☆ 4.6 Review

Development of Different Kinds of Electrocatalyst for the Electrochemical Reduction of Carbon Dioxide Reactions: An Overview

MOLECULES (2023)

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Summary: This review summarizes the recent research progress of highly efficient electrocatalysts for the electrochemical conversion of CO2 to formic acid or formate. The focus is on nanostructured catalysts, single atom catalysts, doped or alloyed catalysts, and supported catalysts, as well as the synthetic strategies and theoretical designs to improve the Faradaic efficiency, current density, and stability of the electrochemical CO2 reduction reaction. The current challenges and further perspectives of the electrocatalysts for electrochemical CO2 reduction are also discussed.

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Summary: The increase in atmospheric CO2 concentration is a pressing issue that needs immediate resolution due to its negative impact on global warming and climate change. MXenes, with their large surface area, conductivity, abundant active sites, and high stability, are considered excellent materials for catalytic processes in CO2 reduction. This review focuses on the recent developments of MXene-based nanocomposites for electrocatalytic CO2 reduction, discussing various strategies for improving MXene performance and potential applications. The article also explores the key properties, characteristics, and plausible mechanisms of different catalysts, and provides an outlook for further development.

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Summary: Main group indium materials are found to be efficient electrocatalysts for two-electron-involved carbon dioxide reduction to produce formate. However, the synthesis of 2D monometallic nonlayered indium remains challenging. In this study, a facile electrochemical reduction strategy is introduced to transform 2D indium coordination polymer into elemental indium nanosheets. The reconstructed metallic indium exhibits high Faradaic efficiency for formate, with excellent catalytic performance attributed to the enhanced exposure of active sites and mass/charge transport at the triple-phase interface and the restrained electrolyte flooding.

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Simultaneous Electrocatalytic CO2 Reduction and Enhanced Electrochromic Effect at WO3 Nanostructured Electrodes in Acetonitrile

Nestor E. Mendieta-Reyes et al.

ACS CATALYSIS (2018)

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Review Chemistry, Physical

Tunable porous carbon spheres for high-performance rechargeable batteries

Huajun Tian et al.

JOURNAL OF MATERIALS CHEMISTRY A (2018)

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Article Chemistry, Physical

The Predominance of Hydrogen Evolution on Transition Metal Sulfides and Phosphides under CO2 Reduction Conditions: An Experimental and Theoretical Study

Alan T. Landers et al.

ACS ENERGY LETTERS (2018)

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Article Nanoscience & Nanotechnology

Boosting CH3OH Production in Electrocatalytic CO2 Reduction over Partially Oxidized 5 nm Cobalt Nanoparticles Dispersed on Single-Layer Nitrogen-Doped Graphene

Jianzhi Huang et al.

ACS APPLIED MATERIALS & INTERFACES (2018)

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Review Nanoscience & Nanotechnology

Platinum-Based Catalysts on Various Carbon Supports and Conducting Polymers for Direct Methanol Fuel Cell Applications: a Review

Z. A. C. Ramli et al.

NANOSCALE RESEARCH LETTERS (2018)

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Article Chemistry, Multidisciplinary

A Review on Recent Advances for Electrochemical Reduction of Carbon Dioxide to Methanol Using Metal-Organic Framework (MOF) and Non-MOF Catalysts: Challenges and Future Prospects

Fayez Nasir Al-Rowaili et al.

ACS SUSTAINABLE CHEMISTRY & ENGINEERING (2018)

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Article Chemistry, Multidisciplinary

Efficient solar-driven electrochemical CO2 reduction to hydrocarbons and oxygenates

Gurudayal et al.

ENERGY & ENVIRONMENTAL SCIENCE (2017)

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Article Engineering, Environmental

Carbon Capture and Utilization in the Industrial Sector

Peter C. Psarras et al.

ENVIRONMENTAL SCIENCE & TECHNOLOGY (2017)

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Article Chemistry, Physical

Surface-Morphology-Dependent Electrolyte Effects on Gold-Catalyzed Electrochemical CO2 Reduction

Haeri Kim et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2017)

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Article Chemistry, Physical

Carbon Solving Carbon's Problems: Recent Progress of Nanostructured Carbon-Based Catalysts for the Electrochemical Reduction of CO2

Anthony Vasileff et al.

ADVANCED ENERGY MATERIALS (2017)

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Article Multidisciplinary Sciences

Unique copper and reduced graphene oxide nanocomposite toward the efficient electrochemical reduction of carbon dioxide

M. Nur Hossain et al.

SCIENTIFIC REPORTS (2017)

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Article Chemistry, Physical

Nitrogen-containing polymers as a platform for CO2 electroreduction

Sathish Ponnurangam et al.

ADVANCES IN COLLOID AND INTERFACE SCIENCE (2017)

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Article Chemistry, Multidisciplinary

Li Electrochemical Tuning of Metal Oxide for Highly Selective CO2 Reduction

Kun Jiang et al.

ACS NANO (2017)

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Review Chemistry, Inorganic & Nuclear

Carbon dioxide reduction with homogenous early transition metal complexes: Opportunities and challenges for developing CO2 catalysis

Kyle A. Grice

COORDINATION CHEMISTRY REVIEWS (2017)

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Article Chemistry, Analytical

Nanocarbon Electrochemistry and Electroanalysis: Current Status and Future Perspectives

Nianjun Yang et al.

ELECTROANALYSIS (2016)

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Article Chemistry, Physical

Trace Levels of Copper in Carbon Materials Show Significant Electrochemical CO2 Reduction Activity

Yanwei Lum et al.

ACS CATALYSIS (2016)

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Article Chemistry, Physical

Simultaneous electrocatalytic reduction of dinitrogen and carbon dioxide on conducting polymer electrodes

Didem Balun Kayan et al.

APPLIED CATALYSIS B-ENVIRONMENTAL (2016)

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Article Electrochemistry

Nitrogen and Sulfur Dual-Doped Carbon Microtubes with Enhanced Performances for Oxygen Reduction Reaction

Libo Deng et al.

JOURNAL OF THE ELECTROCHEMICAL SOCIETY (2016)

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Article Chemistry, Physical

Electrochemical Reduction of Carbon Dioxide to Ethane Using Nanostructured Cu2O-Derived Copper Catalyst and Palladium(II) Chloride

Chung Shou Chen et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2015)

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Article Chemistry, Multidisciplinary

Metal-Organic Frameworks for Electrocatalytic Reduction of Carbon Dioxide

Nikolay Kornienko et al.

JOURNAL OF THE AMERICAN CHEMICAL SOCIETY (2015)

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Article Chemistry, Physical

Selective Electrochemical Reduction of Carbon Dioxide to Ethylene and Ethanol on Copper(I) Oxide Catalysts

Dan Ren et al.

ACS CATALYSIS (2015)

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Review Chemistry, Multidisciplinary

Structure, Function, and Mechanism of the Nickel Metalloenzymes, CO Dehydrogenase, and Acetyl-CoA Synthase

Mehmet Can et al.

CHEMICAL REVIEWS (2014)

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Article Chemistry, Multidisciplinary

Direct Reduction of Carbon Dioxide to Formate in High-Gas-Capacity Ionic Liquids at Post-Transition-Metal Electrodes

John D. Watkins et al.

CHEMSUSCHEM (2014)

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Article Chemistry, Physical

Recent advances of doped carbon as non-precious catalysts for oxygen reduction reaction

Hao Shi et al.

JOURNAL OF MATERIALS CHEMISTRY A (2014)

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Article Multidisciplinary Sciences

Renewable and metal-free carbon nanofibre catalysts for carbon dioxide reduction

Bijandra Kumar et al.

NATURE COMMUNICATIONS (2013)

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Review Multidisciplinary Sciences

Opportunities and challenges for a sustainable energy future

Steven Chu et al.

NATURE (2012)

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Article Chemistry, Physical

Cobalt-Porphyrin Catalyzed Electrochemical Reduction of Carbon Dioxide in Water. 1. A Density Functional Study of Intermediates

Ida M. B. Nielsen et al.

JOURNAL OF PHYSICAL CHEMISTRY A (2010)

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Article Chemistry, Physical

Development of an Amperometric Cholesterol Biosensor Based on Graphene-Pt Nanoparticle Hybrid Material

Ramendra Sundar Dey et al.

JOURNAL OF PHYSICAL CHEMISTRY C (2010)

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Article Multidisciplinary Sciences

Large-scale pattern growth of graphene films for stretchable transparent electrodes

Keun Soo Kim et al.

NATURE (2009)

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Review Chemistry, Multidisciplinary

Advanced carbon electrode materials for molecular electrochemistry

Richard L. McCreery

CHEMICAL REVIEWS (2008)

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Article Chemistry, Multidisciplinary

Graphene-Based Ultracapacitors

Meryl D. Stoller et al.

NANO LETTERS (2008)

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Article Multidisciplinary Sciences

Contributions to accelerating atmospheric CO2 growth from economic activity, carbon intensity, and efficiency of natural sinks

Josep G. Canadell et al.

PROCEEDINGS OF THE NATIONAL ACADEMY OF SCIENCES OF THE UNITED STATES OF AMERICA (2007)

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Article Multidisciplinary Sciences

Electronic confinement and coherence in patterned epitaxial graphene

Claire Berger et al.

SCIENCE (2006)

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Article Multidisciplinary Sciences

Experimental observation of the quantum Hall effect and Berry's phase in graphene

YB Zhang et al.

NATURE (2005)

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Article Chemistry, Inorganic & Nuclear

Single-Atom Catalysts Supported on the Graphene/Graphdiyne Heterostructure for Effective CO2 Electroreduction

Yun Yang et al.

Summary: Through density functional theory calculations, this study found that the transition metal single-atom catalyst Co-N-4@GRA/GDY anchored on nitrogen-doped graphene/graphdiyne heterostructure exhibits remarkable activity for CO2 reduction reaction, providing a potential avenue for improving catalytic performance and accelerating CO2RR.

INORGANIC CHEMISTRY

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