期刊
NANO LETTERS
卷 23, 期 22, 页码 10532-10537出版社
AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.3c03442
关键词
single-photon source; plasmonics; waveguide; quantum emitter; near-field
Reliable single-photon sources, high coupling efficiency, and low propagation losses are key requirements for quantum plasmonic nanocircuits. The best overall performance of these nanocircuits is achieved by adding a spacer layer between the quantum dot and the plasmonic waveguide, resulting in an improved coupling efficiency through standing wave interference.
Key requirements for quantum plasmonic nanocircuits are reliable single-photon sources, high coupling efficiency to the plasmonic structures, and low propagation losses. Self-assembled epitaxially grown GaAs quantum dots are close to ideal as stable, bright, and narrowband single-photon emitters. Likewise, wet-chemically grown monocrystalline silver nanowires are among the best plasmonic waveguides. However, large propagation losses of surface plasmons on the high-index GaAs substrate prevent their direct combination. Here, we show by experiment and simulation that the best overall performance of the quantum plasmonic nanocircuit based on these building blocks is achieved in the intermediate field regime with an additional spacer layer between the quantum dot and the plasmonic waveguide. High-resolution cathodoluminescence measurements allow a precise determination of the coupling distance and support a simple analytical model to explain the overall performance. The coupling efficiency is increased up to four times by standing wave interference near the end of the waveguide.
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