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Article
Multidisciplinary Sciences
Hao Chen et al.
Summary: The open-circuit voltage deficit in wide-bandgap perovskite solar cells is larger than in perovskites with a bandgap of approximately 1.5 eV. The limiting factor for the open-circuit voltage is found to be recombination at the electron-transport-layer contact, resulting from inhomogeneous surface potential and poor energetic alignment. To address this issue, a new surface treatment using diammonium molecules is introduced to achieve a more uniform distribution of surface potential.
Review
Nanoscience & Nanotechnology
Furkan H. Isikgor et al.
Summary: Metal-oxide-based charge-transport layers are crucial for the development of perovskite solar cells, but the metal-oxide/perovskite interfaces often have defects that hinder charge transfer and cause non-radiative recombination. This review explores the challenges associated with these interfaces and proposes solutions using molecular engineering, such as self-assembled monolayers, to improve their performance and commercial viability.
NATURE REVIEWS MATERIALS
(2023)
Review
Chemistry, Physical
Weiguang Chi et al.
Summary: In recent years, there has been intensive research on perovskite/silicon tandem solar cells, leading to a rapid increase in their efficiencies. The most suitable subcell for tandem devices is a debatable topic, and this study summarizes three attractive silicon solar cells: passivated-emitter rear-cell (PERC), tunnel oxide passivated contact (TOPCon), and heterojunction (HJT) cells. Their structures and features are elucidated to understand their mechanism and potential for optimum performance. Furthermore, the characteristics and performance of perovskite/silicon tandem cells with these subcells are compared and discussed, with emphasis on the contribution of passivation layer and structure design on both sides. The recombination layer between the two subcells is also analyzed in depth, considering material chemistry, light absorption, and charge transport for achieving an optimized structure.
ACS ENERGY LETTERS
(2023)
Article
Chemistry, Multidisciplinary
Michele De Bastiani et al.
Summary: Textured silicon wafers and monolithic perovskite/silicon tandem solar cells both have superior light trapping capability, but the complex silicon surfaces may affect the structural and optoelectronic properties of the overlying perovskite films. Extensive characterization reveals that the main effect of the substrate morphology lies in altering the photoluminescence response of the perovskite, which is associated with thickness variations rather than lattice strain or composition changes. This understanding rationalizes the design of high-performance perovskite/silicon tandems, achieving certified power conversion efficiencies of >28%.
ADVANCED FUNCTIONAL MATERIALS
(2023)
Article
Chemistry, Multidisciplinary
Xin Luo et al.
Summary: An anion-engineered additive strategy is developed to control the crystallization process of wide-bandgap perovskite films on industrially textured silicon, resulting in improved film crystallinity and reduced trap density. This strategy enables the fabrication of 28.6%-efficient perovskite/silicon tandem solar cells, which retain over 80% of their initial performance after 2000 hours of operation under full 1-sun illumination.
ADVANCED MATERIALS
(2023)
Article
Multidisciplinary Sciences
Silvia Mariotti et al.
Summary: To improve the stability and efficiency of perovskite-silicon tandem solar cells, reductions in recombination losses are necessary. This was achieved by combining a triple-halide perovskite with a piperazinium iodide interfacial modification, resulting in improved band alignment, reduced nonradiative recombination losses, and enhanced charge extraction. The tandem solar cells achieved high open-circuit voltages and certified power conversion efficiencies of up to 32.5%.
Article
Multidisciplinary Sciences
Xin Yu Chin et al.
Summary: Silicon solar cells are reaching their efficiency limit of 29%, but this can be surpassed by using advanced device structures. In this study, we created a tandem device with a perovskite layer on top of a silicon bottom cell to enhance the photocurrent. By regulating the perovskite crystallization process and reducing recombination losses, we achieved a certified power conversion efficiency of 31.25% with an active area of 1.17 square centimeters.
Article
Multidisciplinary Sciences
Hao Chen et al.
Summary: The open-circuit voltage (V-OC) deficit in perovskite solar cells is attributed to the poor alignment of surface potential and energetic levels. Introducing diammonium molecules for surface treatment can enhance the quasi-Fermi-level splitting and achieve high efficiency in perovskite solar cells.
Article
Nanoscience & Nanotechnology
Nga Phung et al.
Summary: Metal halide perovskites have excellent electronic properties, and recent advancements in device performance and stability of perovskite solar cells have been achieved with the application of self-assembled monolayers (SAMs). By introducing an intermediate layer of NiO between ITO and SAM, the coverage and homogeneity of SAMs on the substrate can be improved, leading to enhanced device performance. The combination of NiO and SAM results in a more than 20% efficient champion device with a narrower distribution of performance.
ACS APPLIED MATERIALS & INTERFACES
(2022)
Article
Chemistry, Physical
Gaurav Kapil et al.
Summary: According to research, the power conversion efficiency of tin-lead perovskite solar cells can be improved by using specific hole transport layers. By using substances such as 2PACz and MPA, comparable performance to traditional PEDOT:PSS can be achieved. Experimental results showed that coabsorption of 2PACz and MPA on the transparent conducting oxide layer can further enhance the performance of tin-lead perovskite solar cells.
ACS ENERGY LETTERS
(2022)
Article
Energy & Fuels
Wei Chen et al.
Summary: Perovskite/organic tandem solar cells have a promising future in thin-film photovoltaics due to the large chemical composition and tunability of their bandgap. However, their efficiency is currently limited by the open-circuit voltage loss and non-ideal interconnecting layers. In this study, the passivation of nickel oxide hole-transporting layers and the development of an optimized interconnecting layer structure led to a significant increase in efficiency, reaching a maximum of 23.60% (22.95% certified) in perovskite/organic tandem solar cells.
Article
Physics, Applied
Ryota Mishima et al.
Summary: A certified 28.3% efficient monolithic perovskite-silicon tandem solar cell with a mixed self-assembled monolayer (SAM) is reported. The improvement in fill factors in the PST cells can be attributed to the passivation qualities and local interaction between methoxy ligands and perovskite materials.
APPLIED PHYSICS EXPRESS
(2022)
Article
Multidisciplinary Sciences
K. O. Brinkmann et al.
Summary: Multijunction solar cells can surpass the efficiency limits of single-junction devices. Metal halide perovskite solar cells, in combination with silicon and copper indium gallium selenide (CIGS) or as all-perovskite tandems, have shown promising results. Narrow-gap non-fullerene acceptors have also significantly improved the efficiencies of organic solar cells. In this study, perovskite-organic tandem cells with high efficiency and voltage are demonstrated, utilizing optimized charge extraction layers and an ultrathin metal-like indium oxide layer for interconnection. This milestone work outperforms the best perovskite single junctions and is comparable to perovskite-CIGS and all-perovskite multijunctions.
Article
Multidisciplinary Sciences
Shaun Tan et al.
Summary: Optoelectronic devices rely on heterointerfaces between different semiconducting materials, and the energy-level alignment between them plays a crucial role in device performance. Surface treatments for perovskite solar cells can impact the energetics of the heterointerface, potentially affecting device stability. Balancing the pros and cons of surface treatments is essential for improving PSC stability.
Review
Nanoscience & Nanotechnology
Christophe Ballif et al.
Summary: This paper reviews the recent evolution of crystalline silicon solar cells, analyzes the current status of research and industrial development, and looks into the future prospects. The improvements in materials and processing have greatly reduced the cost and increased the efficiency of crystalline silicon photovoltaics, making it an important low-cost source of electricity. The paper also discusses the challenges and requirements for other photovoltaic technologies to compete with silicon on the mass market.
NATURE REVIEWS MATERIALS
(2022)
Article
Energy & Fuels
Andreas Fell et al.
Summary: This article presents an efficient 3-D tandem modeling approach implemented in a solar cell simulation software, which helps in understanding and quantifying the influence of various effects on tandem cell development. The usefulness of this approach is demonstrated by investigating perimeter designs of small-area silicon-perovskite cells.
IEEE JOURNAL OF PHOTOVOLTAICS
(2022)
Article
Multidisciplinary Sciences
Jiang Liu et al.
Summary: The performance of perovskite solar cells with inverted polarity can be improved by adding a MgFx interlayer at the perovskite/C-60 interface. This interlayer facilitates efficient electron extraction, reduces nonradiative recombination, and exhibits good stability under damp-heat conditions.
Editorial Material
Chemistry, Physical
Kari Sveinbjoernsson et al.
Summary: A monolithic two-terminal perovskite/silicon tandem solar cell was fabricated based on an industrial silicon bottom cell with mass-production feasible processes, showing a steady-state power conversion efficiency of 28.7% and an open-circuit voltage of over 1.9 V.
ACS ENERGY LETTERS
(2022)
Article
Multidisciplinary Sciences
Qi Jiang et al.
Summary: In this study, a reactive surface engineering approach was used to enhance the performance of perovskite solar cells with an inverted structure. The resulting p-i-n solar cells showed a high power conversion efficiency of over 25% and remained stable after long-term operation under extreme conditions.
Article
Nanoscience & Nanotechnology
Philipp Tockhorn et al.
Summary: Gentle sinusoidal nanotextures were designed to achieve high-efficiency perovskite-silicon solar cells, offering advantages such as reduced reflection losses, increased fabrication yield, and improved open-circuit voltage.
NATURE NANOTECHNOLOGY
(2022)
Article
Chemistry, Physical
Elizabeth M. Tennyson et al.
Summary: This study characterizes the microscale optoelectronic properties of Halide perovskite/crystalline silicon (c-Si) tandem solar cells, revealing a strong spatial and spectral dependence of the photoluminescence (PL) response on the texturing design. A holistic optimization of the texturing is required to maximize light in- and out-coupling, balancing the optimal geometrical configuration and optoelectronic performance for future device designs.
ACS ENERGY LETTERS
(2021)
Article
Chemistry, Multidisciplinary
Yuchao Zhang et al.
Summary: To significantly impact climate change, the annual production of photovoltaic (PV) modules must increase dramatically to around 3 terawatts (TW) by 2030. However, existing and future commercial PV cell technologies face sustainable manufacturing capacity limitations due to scarce metals, necessitating significant material consumption reductions for sustainable multi-TW scale manufacturing.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
Article
Chemistry, Multidisciplinary
Erkan Aydin et al.
Summary: By developing new contact materials, the research team successfully converted high-efficiency single-junction perovskite solar cells into efficient perovskite/silicon tandem solar cells, achieving a conversion efficiency of up to 27%.
ENERGY & ENVIRONMENTAL SCIENCE
(2021)
Article
Multidisciplinary Sciences
Yi Hou et al.
Review
Nanoscience & Nanotechnology
Nam-Gyu Park et al.
NATURE REVIEWS MATERIALS
(2020)
Article
Multidisciplinary Sciences
Daehan Kim et al.
Article
Multidisciplinary Sciences
Amran Al-Ashouri et al.
Review
Chemistry, Multidisciplinary
Michele De Bastiani et al.
MATERIALS HORIZONS
(2020)
Review
Nanoscience & Nanotechnology
Elizabeth M. Tennyson et al.
NATURE REVIEWS MATERIALS
(2019)
Article
Materials Science, Multidisciplinary
Esteban Rucavado et al.
PHYSICAL REVIEW MATERIALS
(2019)
Article
Energy & Fuels
Andreas Fell et al.
SOLAR ENERGY MATERIALS AND SOLAR CELLS
(2017)
Article
Nanoscience & Nanotechnology
Monica Morales-Masis et al.
ADVANCED ELECTRONIC MATERIALS
(2017)
Article
Energy & Fuels
Kevin A. Bush et al.
Review
Chemistry, Multidisciplinary
Sergio A. Paniagua et al.
Article
Energy & Fuels
Stanislau Y. Herasimenka et al.
SOLAR ENERGY MATERIALS AND SOLAR CELLS
(2016)
Article
Chemistry, Multidisciplinary
Ilja Lange et al.
ADVANCED FUNCTIONAL MATERIALS
(2014)
Article
Materials Science, Multidisciplinary
Amaury Delamarre et al.
JOURNAL OF PHOTONICS FOR ENERGY
(2012)
Article
Chemistry, Physical
Pavel B. Paramonov et al.
CHEMISTRY OF MATERIALS
(2008)