4.4 Article

Development of a 4n detection system for the measurement of the shape of β spectra

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DOI: 10.1016/j.nima.2023.168354

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14C beta spectrum; 204Tl beta spectrum; Si detectors; 4n detection; Experimental shape factor; Monte Carlo simulation

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A specific detection system was developed to meet the need for precise measurements of the energy distribution of emitted beta particles. An ultra-thin radioactive source was used in a compact geometry between two silicon detectors, with a quasi-4n sr solid angle. Distortions were corrected using a dedicated deconvolution process based on mono-energetic Monte Carlo simulations. The measurements and analysis of beta spectra from 14C and 204Tl decays showed consistent results with recommended Q-values and theoretical predictions.
The need of precise measurements of the energy distribution of emitted beta particles has been addressed developing a specific detection system. An ultra-thin radioactive source, prepared on purpose, is enclosed between two silicon detectors in a compact geometry with a quasi-4n sr solid angle. The remaining distortions have been corrected with a dedicated deconvolution process based on mono-energetic Monte Carlo simulations that are used to build the response matrix. The beta spectra from 14C and 204Tl decays have been measured and analyzed. Extracted maximum energies are fully consistent with the AME2020 recommended Q-values. A linear slope of a = -0.430 (37) MeV-1 that comes from the weak magnetism term in the 14C beta spectrum has been determined, in excellent agreement with the theoretical predictions. The measured range of the 204Tl beta spectrum has been extended down to 60 keV and a shape factor (d q2 + A2p2) has been extracted with d = 1.075 (13).

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