期刊
PHYSICS LETTERS A
卷 479, 期 -, 页码 -出版社
ELSEVIER
DOI: 10.1016/j.physleta.2023.128920
关键词
Rashba spin splitting; Intrinsic spin -polarization; First -principles calculation; Na(Cs); Au; Si(111) surface
The Rashba spin splitting of monovalent alkali metal adsorbed on Au/Si(111) surface is explained using first-principles calculations and analyses. It is found that Na adatom donates one electron to the pristine surface, leading to a large Rashba spin splitting in Na/Au/Si(111) system. Cs adsorbate, with larger intra-atomic spin-orbit coupling, not only plays the same role as Na adatom but also induces intrinsic spin-polarization, further enhancing the Rashba spin splitting on the Cs/Au/Si(111) surface. The proposed mechanism of intrinsic spin-polarization significantly enhancing the Rashba spin splitting is generally applicable and can be extended to alkali-earth metal epitaxial layers on Au/Si(111) surface.
Adsorbed/modified surface is usually treated as a prototype to study Rashba spin splitting. Using first -principles calculations and analyses, we first explain the Rashba spin splitting of monovalent alkali metal adsorbed on Au/Si(111) surface as realized in experiment. We clearly identify that Na adatom donates one electron to pristine Au/Si(111) surface, leading to the Fermi level shift upward to the parabolic range of Au d and Si p hybridized states and thus leading to large Rashba spin splitting in Na/Au/Si(111) system. However, for the larger intra-atomic spin-orbit coupling Cs adsorbate, it not only plays the identical role to Na adatom, but induces intrinsic spin-polarization surprisingly, which further enhances the Rashba spin splitting on the Cs/Au/Si(111) surface up to-200 meV. Our proposed mechanism that intrinsic spin -polarization significantly enhancing the Rashba spin splitting is generally applicable and can be extended readily to alkali-earth metal as epitaxial layer grown on Au/Si(111) surface.& COPY; 2023 Elsevier B.V. All rights reserved.
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