mechili et al.

Summary: Zinc-air batteries have great potential in the power sources sector due to their high energy capacity and eco-friendly characteristics. However, the practical large-scale adoption of rechargeable alka-line aqueous ZABs is hindered by poor resistivity and cyclability. This article provides a detailed summary of the electrochemical properties and performance of transition metal oxide-based materials as bifunctional electrocatalysts in zinc-air batteries, aiming to provide a foundation for further research in performance-oriented electrocatalysts. Recent advances in simple metal oxide, spinel oxide, and perovskite oxide-based nanomaterials and nanohybrids are also examined in rechargeable liquid alkaline ZAB configurations.

RENEWABLE & SUSTAINABLE ENERGY REVIEWS (2022)

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Article Chemistry, Applied

Enhanced bifunctional catalytic activities of N-doped graphene by Ni in a 3D trimodal nanoporous nanotubular network and its ultralong cycling performance in Zn-air batteries

Yanyi Zhang et al.

Summary: This work synthesized a flexible air electrode consisting of 3D nanoporous N-doped graphene and Ni particles, showing enhanced ORR and OER activities with improved durability. Synergetic effects between Ni and N-doped graphene were revealed, boosting bifunctional activities and enhancing stability for long-lasting discharge/recharge cycles. The trimodal graphene/Ni structure shows potential for various flexible energy conversion/storage devices.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Applied

One-pot synthesis of FeNxC as efficient catalyst for high-performance zinc-air battery

Yang Li et al.

Summary: Rechargeable zinc-air batteries have high theoretical energy density but suffer from high polarization and low energy efficiency. A noble-metal-free FeNxC electrocatalyst was developed to enhance oxygen reduction reaction kinetics, leading to improved performance in charge-discharge voltage gap, peak power density, and long-term durability. This work provides significant support for the practical application of zinc-air batteries in the future.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Applied

In-situ growth of CoNi bimetal anchored on carbon nanoparticle/nanotube hybrid for boosting rechargeable Zn-air battery

Jun Li et al.

Summary: In this study, a facile coprecipitation method was used to synthesize CoNi anchored carbon nanoparticle/nanotube (CoNi/N-CNN) hybrid with MOFs as precursors for efficient bifunctional oxygen electrode in metal-air batteries. The CoNi/N-CNN catalyst exhibited excellent performance for both ORR and OER, providing high discharge power density and outstanding cycling stability for rechargeable Zn-air batteries. The enhanced electrocatalytic activity was attributed to the strong coupling effect between Co/Ni center sites and defect-rich N-anchored carbon structures.

JOURNAL OF ENERGY CHEMISTRY (2022)

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Article Chemistry, Multidisciplinary

In Situ Monitored (N, O)-Doping of Flexible Vertical Graphene Films with High-Flux Plasma Enhanced Chemical Vapor Deposition for Remarkable Metal-Free Redox Catalysis Essential to Alkaline Zinc-Air Batteries

Zhiheng Wu et al.

Summary: A high-performance metal-free bifunctional catalyst was successfully synthesized for rechargeable zinc-air batteries, outperforming traditional precious-metal catalysts in terms of performance. This research provides a solid foundation for developing low-cost, resource-sustainable, and eco-friendly metal-free zinc-air batteries.

ADVANCED SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Interfacial Engineering of a Phase-Controlled Heterojunction for High-Efficiency HER, OER, and ORR Trifunctional Electrocatalysis

Yichuan Li et al.

Summary: The development of low-cost and high-performance electrocatalysts for the hydrogen evolution reaction (HER), oxygen evolution reaction (OER), and oxygen reduction reaction (ORR) is crucial. The researchers developed a strategy for scalable synthesis of a FexP/Fe3C-based heterojunction with controllable iron phosphide crystal phases. The resulting catalyst exhibited excellent electrocatalytic performance for HER, OER, and ORR due to the synergistic effect between FeP/Fe3C and N- and P-codoped carbon (NPC).

ACS OMEGA (2022)

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Article Chemistry, Physical

Interpretable machine learning for knowledge generation in heterogeneous catalysis

Jacques A. Esterhuizen et al.

Summary: Most applications of machine learning in heterogeneous catalysis use black-box models, which are not easily interpretable. Interpretable machine learning methods offer an alternative by merging the predictive capacity of black-box models with the interpretability of physics-based models. This Perspective discusses the potential, challenges, and opportunities of interpretable machine learning in catalysis research.

NATURE CATALYSIS (2022)

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Article Chemistry, Physical

Pd@SmMn2O5 as an Efficient Oxygen Reduction Reaction Catalyst via Triggering the Synergistic Effect between Dual Crystal Fields in Mullite

Chunning Zhao et al.

Summary: By optimizing the metal-semiconductor interface, the catalytic activity of the catalyst is enhanced for electrochemical reactions.

ACS APPLIED ENERGY MATERIALS (2022)

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Article Engineering, Environmental

Activating Cu/Fe2O3 nanoislands rooted on N-rich porous carbon nanosheets via the Mott-Schottky effect for rechargeable Zn-air battery

Qing Dong et al.

Summary: The study developed a Mott-Schottky electrocatalyst Cu NDs/Fe2O3-NPCs to enhance electron transfer and catalytic activities for ORR and OER in ZABs. The porous structure of the catalyst contributed to improved mass transfer efficiency, leading to excellent electrocatalytic performance.

CHEMICAL ENGINEERING JOURNAL (2022)

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Article Chemistry, Physical

A photonic hydrogel for health self-monitoring of solid-state electrolytes in zinc-air batteries

Yayu Zuo et al.

Summary: This study presents a novel strategy for the health monitoring of solid-state electrolytes based on photonic metamaterials. By combining double-network hydrogels with photonic crystals, the water content of solid-state electrolytes can be monitored in real-time. The method allows for the characterization of ionic conductivity and offers a flexible zinc-air battery design with high charging-discharging efficiency and low-temperature operation capability.

ENERGY STORAGE MATERIALS (2022)

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Article Chemistry, Physical

Three-phases Co/Co9S8/MnS heterostructures engineering for boosted ORR/OER activities in Zn-air batteries

Kaiyue Chen et al.

Summary: This study introduces the MnS phase into the Mott-Schottky Co/Co9S8 to create a three-phases Co/Co9S8/MnS heterojunction catalyst on defect-rich N-doped mesoporous carbon substrate. It improves the bifunctional ORR/OER activities and shows promising potential for practical applications.

MATERIALS TODAY ENERGY (2022)

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Review Engineering, Multidisciplinary

Recent advances in bifunctional catalysts for zinc-air batteries: Synthesis and potential mechanisms

Zhao LinWei et al.

Summary: Zinc-air batteries are promising candidates for clean and sustainable energy storage, but their practical application is challenging. The design of bifunctional ORR/OER electrocatalysts is crucial for the development of ZABs, and significant progress has been made in this area.

SCIENCE CHINA-TECHNOLOGICAL SCIENCES (2022)

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Article Chemistry, Physical

Open Challenges in Developing Generalizable Large-Scale Machine-Learning Models for Catalyst Discovery

Adeesh Kolluru et al.

Summary: This article discusses the application of machine learning in catalyst discovery and introduces the importance and challenges of the Open Catalyst 2020 Data set (OC20). The article emphasizes the potential of building universal machine-learning potentials to accelerate catalyst discovery and discusses the performance of current models and some method improvements.

ACS CATALYSIS (2022)

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Article Chemistry, Physical

Co2FeO4@rGO composite: Towards trifunctional water splitting in alkaline media

Abdul Hanan et al.

Summary: This study develops a composite system based on carbon materials and transition metal-based compounds, resulting in the synthesis of an optimized Co2FeO4@rGO composite. The composite exhibits outstanding multifunctional applications in the oxygen evolution reaction (OER) and hydrogen counterpart (HER) due to its high electrical conductivity, density of active sites, crystal defects, oxygen vacancies, and favorable electronic structure.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2022)

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Article Green & Sustainable Science & Technology

Ag Decorated Co3O4-Nitrogen Doped Porous Carbon as the Bifunctional Cathodic Catalysts for Rechargeable Zinc-Air Batteries

Pingshu Leng et al.

Summary: The synthesis of bifunctional Ag-decorated Co3O4-nitrogen doped porous carbon composite catalysts improved the performance of zinc-air batteries, increasing the open circuit voltage, power density, and specific discharge capacity. Additionally, the charge-discharge performance exhibited better long-term stability.

SUSTAINABILITY (2022)

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Article Chemistry, Physical

Transition metal embedded graphynes as advanced bifunctional single atom catalysts for oxygen reduction and evolution reactions

Shu-Long Li et al.

Summary: Noble metals are efficient for ORR and OER, but their scarcity and high price limit commercial applications. This study screened 26 TM-GY as potential SACs for ORR/OER, revealing candidates like Fe, Ir, Co, Rh, Cu, Ni, Pd and Pt-GY, with Co-GY as the optimal bifunctional SAC.

APPLIED SURFACE SCIENCE (2022)

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Article Chemistry, Multidisciplinary

Self-standing Fe3O4 decorated paper electrode as a binder-free trifunctional electrode for electrochemical ammonia synthesis and Zn-O2 batteries

Alankar Kafle et al.

Summary: The conversion of abundant biodegradable materials into electroactive electrode material can provide sustainable energy conversion and storage solutions. In this study, a simple and cost-effective method using electroless-electrodeposition is presented to fabricate flexible cellulose paper electrodes. The as-fabricated paper electrode shows promising activity and stability in electrochemical reactions, making it suitable for various applications.

NANOSCALE (2022)

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Article Chemistry, Applied

Copper-doped nickel oxyhydroxide for efficient electrocatalytic ethanol oxidation

Huining Wang et al.

Summary: In this study, a copper-doped nickel oxyhydroxide catalyst was successfully developed via in-situ electrochemical reconstruction of a NiCu alloy. The introduction of copper dopants increased the specific surface area, defect sites, and high-valence nickel sites of the catalyst. The Cu-doped NiOOH catalyst exhibited excellent performance in the ethanol oxidation reaction, with high peak current density, high Faradic efficiencies for acetate production, and good electrochemical stability.

CHINESE JOURNAL OF CATALYSIS (2022)

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Article Chemistry, Multidisciplinary

Electrochemical Reduction of Carbon Dioxide and Iron Oxide in Molten Salts to Fe/Fe3C Modified Carbon for Electrocatalytic Oxygen Evolution

Xinxin Liang et al.

Summary: By combining the electrochemical reduction of CO2 with Fe2O3 in molten salts, an enhanced Fe3C-based electrocatalyst is prepared with improved current efficiency, outperforming precious metal catalysts in 1 M KOH for more effective OER operation.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2021)

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Article Chemistry, Multidisciplinary

Stable confinement of Fe/Fe3C in Fe, N-codoped carbon nanotube towards robust zinc-air batteries

Lingbo Zong et al.

Summary: A superior nonprecious bifunctional oxygen electrocatalyst, Fe/Fe3C-N-CNTs, was developed through spatial confinement of Fe/Fe3C nanocrystals in pyridinic N and Fe-N-x rich carbon nanotubes. This electrocatalyst showed high activity, durability and stability in oxygen reduction and evolution reactions, presenting a potential alternative to precious metal-based catalysts for metal-air batteries.

CHINESE CHEMICAL LETTERS (2021)

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Article Chemistry, Physical

FeS2-CoS2 incorporated into nitrogen-doped carbon nanofibers to boost oxygen electrocatalysis for durable rechargeable Zn-air batteries

Xiaojun Shi et al.

Summary: The FeS2-CoS2/NCFs integrated electrocatalyst shows high bifunctional activity and durability in alkaline medium, outperforming precious metal-based zinc-air batteries. It also demonstrates practical potentials in flexible solid-state zinc-air batteries, powering LED panels even under twisting state.

JOURNAL OF POWER SOURCES (2021)

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Article Chemistry, Applied

ZIF-67-templated synthesis of core-shell-structured POP@MOF composite derived porous carbon with embedding FeCo alloy nanoparticles as high-performance bifunctional oxygen electrocatalysts

Meng Zhang et al.

Summary: A new composite material with controllable morphology and Fe/Co molar ratio was prepared, which can be further converted into N-doped porous carbons embedded with highly active sites. The optimal catalyst with hierarchical pore structure showed high ORR and OER activity in alkaline conditions, due to enhanced mass transfer efficiency and exposure of active sites.

MICROPOROUS AND MESOPOROUS MATERIALS (2021)

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Article Chemistry, Physical

Oxygen evolution reaction over catalytic single-site Co in a well-defined brookite TiO2 nanorod surface

Chang Liu et al.

Summary: Efficient single-site Co catalysts supported on well-defined TiO2 nanorods were found to exhibit excellent performance in the oxygen evolution reaction (OER), with turnover frequencies among the highest reported for Co-based catalysts. Computational and experimental results showed good agreement in describing the catalytic reaction kinetics and mechanisms.

NATURE CATALYSIS (2021)

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Article Chemistry, Physical

Efficient oxygen evolution reaction in SrCo0.8Fe0.2O3-δ perovskite and surface reconstruction for practical zinc-air batteries

Rigang Nie et al.

Summary: The synthetic catalyst SCF-0.2, obtained by simple heating of SrCo0.8Fe0.2O3-δ (SCF-0) material in a H3BO3 solution, exhibits excellent OER activity, with significant enhancement in specific surface area attributed to improved surface morphology.

APPLIED SURFACE SCIENCE (2021)

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Article Electrochemistry

A Highly Active Bifunctional Catalyst of Mn-Co-Fe-N/S@CNT for Rechargeable Zinc-Air Batteries

Keliang Wang et al.

Summary: The article introduces a highly efficient catalyst for the oxygen reduction reaction and demonstrates its potential application in rechargeable zinc-air batteries. The research findings indicate that Mn-Co-Fe-N/S@CNT has higher electrocatalytic activity than commercial catalysts, improving battery performance.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2021)

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Article Chemistry, Physical

Recent perspectives on the structure and oxygen evolution activity for non-noble metal-based catalysts

Qiwen Pan et al.

Summary: This review presents recent perspectives on the OER mechanisms of non-precious metal-based catalysts, discussing construction strategies of electrocatalysts and fundamental mechanisms for enhancing catalytic activity.

JOURNAL OF POWER SOURCES (2021)

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Article Chemistry, Multidisciplinary

Ultrastable FeCo Bifunctional Electrocatalyst on Se-Doped CNTs for Liquid and Flexible All-Solid-State Rechargeable Zn-Air Batteries

Hongwei Zhang et al.

Summary: In this study, an ultrastable FeCo bifunctional oxygen electrocatalyst on Se-doped CNTs was synthesized, showing excellent oxygen reduction and oxygen evolution reaction activities, surpassing commercial catalysts. The FeCo/Se-CNT catalyst demonstrated extraordinary stability and superior performance in rechargeable Zn-air batteries.

NANO LETTERS (2021)

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Article Chemistry, Physical

Zinc dendrite growth and inhibition strategies

Y. Zuo et al.

Summary: Zinc is an ideal energy carrier with high energy density, low cost, and environmental friendliness, but the issue of zinc dendrite growth remains unresolved. Understanding the formation mechanism of zinc dendrites is necessary to guide inhibition strategies.

MATERIALS TODAY ENERGY (2021)

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Article Energy & Fuels

Microwave-Assisted Facile Hydrothermal Synthesis of Fe3O4-GO Nanocomposites for the Efficient Bifunctional Electrocatalytic Activity of OER/ORR

Kashinath Lellala

Summary: The study introduces a successful development of ultrafine Fe3O4 nanoparticles uniformly decorated on graphene oxide sheets using a microwave-assisted hydrothermal method, showing promising bifunctional oxygen reaction activities. The heterostructure composites exhibit highly efficient performance for oxygen evolution/reduction reactions in both KOH and H2SO4 solutions, providing potential insights for designing efficient catalysts in various electrochemical activities.

ENERGY & FUELS (2021)

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Article Chemistry, Physical

Enhancing the electrocatalytic activity via hybridization of Cu(I/II) oxides with Co3O4 towards oxygen electrode reactions

Kumar Kashyap Hazarika et al.

Summary: The transition metal oxide based electrocatalyst with mixed valence state exhibits high activity and stability, showing promising potential for oxygen electrocatalysis.

JOURNAL OF POWER SOURCES (2021)

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Article Nanoscience & Nanotechnology

Atomic layer deposited nickel sulfide for bifunctional oxygen evolution/reduction electrocatalysis and zinc-air batteries

Shihan Yan et al.

Summary: This study introduces a novel non-precious NiS(x)/CNT electrocatalyst, which enhances the kinetics of oxygen reduction and oxygen evolution reactions in zinc-air batteries, resulting in improved battery performance.

NANOTECHNOLOGY (2021)

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Review Materials Science, Multidisciplinary

Recent advances in carbonized non-noble metal-organic frameworks for electrochemical catalyst of oxygen reduction reaction

Chan Li et al.

Summary: This review systematically summarizes recent developments on non-noble metal ORR catalysts prepared by carbonization of various MOFs and discusses the effects of synthesis strategies and pyrolysis conditions on the catalyst properties.

RARE METALS (2021)

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Review Chemistry, Physical

Dopants in the Design of Noble Metal Nanoparticle Electrocatalysts and their Effect on Surface Energy and Coordination Chemistry at the Nanocrystal Surface

Taehyun Kwon et al.

Summary: This review discusses the versatility of dopants in nanoparticle-based catalysis, showing how doping can enhance catalytic activity and selectivity by modulating band structure, optimizing surface energy, and controlling binding strength of adsorbates. Additionally, dopants can also influence nanocrystal growth mechanisms, leading to shape- and phase-controlled nanocrystals.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Physical

Electronic tuning of confined sub-nanometer cobalt oxide clusters boosting oxygen catalysis and rechargeable Zn-air batteries

Yangyang Tan et al.

Summary: This study predicted the electronic structure regulation of cobalt oxide nanoclusters using DFT simulation, and experimentally verified the enhancement of bifunctional oxygen performance through microporous MOFs confinement strategy. The optimized catalyst demonstrated outstanding performance in rechargeable Zn-air batteries, outperforming benchmark electrodes. DFT calculations showed that reducing particle size and coupling with Co-N can effectively regulate the charge distribution of CoOx nanoclusters and accelerate the overall ORR/OER kinetic process.

NANO ENERGY (2021)

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Article Chemistry, Multidisciplinary

Anchoring Single Copper Atoms to Microporous Carbon Spheres as High-Performance Electrocatalyst for Oxygen Reduction Reaction

Lingbo Zong et al.

Summary: This study reports a method of anchoring transition metal single atoms on carbon support by creating defects and vacancies, resulting in electrocatalysts with superior oxygen reduction reaction catalytic activity. Among them, Cu-SAs@N-CNS exhibits excellent bifunctional activity for oxygen reduction and oxygen evolution reactions, and is successfully used as an efficient air cathode material for zinc-air batteries; the study suggests that N-terminated vacancies on graphitic carbons are the preferred sites for anchoring Cu single atoms.

ADVANCED FUNCTIONAL MATERIALS (2021)

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Article Biochemical Research Methods

Photo-induced green synthesis of bimetallic Ag/Pd nanoparticles decorated reduced graphene oxide/nitrogen-doped graphene quantum dots nanocomposite as an amperometric sensor for nitrite detection

Alireza Tajiki et al.

Summary: This study successfully prepared a novel nanocomposite based on reduced graphene oxide, nitrogen-doped graphene quantum dots, and palladium and silver nanoparticles for nitrite oxidation reaction as an electrocatalyst. The efficiency of the prepared sensing platform on the surface of a gold working electrode was evaluated through various electrochemical tests, showing high sensitivity and low detection limit for nitrite ions. The proposed sensor was effectively applied for the determination of nitrite ions in river and mineral water samples as natural water sources.

ANALYTICAL AND BIOANALYTICAL CHEMISTRY (2021)

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Article Chemistry, Physical

Cactus-like NiCo2S4@NiFe LDH hollow spheres as an effective oxygen bifunctional electrocatalyst in alkaline solution

Xueting Feng et al.

Summary: The study introduces a novel cactus-like NiCo2S4@NiFe LDH hollow sphere prepared by a hydrothermal method, which effectively enhances the catalytic activities for oxygen reduction reaction (ORR) and oxygen evolution reaction (OER), demonstrating stability in long-term tests and achieving a small potential gap.

APPLIED CATALYSIS B-ENVIRONMENTAL (2021)

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Article Chemistry, Physical

Electrostatic spun hierarchically porous carbon matrix with CoSe2/Co heterostructure as bifunctional electrocatalysts for zinc-air batteries

Junfeng Huang et al.

Summary: A N-doped carbon matrix with CoSe2/Co heterostructures was fabricated using a four-step method, showing excellent bifunctional electrocatalytic performance. The optimized CoSe2/Co@NCNF-3 exhibited outstanding ORR and OER performance, long-term stability, and resistance to methanol. The heterostructure also demonstrated enhanced intermediate adsorption ability and catalytic capacity for OER, leading to high performance in zinc-air battery applications.

JOURNAL OF ALLOYS AND COMPOUNDS (2021)

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Review Materials Science, Multidisciplinary

Metal-free carbon based air electrodes for Zn-air batteries: Recent advances and perspective

Yasir Arafat et al.

Summary: This review summarizes the recent progress in utilizing metal-free carbon materials as air electrodes in Zn-air batteries (ZABs), highlighting the two main methods to enhance the catalytic performance for oxygen reduction and oxygen evolution reactions. The article also discusses the latest challenges and future opportunities associated with metal-free carbon materials as air electrodes in ZABs.

MATERIALS RESEARCH BULLETIN (2021)

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Article Nanoscience & Nanotechnology

Synergizing metal-support interactions and spatial confinement boosts dynamics of atomic nickel for hydrogenations

Jian Gu et al.

Summary: The synergistic effect of metal-support interactions and spatial confinement enhances the catalytic performance of highly loaded atomic nickel on a graphitic carbon nitride support, leading to improved coke inhibition and outstanding activity in hydrogenation reactions. This approach provides a pathway to design efficient, stable, and highly loaded atomically dispersed catalysts with superior catalytic performance compared to traditional metal nanoparticles.

NATURE NANOTECHNOLOGY (2021)

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Review Chemistry, Multidisciplinary

Advanced Transition Metal-Based OER Electrocatalysts: Current Status, Opportunities, and Challenges

Kexin Zhang et al.

Summary: Oxygen evolution reaction (OER) is crucial in electrochemical applications like water splitting and rechargeable metal-air batteries, but its slow kinetics presents a performance bottleneck. Therefore, rational design of OER electrocatalysts based on understanding mechanisms and structure-activity relationship is essential. Study of reaction pathways, intermediates, and descriptors can lead to more efficient design of transition metal-based OER electrocatalysts.

SMALL (2021)

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Review Chemistry, Multidisciplinary

Structural Design Strategy and Active Site Regulation of High-Efficient Bifunctional Oxygen Reaction Electrocatalysts for Zn-Air Battery

Xu Liu et al.

Summary: This review discusses the crucial oxygen reduction reaction (ORR) and oxygen evolution reaction (OER) mechanisms in zinc-air batteries (ZABs) and the importance of developing efficient and stable bifunctional ORR/OER catalysts to enhance ZAB performance. Additionally, it summarizes the improvements in energy efficiency, stability, and environmental adaptability of ZAB by introducing additional reactions and altering the OER pathway.

SMALL (2021)

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Review Chemistry, Multidisciplinary

Development of Perovskite Oxide-Based Electrocatalysts for Oxygen Evolution Reaction

Dong Liu et al.

Summary: Perovskite oxides are studied as electrocatalysts for oxygen evolution reactions due to their low cost, customizable structure, high stability, and good catalytic activity. Two main challenges for efficient OER performance are limited active sites and low electrical conductivity, which can be overcome by strategies such as composition engineering, crystal facet control, morphology modulation, defect engineering, and hybridization. The review comprehensively summarizes recent developments in enhancing catalytic activities of perovskite oxide-based electrocatalysts for practical applications in OER.

SMALL (2021)

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Article Chemistry, Physical

Ultrahigh-Rate and Long-Life Zinc-Metal Anodes Enabled by Self-Accelerated Cation Migration

Peichao Zou et al.

Summary: A novel ferroelectric polymer-inorganic composite thin film coating is proposed for aqueous zinc ion batteries, which can enhance the reversibility of zinc metal anodes, increase the cumulative plating capacity, and achieve a compact and horizontally-aligned zinc morphology even at ultrahigh rates. This work provides new insights into stabilizing zinc metal electrodeposition at the scale of interfacial ion diffusion.

ADVANCED ENERGY MATERIALS (2021)

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Article Chemistry, Multidisciplinary

Advanced Trifunctional Electrocatalysis with Cu-, N-, S-Doped Defect-Rich Porous Carbon for Rechargeable Zn-Air Batteries and Self-Driven Water Splitting

Mingwen Wang et al.

Summary: This study presents a new type of porous carbon doped with Cu, N, S as a trifunctional catalyst, which exhibits excellent electrocatalytic performance and stability for the ORR, OER, and HER reactions, surpassing noble metals in certain aspects. The catalyst shows promising potential for applications in Zn-air batteries and overall water splitting, demonstrating superior performance. The synthesis method offers opportunities for new catalyst design and discovery, enabling versatile and robust energy applications.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2021)

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Article Chemistry, Multidisciplinary

Photochemical reduction of nanocrystalline maghemite to magnetite

Hankyeol Jung et al.

Summary: The study introduces a method for photochemical conversion of inverse spinel iron oxides to mixed-valent magnetite phase with controlled Fe2+ composition. Through UV irradiation and sacrificial reductants, topotactic reduction of nanocrystals to form Fe3O4 can be achieved, resulting in increased magnetization and characteristic magnetic features.

NANOSCALE (2021)

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Article Chemistry, Physical

Origin of the hydrophobicity of sulfur-containing iron surfaces

Hao Li et al.

Summary: This study examines the hydrophobicity of sulfur-containing iron materials through molecular dynamics simulation, revealing that the hydrophobic nature of sulfur plays a key role in enhancing surface hydrophobicity. Experimental analysis confirms the theoretical findings, and it is also suggested that doping other p-block elements can induce a similar hydrophobic phenomenon on iron surfaces. This study highlights the importance of considering hydrophobicity in mechanistic analysis of liquid-phase reaction materials.

PHYSICAL CHEMISTRY CHEMICAL PHYSICS (2021)

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Review Chemistry, Multidisciplinary

Transition metal-based bimetallic MOFs and MOF-derived catalysts for electrochemical oxygen evolution reaction

Songsong Li et al.

Summary: Transition metal-based bimetallic MOFs show superior performance and stability in the oxygen evolution reaction, offering potential for enhancing efficiency in clean-energy production and energy storage. They can also serve as precursors for obtaining high surface area carbon materials or metal compounds, thereby improving catalytic activity.

ENERGY & ENVIRONMENTAL SCIENCE (2021)

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Article Chemistry, Multidisciplinary

3D porous Ni/NiOx as a bifunctional oxygen electrocatalyst derived from freeze-dried Ni(OH)2

Yuta Shudo et al.

Summary: The bifunctional electrocatalytic properties of freeze-dried Ni/NiOx, NiO, and Ni(OH)2 were studied, showing promising performance for a wide range of applications without the need for carbon support. The freeze-dried Ni/NiOx exhibited excellent bifunctional catalytic activities and could be a potential alternative to expensive benchmark catalysts for various electrocatalytic applications.

NANOSCALE (2021)

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Review Materials Science, Multidisciplinary

Recent advances in the field of carbon-based cathode electrocatalysts for Zn-air batteries

Xinxin Shu et al.

Summary: Carbon-based catalysts are highly regarded for energy storage and conversion technologies due to their high electrical conductivity and tunable micro- and nanostructures, but developing efficient, low-cost, and durable bifunctional carbon-based electrocatalysts remains a challenge. Recent research has focused on fabrication strategies for carbon-based oxygen reduction reaction/oxygen evolution reaction electrocatalysts for Zn-air batteries, outlining the current challenges and perspectives in developing advanced bifunctional carbon-based electrocatalysts.

MATERIALS ADVANCES (2021)

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Article Chemistry, Physical

Engineering the electronic states of Ni3FeN via zinc ion regulation for promoting oxygen electrocatalysis in rechargeable Zn-air batteries

Xiaoyang He et al.

Summary: This study developed a highly efficient Zn-doped Ni3FeN/nitrogen-doped graphene (Zn-Ni3FeN/NG) bifunctional electrocatalyst, which showed remarkable electrochemical activity and stability due to the lattice distortion stress caused by the Zn dopant. The Zn-Ni3FeN/NG also exhibited a high-power density in Zn-air batteries compared to commercial materials, offering a facile strategy for designing efficient oxygen bifunctional electrocatalysts.

JOURNAL OF MATERIALS CHEMISTRY A (2021)

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Article Chemistry, Multidisciplinary

Co0.7Fe0.3 NPs confined in yolk-shell N-doped carbon: engineering multi-beaded fibers as an efficient bifunctional electrocatalyst for Zn-air batteries

Ling Long et al.

Summary: This study developed a bifunctional electrocatalyst consisting of Co0.7Fe0.3 alloy nanoparticles confined in N-doped carbon with a yolk-shell structure in multi-beaded fibers, exhibiting excellent OER and ORR performance. The hierarchical structure with abundant mesopores, high BET surface area, good electronic conductivity, and uniformly distributed active sites showed superior electrochemical performance compared to commercial catalysts. The Co0.7Fe0.3@NC2:1-800 Zn-air battery displayed higher open circuit voltage, larger power density, and better cycling stability, suggesting potential applications in energy conversion systems.

NANOSCALE (2021)

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Article Chemistry, Multidisciplinary

Transition-metal single atoms embedded into defective BC3 as efficient electrocatalysts for oxygen evolution and reduction reactions

Yanan Zhou et al.

Summary: Finding high-activity, stable, and low-cost catalysts for the oxygen evolution reaction (OER) and oxygen reduction reaction (ORR) is crucial for the development of renewable energy technologies. Using computational screening based on density functional theory, it was found that transition metal atoms doped on defective BC3 monolayers exhibit efficient catalytic properties for OER and ORR. The study highlights the potential of single atom catalysts based on carbon materials for efficient and stable catalytic activity.

NANOSCALE (2021)

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Review Chemistry, Multidisciplinary

Synergistically Interactive Pyridinic-N-MoP Sites: Identified Active Centers for Enhanced Hydrogen Evolution in Alkaline Solution

Di Zhao et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Article Chemistry, Physical

Multi-component nanoporous alloy/(oxy)hydroxide for bifunctional oxygen electrocatalysis and rechargeable Zn-air batteries

Gang Fang et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Physical

Enhanced cathodic catalytic activity of an N-doped micropore structure obtained through the six-coordinate bond of an EDTA-Ce composite for the oxygen reduction reaction

Kwanwoo Kim et al.

APPLIED SURFACE SCIENCE (2020)

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Article Chemistry, Multidisciplinary

In Situ Induction of Strain in Iron Phosphide (FeP2) Catalyst for Enhanced Hydroxide Adsorption and Water Oxidation

Guowei Li et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Review Chemistry, Multidisciplinary

Non-Noble-Metal-Based Electrocatalysts toward the Oxygen Evolution Reaction

Zhi-Peng Wu et al.

ADVANCED FUNCTIONAL MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Manipulating Layered P2@P3 Integrated Spinel Structure Evolution for High-Performance Sodium-Ion Batteries

Yan-Fang Zhu et al.

ANGEWANDTE CHEMIE-INTERNATIONAL EDITION (2020)

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Review Chemistry, Multidisciplinary

Well-Defined Materials for Heterogeneous Catalysis: From Nanoparticles to Isolated Single-Atom Sites

Zhi Li et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Boosting Oxygen Reduction of Single Iron Active Sites via Geometric and Electronic Engineering: Nitrogen and Phosphorus Dual Coordination

Kai Yuan et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2020)

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Article Chemistry, Multidisciplinary

Atomic-Level Fe-N-C Coupled with Fe3C-Fe Nanocomposites in Carbon Matrixes as High-Efficiency Bifunctional Oxygen Catalysts

Xueping Sun et al.

SMALL (2020)

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Article Multidisciplinary Sciences

Electrochemical deposition as a universal route for fabricating single-atom catalysts

Zhirong Zhang et al.

NATURE COMMUNICATIONS (2020)

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Review Chemistry, Physical

A Critical Review of Machine Learning of Energy Materials

Chi Chen et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Nanoscience & Nanotechnology

Trifunctional Electrocatalysts with High Efficiency for the Oxygen Reduction Reaction, Oxygen Evolution Reaction, and Na-O2 Battery in Heteroatom-Doped Janus Monolayer MoSSe

Qian Wu et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Multidisciplinary

Interfacial Engineering of MoO2-FeP Heterojunction for Highly Efficient Hydrogen Evolution Coupled with Biomass Electrooxidation

Ganceng Yang et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Sulfur Loading and Speciation Control the Hydrophobicity, Electron Transfer, Reactivity, and Selectivity of Sulfidized Nanoscale Zerovalent Iron

Jiang Xu et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Multidisciplinary

Identifying Dense NiSe2/CoSe2 Heterointerfaces Coupled with Surface High-Valence Bimetallic Sites for Synergistically Enhanced Oxygen Electrocatalysis

Xuerong Zheng et al.

ADVANCED MATERIALS (2020)

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Article Chemistry, Physical

Holey graphitic carbon nitride (g-CN) supported bifunctional single atom electrocatalysts for highly efficient overall water splitting

Xingshuai Lv et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Physical

Highly efficient water splitting driven by zinc-air batteries with a single catalyst incorporating rich active species

Hao Sun et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Review Chemistry, Multidisciplinary

Chemical Synthesis of Single Atomic Site Catalysts

Shufang Ji et al.

CHEMICAL REVIEWS (2020)

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Article Chemistry, Multidisciplinary

Enhancing bifunctionality of CoN nanowires by Mn doping for long-lasting Zn-air batteries

Yongqi Zhang et al.

SCIENCE CHINA-CHEMISTRY (2020)

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Article Chemistry, Physical

Mesoporous Single-Atom-Doped Graphene-Carbon Nanotube Hybrid: Synthesis and Tunable Electrocatalytic Activity for Oxygen Evolution and Reduction Reactions

Mohammad Tavakkoli et al.

ACS CATALYSIS (2020)

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Review Chemistry, Physical

Modulating the local coordination environment of single-atom catalysts for enhanced catalytic performance

Xinyuan Li et al.

NANO RESEARCH (2020)

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Article Nanoscience & Nanotechnology

Exploiting a High-Performance Double-Carbon Structure Co9S8/GN Bifunctional Catalysts for Rechargeable Zn-Air Batteries

Xiaoling Sun et al.

ACS APPLIED MATERIALS & INTERFACES (2020)

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Article Chemistry, Physical

CoOx/CoNy nanoparticles encapsulated carbon-nitride nanosheets as an efficiently trifunctional electrocatalyst for overall water splitting and Zn-air battery

Jiameng Liu et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Physical

Densely colonized isolated Cu-N single sites for efficient bifunctional electrocatalysts and rechargeable advanced Zn-air batteries

Nayantara K. Wagh et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2020)

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Article Chemistry, Inorganic & Nuclear

Cu powder decorated 3D Mn-MOF with excellent electrochemical properties for supercapacitors

Ping-Ping Sun et al.

INORGANICA CHIMICA ACTA (2020)

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Article Energy & Fuels

Highly durable carbon supportedFe-Nnanocrystals feature as efficient bi-functional oxygen electrocatalyst

Narayanamoorthy Bhuvanendran et al.

INTERNATIONAL JOURNAL OF ENERGY RESEARCH (2020)

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Article Chemistry, Physical

Lanthanum doped copper oxide nanoparticles enabled proficient bi-functional electrocatalyst for overall water splitting

John D. Rodney et al.

INTERNATIONAL JOURNAL OF HYDROGEN ENERGY (2020)

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Review Chemistry, Physical

Aqueous metal-air batteries: Fundamentals and applications

Qianfeng Liu et al.

ENERGY STORAGE MATERIALS (2020)

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Article Chemistry, Physical

3D N, S-co-doped carbon nanotubes/graphene/MnS ternary hybrid derived from Hummers' method for highly efficient oxygen reduction reaction

Yangyang Chen et al.

MATERIALS TODAY ENERGY (2020)

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Article Chemistry, Multidisciplinary

Efficient Bifunctional Catalytic Electrodes with Uniformly Distributed NiN2Active Sites and Channels for Long-Lasting Rechargeable Zinc-Air Batteries

Zihe Cai et al.

SMALL (2020)

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Article Chemistry, Applied

N -doped porous carbon hollow microspheres encapsulated with iron -based nanocomposites as advanced bifunctional catalysts for rechargeable Zn-air battery

Ran Hao et al.

JOURNAL OF ENERGY CHEMISTRY (2020)

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Article Green & Sustainable Science & Technology

Rational design of sustainable transition metal-based bifunctional electrocatalysts for oxygen reduction and evolution reactions

Yuhui Tian et al.

SUSTAINABLE MATERIALS AND TECHNOLOGIES (2020)

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Article Electrochemistry

Bifunctional α-MnO2 and Co3O4 Catalyst for Oxygen Electrocatalysis in Alkaline Solution

Michael F. Fink et al.

CHEMELECTROCHEM (2020)

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Review Materials Science, Multidisciplinary

Recent Advances on the Modulation of Electrocatalysts Based on Transition Metal Nitrides for the Rechargeable Zn-Air Battery

Xinxin Yu et al.

ACS MATERIALS LETTERS (2020)

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Review Chemistry, Physical

Recent Advances in the Development of Single-Atom Catalysts for Oxygen Electrocatalysis and Zinc-Air Batteries

Lishan Peng et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Physical

Atomically Dispersed Cobalt Trifunctional Electrocatalysts with Tailored Coordination Environment for Flexible Rechargeable Zn-Air Battery and Self-Driven Water Splitting

Zheye Zhang et al.

ADVANCED ENERGY MATERIALS (2020)

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Article Chemistry, Physical

Integrating PtNi nanoparticles on NiFe layered double hydroxide nanosheets as a bifunctional catalyst for hybrid sodium-air batteries

Xueqing Yu et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Chemistry, Multidisciplinary

A facile approach to high-performance trifunctional electrocatalysts by substrate-enhanced electroless deposition of Pt/NiO/Ni on carbon nanotubes

Yaru Bian et al.

NANOSCALE (2020)

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Article Chemistry, Physical

A bimetallic alloy anchored on biomass-derived porous N-doped carbon fibers as a self-supporting bifunctional oxygen electrocatalyst for flexible Zn-air batteries

Yanli Niu et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Review Chemistry, Multidisciplinary

A review on fundamentals for designing oxygen evolution electrocatalysts

Jiajia Song et al.

CHEMICAL SOCIETY REVIEWS (2020)

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Article Chemistry, Physical

Directly predicting limiting potentials from easily obtainable physical properties of graphene-supported single-atom electrocatalysts by machine learning

Shiru Lin et al.

JOURNAL OF MATERIALS CHEMISTRY A (2020)

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Article Chemistry, Multidisciplinary

Bamboo-like nitrogen-doped porous carbon nanofibers encapsulated nickel-cobalt alloy nanoparticles composite material derived from the electrospun fiber of a bimetal-organic framework as efficient bifunctional oxygen electrocatalysts

Chao Feng et al.

NANOSCALE (2020)

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Article Chemistry, Multidisciplinary

Co5.47N loaded N-doped carbon as an efficient bifunctional oxygen electrocatalyst for a Zn-air battery

Zichao Rong et al.

NANOSCALE (2020)

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Review Chemistry, Multidisciplinary

Surface/interface nanoengineering for rechargeable Zn-air batteries

Tianpei Zhou et al.

ENERGY & ENVIRONMENTAL SCIENCE (2020)

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Article Chemistry, Physical

Promoting electrocatalytic overall water splitting with nanohybrid of transition metal nitride-oxynitride

Soumen Dutta et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2019)

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Article Electrochemistry

N-doped mesoporous FeNx/carbon as ORR and OER bifunctional electrocatalyst for rechargeable zinc-air batteries

Jieting Ding et al.

ELECTROCHIMICA ACTA (2019)

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Article Chemistry, Physical

2D transition metal-TCNQ sheets as bifunctional single-atom catalysts for oxygen reduction and evolution reaction (ORR/OER)

Qingming Deng et al.

JOURNAL OF CATALYSIS (2019)

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Article Multidisciplinary Sciences

Cascade anchoring strategy for general mass production of high-loading single-atomic metal-nitrogen catalysts

Lu Zhao et al.

NATURE COMMUNICATIONS (2019)

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Article Chemistry, Physical

Efficient quantum dots anchored nanocomposite for highly active ORR/OER electrocatalyst of advanced metal-air batteries

Nengneng Xu et al.

NANO ENERGY (2019)

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Article Chemistry, Multidisciplinary

Hierarchical Co3O4 Nano-Micro Arrays Featuring Superior Activity as Cathode in a Flexible and Rechargeable Zinc-Air Battery

Yaotang Zhong et al.

ADVANCED SCIENCE (2019)

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Article Chemistry, Multidisciplinary

Ship in a Bottle Design of Highly Efficient Bifunctional Electrocatalysts for Long-Lasting Rechargeable Zn-Air Batteries

Zhen Zhang et al.

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The Role of Anions in Metal Chalcogenide Oxygen Evolution Catalysis: Electrodeposited Thin Films of Nickel Sulfide as Pre-catalysts

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Hollow-Structured Carbon-Supported Nickel Cobaltite Nanoparticles as an Efficient Bifunctional Electrocatalyst for the Oxygen Reduction and Evolution Reactions

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A Co/metal-organic-framework bifunctional electrocatalyst: The effect of the surface cobalt oxidation state on oxygen evolution/reduction reactions in an alkaline electrolyte

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High-Loading Cobalt Oxide Coupled with Nitrogen-Doped Graphene for Oxygen Reduction in Anion-Exchange-Membrane Alkaline Fuel Cells

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Co3O4 nanocrystals on graphene as a synergistic catalyst for oxygen reduction reaction

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Metal-Air Batteries with High Energy Density: Li-Air versus Zn-Air

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Electrocatalysis of oxygen reduction and small alcohol oxidation in alkaline media

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Perovskite thin films deposited by pulsed laser ablation as model systems for electrochemical applications

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Towards complete cofactor arrangement in the 3.0 Å resolution structure of photosystem II

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Origin of the overpotential for oxygen reduction at a fuel-cell cathode

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Crystal structure of photosystem II from Synechococcus elongatus at 3.8 Å resolution

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RRDE study of oxygen reduction on Pt nanoparticles inside Nafion®:: H2O2 production in PEMFC cathode conditions

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